3,293 research outputs found
Cs adsorption on Si(001) surface: ab initio study
First-principles calculations using density functional theory based on
norm-conserving pseudopotentials have been performed to investigate the Cs
adsorption on the Si(001) surface for 0.5 and 1 ML coverages. We found that the
saturation coverage corresponds to 1 ML adsorption with two Cs atoms occupying
the double layer model sites. While the 0.5 ML covered surface is of metallic
nature, we found that 1 ML of Cs adsorption corresponds to saturation coverage
and leads to a semiconducting surface. The results for the electronic behavior
and surface work function suggest that adsorption of Cs takes place via
polarized covalent bonding.Comment: 8 pages, 7 figure
Collider design issues based on proton-driven plasma wakefield acceleration
Recent simulations have shown that a high-energy proton bunch can excite
strong plasma wakefields and accelerate a bunch of electrons to the energy
frontier in a single stage of acceleration. It therefore paves the way towards
a compact future collider design using the proton beams from existing
high-energy proton machines, e.g. Tevatron or the LHC. This paper addresses
some key issues in designing a compact electron-positron linear collider and an
electron-proton collider based on existing CERN accelerator infrastructure
A plasma wakefield acceleration experiment using CLARA beam
We propose a Plasma Accelerator Research Station (PARS) based at proposed FEL
test facility CLARA (Compact Linear Accelerator for Research and Applications)
at Daresbury Laboratory. The idea is to use the relativistic electron beam from
CLARA, to investigate some key issues in electron beam transport and in
electron beam driven plasma wakefield acceleration, e.g. high gradient plasma
wakefield excitation driven by a relativistic electron bunch, two bunch
experiment for CLARA beam energy doubling, high transformer ratio, long bunch
self-modulation and some other advanced beam dynamics issues. This paper
presents the feasibility studies of electron beam transport to meet the
requirements for beam driven wakefield acceleration and presents the plasma
wakefield simulation results based on CLARA beam parameters. Other possible
experiments which can be conducted at the PARS beam line are also discussed
Influence of steps on the tilting and adsorption dynamics of ordered Pn films on vicinal Ag(111) surfaces
Here we present a structural study of pentacene (Pn) thin films on vicinal
Ag(111) surfaces by He atom diffraction measurements and density functional
theory (DFT) calculations supplemented with van der Waals (vdW) interactions.
Our He atom diffraction results suggest initial adsorption at the step edges
evidenced by initial slow specular reflection intensity decay rate as a
function of Pn deposition time. In parallel with the experimental findings, our
DFT+vdW calculations predict the step edges as the most stable adsorption site
on the surface. An isolated molecule adsorbs as tilted on the step edge with a
binding energy of 1.4 eV. In addition, a complete monolayer (ML) with
pentacenes flat on the terraces and tilted only at the step edges is found to
be more stable than one with all lying flat or tilted molecules, which in turn
influences multilayers. Hence our results suggest that step edges can trap Pn
molecules and act as nucleation sites for the growth of ordered thin films with
a crystal structure similar to that of bulk Pn.Comment: 4 pages, 4 figures, 1 tabl
Counter-propagating entangled photons from a waveguide with periodic nonlinearity
The conditions required for spontaneous parametric down-conversion in a
waveguide with periodic nonlinearity in the presence of an unguided pump field
are established. Control of the periodic nonlinearity and the physical
properties of the waveguide permits the quasi-phase matching equations that
describe counter-propagating guided signal and idler beams to be satisfied. We
compare the tuning curves and spectral properties of such counter-propagating
beams to those for co-propagating beams under typical experimental conditions.
We find that the counter-propagating beams exhibit narrow bandwidth permitting
the generation of quantum states that possess discrete-frequency entanglement.
Such states may be useful for experiments in quantum optics and technologies
that benefit from frequency entanglement.Comment: submitted to Phys. Rev.
The Design and Cytotoxic Evaluation of Some 1-Aryl-3- isopropylamino-1-propanone Hydrochlorides towards Human Huh-7 Hepatoma Cells
Cataloged from PDF version of article.A series of 1-aryl-3-isopropylamino-1-propanone hydrochlorides 1 and a related heterocyclic analog 2 as candidate antineoplastic agents were prepared and the rationale for designing these compounds is presented. A specific objective in this study is the discovery of novel compounds possessing growth-inhibiting properties of hepatoma cells. The compounds in series 1 and 2 were prepared and their structures established unequivocally. X-ray crystallography of two representative compounds 1d and 1g were achieved. Over half of the compounds are more potent than 5-fluorouracil which is an established drug used in treating liver cancers. QSAR evaluations and molecular modeling studies were undertaken with a view to detecting some physicochemical parameters which govern cytotoxic potencies. A number of guidelines for amplification of the project have been formulated. A number of Mannich bases displayed greater potency than the reference drug 5-fluorouracil against human Huh-7 hepatoma cells. In particular, 1i emerged as a lead compound possessing 2.8 fold higher activity than that of the reference drug. Copyright © 2011 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim
Multi-Parameter Entanglement in Femtosecond Parametric Down-Conversion
A theory of spontaneous parametric down-conversion, which gives rise to a
quantum state that is entangled in multiple parameters, such as
three-dimensional wavevector and polarization, allows us to understand the
unusual characteristics of fourth-order quantum interference in many
experiments, including ultrafast type-II parametric down-conversion, the
specific example illustrated in this paper. The comprehensive approach provided
here permits the engineering of quantum states suitable for quantum information
schemes and new quantum technologies.Comment: to appear in Physical Review
The electron accelerator for the AWAKE experiment at CERN
The AWAKE collaboration prepares a proton driven plasma wakefield acceleration experiment using the SPS beam at CERN. A long proton bunch extracted from the SPS interacts with a high power laser and a 10 m long rubidium vapour plasma cell to create strong wakefields allowing sustained electron acceleration. The electron bunch to probe these wakefields is supplied by a 20 MeV electron accelerator. The electron accelerator consists of an RF-gun and a short booster structure. This electron source should provide beams with intensities between 0.1 and 1 nC, bunch lengths between 0.3 and 3 ps and an emittance of the order of 2 mm mrad. The wide range of parameters should cope with the uncertainties and future prospects of the planned experiments. The layout of the electron accelerator, its instrumentation and beam dynamics simulations are presented
Large-scale quantum-emitter arrays in atomically thin semiconductors.
Quantum light emitters have been observed in atomically thin layers of transition metal dichalcogenides. However, they are found at random locations within the host material and usually in low densities, hindering experiments aiming to investigate this new class of emitters. Here, we create deterministic arrays of hundreds of quantum emitters in tungsten diselenide and tungsten disulphide monolayers, emitting across a range of wavelengths in the visible spectrum (610-680 nm and 740-820 nm), with a greater spectral stability than their randomly occurring counterparts. This is achieved by depositing monolayers onto silica substrates nanopatterned with arrays of 150-nm-diameter pillars ranging from 60 to 190 nm in height. The nanopillars create localized deformations in the material resulting in the quantum confinement of excitons. Our method may enable the placement of emitters in photonic structures such as optical waveguides in a scalable way, where precise and accurate positioning is paramount
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