39 research outputs found
The Hahn Quantum Variational Calculus
We introduce the Hahn quantum variational calculus. Necessary and sufficient
optimality conditions for the basic, isoperimetric, and Hahn quantum Lagrange
problems, are studied. We also show the validity of Leitmann's direct method
for the Hahn quantum variational calculus, and give explicit solutions to some
concrete problems. To illustrate the results, we provide several examples and
discuss a quantum version of the well known Ramsey model of economics.Comment: Submitted: 3/March/2010; 4th revision: 9/June/2010; accepted:
18/June/2010; for publication in Journal of Optimization Theory and
Application
Dislocation-induced spin tunneling in Mn-12 acetate
Comprehensive theory of quantum spin relaxation in Mn-12 acetate crystals is
developed, that takes into account imperfections of the crystal structure and
is based upon the generalization of the Landau-Zener effect for incoherent
tunneling from excited energy levels. It is shown that linear dislocations at
plausible concentrations provide the transverse anisotropy which is the main
source of tunneling in Mn-12. Local rotations of the easy axis due to
dislocations result in a transverse magnetic field generated by the field
applied along the c-axis of the crystal, which explains the presence of odd
tunneling resonances. Long-range deformations due to dislocations produce a
broad distribution of tunnel splittings. The theory predicts that at subkelvin
temperatures the relaxation curves for different tunneling resonances can be
scaled onto a single master curve. The magnetic relaxation in the thermally
activated regime follows the stretched-exponential law with the exponent
depending on the field, temperature, and concentration of defects.Comment: 17 pages, 14 figures, 1 table, submitted to PR
Effect of initial conditions on the speed of reaction-diffusion fronts
The effect of initial conditions on the speed of propagating fronts in reaction-diffusion equations is examined in the framework of the Hamilton-Jacobi theory. We study the transition between quenched and nonquenched fronts both analytically and numerically for parabolic and hyperbolic reaction diffusion. Nonhomogeneous media are also analyzed and the effect of algebraic initial conditions is also discussed
Spin dynamics of Mn12-acetate in the thermally-activated tunneling regime: ac-susceptibility and magnetization relaxation
In this work, we study the spin dynamics of Mn12-acetate molecules in the
regime of thermally assisted tunneling. In particular, we describe the system
in the presence of a strong transverse magnetic field. Similar to recent
experiments, the relaxation time/rate is found to display a series of
resonances; their Lorentzian shape is found to stem from the tunneling. The
dynamic susceptibility is calculated starting from the microscopic
Hamiltonian and the resonant structure manifests itself also in .
Similar to recent results reported on another molecular magnet, Fe8, we find
oscillations of the relaxation rate as a function of the transverse magnetic
field when the field is directed along a hard axis of the molecules. This
phenomenon is attributed to the interference of the geometrical or Berry phase.
We propose susceptibility experiments to be carried out for strong transverse
magnetic fields to study of these oscillations and for a better resolution of
the sharp satellite peaks in the relaxation rates.Comment: 22 pages, 23 figures; submitted to Phys. Rev. B; citations/references
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Effect of local Coulomb interactions on the electronic structure and exchange interactions in Mn12 magnetic molecules
We have studied the effect of local Coulomb interactions on the electronic
structure of the molecular magnet Mn12-acetate within the LDA+U approach. The
account of the on-site repulsion results in a finite energy gap and an integer
value of the molecule's magnetic moment, both quantities being in a good
agreement with the experimental results. The resulting magnetic moments and
charge states of non-equivalent manganese ions agree very well with
experiments. The calculated values of the intramolecular exchange parameters
depend on the molecule's spin configuration, differing by 25-30% between the
ferrimagnetic ground state and the completely ferromagnetic configurations. The
values of the ground-state exchange coupling parameters are in reasonable
agreement with the recent data on the magnetization jumps in megagauss magnetic
fields. Simple estimates show that the obtained exchange parameters can be
applied, at least qualitatively, to the description of the spin excitations in
Mn12-acetate.Comment: RevTeX, LaTeX2e, 4 EPS figure