7,082 research outputs found
Frustrated magnetism and resonating valence bond physics in two-dimensional kagome-like magnets
We explore the phase diagram and the low-energy physics of three Heisenberg
antiferromagnets which, like the kagome lattice, are networks of corner-sharing
triangles but contain two sets of inequivalent short-distance resonance loops.
We use a combination of exact diagonalization, analytical strong-coupling
theories, and resonating valence bond approaches, and scan through the ratio of
the two inequivalent exchange couplings. In one limit, the lattices effectively
become bipartite, while at the opposite limit heavily frustrated nets emerge.
In between, competing tunneling processes result in short-ranged spin
correlations, a manifold of low-lying singlets (which can be understood as
localized bound states of magnetic excitations), and the stabilization of
valence bond crystals with resonating building blocks.Comment: Published versio
KCrF_3: Electronic Structure, Magnetic and Orbital Ordering from First Principles
The electronic, magnetic and orbital structures of KCrF_3 are determined in
all its recently identified crystallographic phases (cubic, tetragonal, and
monoclinic) with a set of {\it ab initio} LSDA and LSDA+U calculations. The
high-temperature undistorted cubic phase is metallic within the LSDA, but at
the LSDA+U level it is a Mott insulator with a gap of 1.72 eV. The tetragonal
and monoclinic phases of KCrF_3 exhibit cooperative Jahn-Teller distortions
concomitant with staggered 3x^2-r^2/3y^2-r^2 orbital order. We find that the
energy gain due to the Jahn-Teller distortion is 82/104 meV per chromium ion in
the tetragonal/monoclinic phase, respectively. These phases show A-type
magnetic ordering and have a bandgap of 2.48 eV. In this Mott insulating state
KCrF_3 has a substantial conduction bandwidth of 2.1 eV, leading to the
possibility for the kinetic energy of charge carriers in electron- or
hole-doped derivatives of KCrF_3 to overcome the polaron localization at low
temperatures, in analogy with the situation encountered in the colossal
magnetoresistive manganites.Comment: 7 pages, 11 figure
Non conventional screening of the Coulomb interaction in low dimensional and finite size system
We study the screening of the Coulomb interaction in non polar systems by
polarizable atoms. We show that in low dimensions and small finite size systems
this screening deviates strongly from that conventionally assumed. In fact in
one dimension the short range interaction is strongly screened and the long
range interaction is anti-screened thereby strongly reducing the gradient of
the Coulomb interaction and therefore the correlation effects. We argue that
this effect explains the success of mean field single particle theories for
large molecules.Comment: 4 pages, 5 figure
Spacetime Encodings II - Pictures of Integrability
I visually explore the features of geodesic orbits in arbitrary stationary
axisymmetric vacuum (SAV) spacetimes that are constructed from a complex Ernst
potential. Some of the geometric features of integrable and chaotic orbits are
highlighted. The geodesic problem for these SAV spacetimes is rewritten as a
two degree of freedom problem and the connection between current ideas in
dynamical systems and the study of two manifolds sought. The relationship
between the Hamilton-Jacobi equations, canonical transformations, constants of
motion and Killing tensors are commented on. Wherever possible I illustrate the
concepts by means of examples from general relativity. This investigation is
designed to build the readers' intuition about how integrability arises, and to
summarize some of the known facts about two degree of freedom systems. Evidence
is given, in the form of orbit-crossing structure, that geodesics in SAV
spacetimes might admit, a fourth constant of motion that is quartic in momentum
(by contrast with Kerr spacetime, where Carter's fourth constant is quadratic).Comment: 11 pages, 10 figure
Electronic Correlations in Oligo-acene and -thiophene Organic Molecular Crystals
From first principles calculations we determine the Coulomb interaction
between two holes on oligo-acene and -thiophene molecules in a crystal, as a
function of the oligomer length. The relaxation of the molecular geometry in
the presence of holes is found to be small. In contrast, the electronic
polarization of the molecules that surround the charged oligomer, reduces the
bare Coulomb repulsion between the holes by approximately a factor of two. In
all cases the effective hole-hole repulsion is much larger than the calculated
valence bandwidth, which implies that at high doping levels the properties of
these organic semiconductors are determined by electron-electron correlations.Comment: 5 pages, 3 figure
Theory for Magnetism and Triplet Superconductivity in LiFeAs
Superconducting pnictides are widely found to feature spin-singlet pairing in
the vicinity of an antiferromagnetic phase, for which nesting between electron
and hole Fermi surfaces is crucial. LiFeAs differs from the other pnictides by
(i) poor nesting properties and (ii) unusually shallow hole pockets.
Investigating magnetic and pairing instabilities in an electronic model that
incorporates these differences, we find antiferromagnetic order to be absent.
Instead we observe almost ferromagnetic fluctuations which drive an instability
toward spin-triplet p-wave superconductivity.Comment: Published versio
A Potts model for the distortion transition in LaMnO
The Jahn-Teller distortive transition of \lmo is described by a modified
3-state Potts model. The interactions between the three possible orbits depends
both on the orbits and their relative orientation on the lattice. Values of the
two exchange parameters which are chosen to give the correct low temperature
phase and the correct value for the transition temperature are shown to be
consistent with microscopy theory. The model predicts a first order transitions
and also a value for the entropy above the transition in good agreement with
experiment. The theory with the same parameters also predicts the temperature
dependence of the order parameter of orbital ordering agreeing well with
published experimental results. Finally, the type of the transition is shown to
be close to one of the most disordered phases of the generalised Potts model.
The short range order found experimentally above the transition is investigated
by this model.Comment: 16 pages, 7 figures and no tables. Re-submitted to Phys. Rev.
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