268 research outputs found
Statistics of low-energy levels of a one-dimensional weakly localized Frenkel exciton: A numerical study
Numerical study of the one-dimensional Frenkel Hamiltonian with on-site
randomness is carried out. We focus on the statistics of the energy levels near
the lower exciton band edge, i. e. those determining optical response. We found
that the distribution of the energy spacing between the states that are well
localized at the same segment is characterized by non-zero mean, i.e. these
states undergo repulsion. This repulsion results in a local discrete energy
structure of a localized Frenkel exciton. On the contrary, the energy spacing
distribution for weakly overlapping local ground states (the states with no
nodes within their localization segments) that are localized at different
segments has zero mean and shows almost no repulsion. The typical width of the
latter distribution is of the same order as the typical spacing in the local
discrete energy structure, so that this local structure is hidden; it does not
reveal itself neither in the density of states nor in the linear absorption
spectra. However, this structure affects the two-exciton transitions involving
the states of the same segment and can be observed by the pump-probe
spectroscopy. We analyze also the disorder degree scaling of the first and
second momenta of the distributions.Comment: 10 pages, 6 figure
Magnetic Resonance of the Intrinsic Defects of the Spin-Peierls Magnet CuGeO3
ESR of the pure monocrystals of CuGeO3 is studied in the frequency range 9-75
GHz and in the temperature interval 1.2-25 K. The splitting of the ESR line
into several spectral components is observed below 5 K, in the temperature
range where the magnetic susceptibility is suppressed by the spin-Peierls
dimerization. The analysis of the magnetic resonance signals allows one to
separate the signals of the S=1/2- and S=1 defects of the spin-Peierls phase.
The value of g-factor of these signals is close to that of the Cu-ion. The
additional line of the magnetic resonance is characterized by an anomalous
value of the g-factor and by the threshold-like increase of the microwave
susceptibility when the microwave power is increasing. The ESR signals are
supposingly attributed to two types of the planar magnetic defects, arising at
the boundaries of the domains of the spin-Peierls state with the different
values of the phase of the dimerization.Comment: LATEX-text, 12 PS-figures, typos corrected, LATEX-style change
Separation of the magnetic phases at the N\'{e}el point in the diluted spin-Peierls magnet CuGeO3
The impurity induced antiferromagnetic ordering of the doped spin-Peierls
magnet Cu(1-x)Mg(x)GeO(3) was studied by ESR technique. Crystals with the Mg
concentration x<4% demonstrate a coexistence of paramagnetic and
antiferromagnetic ESR modes. This coexistence indicates the separation of a
macroscopically uniform sample in the paramagnetic and antiferromagnetic
phases. In the presence of the long-range spin-Peierls order (in a sample with
x=1.71%) the volume of the antiferromagnetic phase immediately below the
N\'{e}el point T_N is much smaller than the volume of the paramagnetic phase.
In the presence of the short-range spin-Peierls order (in samples with x=2.88%,
x= 3.2%) there are comparable volumes of paramagnetic and antiferromagnetic
phases at T=T_N. The fraction of the antiferromagnetic phase increases with
lowering temperature. In the absence of the spin-Peierls dimerization (at
x=4.57%)the whole sample exhibits the transition into the antiferromagnetic
state and there is no phase separation. The phase separation is explained by
the consideration of clusters of staggered magnetization located near impurity
atoms. In this model the areas occupied by coherently correlated spins expand
with decreasing temperature and the percolation of the ordered area through a
macroscopic distance occurs.Comment: 7pages, 10 figure
Finite strain Landau theory of high pressure phase transformations
The properties of materials near structural phase transitions are often
successfully described in the framework of Landau theory. While the focus is
usually on phase transitions, which are induced by temperature changes
approaching a critical temperature T-c, here we will discuss structural phase
transformations driven by high hydrostatic pressure, as they are of major
importance for understanding processes in the interior of the earth. Since at
very high pressures the deformations of a material are generally very large,
one needs to apply a fully nonlinear description taking physical as well as
geometrical nonlinearities (finite strains) into account. In particular it is
necessary to retune conventional Landau theory to describe such phase
transitions. In Troster et al (2002 Phys. Rev. Lett. 88 55503) we constructed a
Landau-type free energy based on an order parameter part, an order
parameter-(finite) strain coupling and a nonlinear elastic term. This model
provides an excellent and efficient framework for the systematic study of phase
transformations for a wide range of materials up to ultrahigh pressures
Clinical-pathological study on Ξ²-APP, IL-1Ξ², GFAP, NFL, SpectrinΒ II, 8OHdG, TUNEL, miR-21, miR-16, miR-92 expressions to verify DAI-diagnosis, grade and prognosis
Traumatic brain injury (TBI) is one of the most important death and disability cause, involving substantial costs, also in economic terms, when considering the young age of the involved subject. Aim of this paper is to report a series of patients treated at our institutions, to verify neurological results at six months or survival; in fatal cases we searched for Ξ²APP, GFAP, IL-1Ξ², NFL, Spectrin II, TUNEL and miR-21, miR-16, and miR-92 expressions in brain samples, to verify DAI diagnosis and grade as strong predictor of survival and inflammatory response. Concentrations of 8OHdG as measurement of oxidative stress was performed. Immunoreaction of Ξ²-APP, IL-1Ξ², GFAP, NFL, Spectrin II and 8OHdG were significantly increased in the TBI group with respect to control group subjects. Cell apoptosis, measured by TUNEL assay, were significantly higher in the study group than control cases. Results indicated that miR-21, miR-92 and miR-16 have a high predictive power in discriminating trauma brain cases from controls and could represent promising biomarkers as strong predictor of survival, and for the diagnosis of postmortem traumatic brain injury
A management algorithm for patients with intracranial pressure monitoring: the Seattle International Severe Traumatic Brain Injury Consensus Conference (SIBICC).
BACKGROUND: Management algorithms for adult severe traumatic brain injury (sTBI) were omitted in later editions of the Brain Trauma Foundation's sTBI Management Guidelines, as they were not evidence-based. METHODS: We used a Delphi-method-based consensus approach to address management of sTBI patients undergoing intracranial pressure (ICP) monitoring. Forty-two experienced, clinically active sTBI specialists from six continents comprised the panel. Eight surveys iterated queries and comments. An in-person meeting included whole- and small-group discussions and blinded voting. Consensus required 80% agreement. We developed heatmaps based on a traffic-light model where panelists' decision tendencies were the focus of recommendations. RESULTS: We provide comprehensive algorithms for ICP-monitor-based adult sTBI management. Consensus established 18 interventions as fundamental and ten treatments not to be used. We provide a three-tier algorithm for treating elevated ICP. Treatments within a tier are considered empirically equivalent. Higher tiers involve higher risk therapies. Tiers 1, 2, and 3 include 10, 4, and 3 interventions, respectively. We include inter-tier considerations, and recommendations for critical neuroworsening to assist the recognition and treatment of declining patients. Novel elements include guidance for autoregulation-based ICP treatment based on MAP Challenge results, and two heatmaps to guide (1) ICP-monitor removal and (2) consideration of sedation holidays for neurological examination. CONCLUSIONS: Our modern and comprehensive sTBI-management protocol is designed to assist clinicians managing sTBI patients monitored with ICP-monitors alone. Consensus-based (class III evidence), it provides management recommendations based on combined expert opinion. It reflects neither a standard-of-care nor a substitute for thoughtful individualized management
The Founderβs Lecture 2009: advances in imaging of osteoporosis and osteoarthritis
The objective of this review article is to provide an update on new developments in imaging of osteoporosis and osteoarthritis over the past three decades. A literature review is presented that summarizes the highlights in the development of bone mineral density measurements, bone structure imaging, and vertebral fracture assessment in osteoporosis as well as MR-based semiquantitative assessment of osteoarthritis and quantitative cartilage matrix imaging. This review focuses on techniques that have impacted patient management and therapeutic decision making or that potentially will affect patient care in the near future. Results of pertinent studies are presented and used for illustration. In summary, novel developments have significantly impacted imaging of osteoporosis and osteoarthritis over the past three decades
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