470 research outputs found
Determination of reaction rate constants and T-2 relaxation times using integrated NMR power spectra
Parity Effects in Stacked Nanoscopic Quantum Rings
The ground state and the dielectric response of stacked quantum rings are
investigated in the presence of an applied magnetic field along the ring axis.
For odd number of rings and an electric field perpendicular to the axis, a
linear Stark effect occurs at distinct values of the magnetic field. At those
fields energy levels cross in the absence of electric field. For even values of
a quadratic Stark effect is expected in all cases, but the induced electric
polarization is discontinuous at those special magnetic fields. Experimental
consequences for related nanostructures are discussed.Comment: typos corrected, to appear Phys. Rev. B (Rapid Communication) 15 Au
Effect of a zero g environment on flammability limits as determined using a standard flammability tube apparatus
Flammability limits in a zero gravity environment were defined. Key aspects of a possible spacelab experiment were investigated analytically, experimentally on the bench, and in drop tower facilities. A conceptual design for a spacelab experiment was developed
Effect of Nuclear Quadrupole Interaction on the Relaxation in Amorphous Solids
Recently it has been experimentally demonstrated that certain glasses display
an unexpected magnetic field dependence of the dielectric constant. In
particular, the echo technique experiments have shown that the echo amplitude
depends on the magnetic field. The analysis of these experiments results in the
conclusion that the effect seems to be related to the nuclear degrees of
freedom of tunneling systems. The interactions of a nuclear quadrupole
electrical moment with the crystal field and of a nuclear magnetic moment with
magnetic field transform the two-level tunneling systems inherent in amorphous
dielectrics into many-level tunneling systems. The fact that these features
show up at temperatures , where the properties of amorphous materials
are governed by the long-range interaction between tunneling systems,
suggests that this interaction is responsible for the magnetic field dependent
relaxation. We have developed a theory of many-body relaxation in an ensemble
of interacting many-level tunneling systems and show that the relaxation rate
is controlled by the magnetic field. The results obtained correlate with the
available experimental data. Our approach strongly supports the idea that the
nuclear quadrupole interaction is just the key for understanding the unusual
behavior of glasses in a magnetic field.Comment: 18 pages, 9 figure
Correlated Persistent Tunneling Currents in Glasses
Low temperature properties of glasses are derived within a generalized
tunneling model, considering the motion of charged particles on a closed path
in a double-well potential. The presence of a magnetic induction field B
violates the time reversal invariance due to the Aharonov-Bohm phase, and leads
to flux periodic energy levels. At low temperature, this effect is shown to be
strongly enhanced by dipole-dipole and elastic interactions between tunneling
systems and becomes measurable. Thus, the recently observed strong sensitivity
of the electric permittivity to weak magnetic fields can be explained. In
addition, superimposed oscillations as a function of the magnetic field are
predicted.Comment: 4 page
Magnetic field effect on the dielectric constant of glasses: Evidence of disorder within tunneling barriers
The magnetic field dependence of the low frequency dielectric constant
(H) of a structural glass a - SiO2 + xCyHz was studied from 400 mK to 50
mK and for H up to 3T. Measurement of both the real and the imaginary parts of
is used to eliminate the difficult question of keeping constant the
temperature of the sample while increasing H: a non-zero (H) dependence is
reported in the same range as that one very recently reported on multicomponent
glasses. In addition to the recently proposed explanation based on
interactions, the reported (H) is interpreted quantitatively as a
consequence of the disorder lying within the nanometric barriers of the
elementary tunneling systems of the glass.Comment: latex Bcorrige1.tex, 5 files, 4 figures, 7 pages [SPEC-S02/009
Low temperature acoustic properties of amorphous silica and the Tunneling Model
Internal friction and speed of sound of a-SiO(2) was measured above 6 mK
using a torsional oscillator at 90 kHz, controlling for thermal decoupling,
non-linear effects, and clamping losses. Strain amplitudes e(A) = 10^{-8} mark
the transition between the linear and non-linear regime. In the linear regime,
excellent agreement with the Tunneling Model was observed for both the internal
friction and speed of sound, with a cut-off energy of E(min) = 6.6 mK. In the
non-linear regime, two different behaviors were observed. Above 10 mK the
behavior was typical for non-linear harmonic oscillators, while below 10 mK a
different behavior was found. Its origin is not understood.Comment: 1 tex file, 6 figure
Linear stability of planar premixed flames: reactive Navier-Stokes equations with finite activation energy and arbitrary Lewis number
A numerical shooting method for performing linear stability analyses of travelling waves is described and applied to the problem of freely propagating planar premixed flames. Previous linear stability analyses of premixed flames either employ high activation temperature asymptotics or have been performed numerically with finite activation temperature, but either for unit Lewis numbers (which ignores thermal-diffusive effects) or in the limit of small heat release (which ignores hydrodynamic effects). In this paper the full reactive Navier-Stokes equations are used with arbitrary values of the parameters (activation temperature, Lewis number, heat of reaction, Prandtl number), for which both thermal-diffusive and hydrodynamic effects on the instability, and their interactions, are taken into account. Comparisons are made with previous asymptotic and numerical results. For Lewis numbers very close to or above unity, for which hydrodynamic effects caused by thermal expansion are the dominant destablizing mechanism, it is shown that slowly varying flame analyses give qualitatively good but quantitatively poor predictions, and also that the stability is insensitive to the activation temperature. However, for Lewis numbers sufficiently below unity for which thermal-diffusive effects play a major role, the stability of the flame becomes very sensitive to the activation temperature. Indeed, unphysically high activation temperatures are required for the high activation temperature analysis to give quantitatively good predictions at such low Lewis numbers. It is also shown that state-insensitive viscosity has a small destabilizing effect on the cellular instability at low Lewis numbers
Anomalous magnetic noise in an imperfectly flat landscape in the topological magnet Dy2Ti2O7.
Noise generated by motion of charge and spin provides a unique window into materials at the atomic scale. From temperature of resistors to electrons breaking into fractional quasiparticles, "listening" to the noise spectrum is a powerful way to decode underlying dynamics. Here, we use ultrasensitive superconducting quantum interference device (SQUIDs) to probe the puzzling noise in a frustrated magnet, the spin-ice compound Dy2Ti2O7 (DTO), revealing cooperative and memory effects. DTO is a topological magnet in three dimensions-characterized by emergent magnetostatics and telltale fractionalized magnetic monopole quasiparticles-whose real-time dynamical properties have been an enigma from the very beginning. We show that DTO exhibits highly anomalous noise spectra, differing significantly from the expected Brownian noise of monopole random walks, in three qualitatively different regimes: equilibrium spin ice, a "frozen" regime extending to ultralow temperatures, and a high-temperature "anomalous" paramagnet. We present several distinct mechanisms that give rise to varied colored noise spectra. In addition, we identify the structure of the local spin-flip dynamics as a crucial ingredient for any modeling. Thus, the dynamics of spin ice reflects the interplay of local dynamics with emergent topological degrees of freedom and a frustration-generated imperfectly flat energy landscape, and as such, it points to intriguing cooperative and memory effects for a broad class of magnetic materials
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