503 research outputs found
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Direct measurement of Coulomb-laser coupling
The Coulomb interaction between a photoelectron and its parent ion plays an important role in a large range of light-matter interactions. In this paper we obtain a direct insight into the Coulomb interaction and resolve, for the first time, the phase accumulated by the laser-driven electron as it interacts with the Coulomb potential. Applying extreme-ultraviolet interferometry enables us to resolve this phase with attosecond precision over a large energy range. Our findings identify a strong laser-Coulomb coupling, going beyond the standard recollision picture within the strong-field framework. Transformation of the results to the time domain reveals Coulomb-induced delays of the electrons along their trajectories, which vary by tens of attoseconds with the laser field intensity
Studying the universality of field induced tunnel ionization times via high-order harmonic spectroscopy
High-harmonics generation spectroscopy is a promising tool for resolving
electron dynamics and structure in atomic and molecular systems. This scheme,
commonly described by the strong field approximation, requires a deep insight
into the basic mechanism that leads to the harmonics generation. Recently, we
have demonstrated the ability to resolve the first stage of the process --
field induced tunnel ionization -- by adding a weak perturbation to the strong
fundamental field. Here we generalize this approach and show that the
assumptions behind the strong field approximation are valid over a wide range
of tunnel ionization conditions. Performing a systematic study -- modifying the
fundamental wavelength, intensity and atomic system -- we observed a good
agreement with quantum path analysis over a range of Keldysh parameters. The
generality of this scheme opens new perspectives in high harmonics
spectroscopy, holding the potential of probing large, complex molecular
systems.Comment: 11 pages, 5 figure
Quantum Control of Photodissociation via Manipulation of Bond Softening
We present a method to control photodissociation by manipulating the bond
softening mechanism occurring in strong shaped laser fields, by varying the
chirp sign and magnitude of an ultra-short laser pulse. Manipulation of
bond-softening is experimentally demonstrated for strong field (795 nm, 10^12 -
10^13 W/cm^2) photodissociation of H2+, exhibiting substantial increase of
dissociation by positively chirped pulses with respect to both negatively
chirped and transform limited pulses. The measured kinetic energy release and
angular distributions are used to quantify the degree of control of
dissociation. The control mechanism is attributed to the interplay of dynamic
alignment and chirped light induced potential curves.Comment: 4 pages, 4 figure
Observation of light driven band structure via multi-band high harmonic spectroscopy
Intense light-matter interactions have revolutionized our ability to probe
and manipulate quantum systems at sub-femtosecond time scales, opening routes
to all-optical control of electronic currents in solids at petahertz rates.
Such control typically requires electric field amplitudes , when
the voltage drop across a lattice site becomes comparable to the characteristic
band gap energies. In this regime, intense light-matter interaction induces
significant modifications of electronic and optical properties, dramatically
modifying the crystal band structure. Yet, identifying and characterizing such
modifications remains an outstanding problem. As the oscillating electric field
changes within the driving field's cycle, does the band-structure follow, and
how can it be defined? Here we address this fundamental question, proposing
all-optical spectroscopy to probe laser-induced closing of the band-gap between
adjacent conduction bands. Our work reveals the link between nonlinear light
matter interactions in strongly driven crystals and the sub-cycle modifications
in their effective band structure
Profession Based Hierarchies as Barriers for Genuine Learning Processes
Under embargo until: 2021-06-26This chapter describes how profession based hierarchies (stratified social orders between professions) may appear in a teaching context of interprofessionality involving a variety of health professions presenting challenges to learning and offers suggestions on how these challenges can be overcome.acceptedVersio
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Multidimensional high harmonic spectroscopy of polyatomic molecules: detecting sub-cycle laser-driven hole dynamics upon ionization in strong mid-IR laser fields
High harmonic generation (HHG) spectroscopy has opened up a new frontier in ultrafast science, where electronic dynamics can be measured on an attosecond time scale. The strong laser field that triggers the high harmonic response also opens multiple quantum pathways for multielectron dynamics in molecules, resulting in a complex process of multielectron rearrangement during ionization. Using combined experimental and theoretical approaches, we show how multi-dimensional HHG spectroscopy can be used to detect and follow electronic dynamics of core rearrangement on sub-laser cycle time scales. We detect the signatures of laser-driven hole dynamics upon ionization and reconstruct the relative phases and amplitudes for relevant ionization channels in a CO2 molecule on a sub-cycle time scale. Reconstruction of channel-resolved complex ionization amplitudes on attosecond time scales has been a long-standing goal of high harmonic spectroscopy. Our study brings us one step closer to fulfilling this initial promise and developing robust schemes for sub-femtosecond imaging of multielectron rearrangement in complex molecular systems
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CORPORATE GOVERNANCE AND INVESTORS' PERCEPTIONS OF FOREIGN IPO VALUE: AN INSTITUTIONAL PERSPECTIVE
We build on sociology-grounded research on financial market behavior and suggest a ânestedâ legitimacy framework to explore U.S. investor perceptions of foreign IPO value. We draw on a fuzzy-set theoretic approach to demonstrate how different combinations of monitoring and incentive-based corporate governance mechanisms lead to the same level of investor valuations of firms. We also argue that institutional factors related to the minority shareholder protection strength in the foreign IPOâs home country represent a boundary condition that affects the number of governance mechanisms required to achieve U.S. investorsâ high value perceptions. Our findings, drawn from a unique, hand-collected dataset of foreign IPOs in the U.S, contribute to the sociological perspective on comparative corporate governance and the inter-dependencies between organizations and institutions
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