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Polarization control at the microscopic and electronic structure observatory
The new Microscopic and Electronic Structure Observatory (MAESTRO) at the Advanced Light Source (ALS) in Berkeley provides X-rays of variable polarization, produced by an elliptically polarized undulator (EPU), for angle resolved photoemission (ARPES) and photoemission electron microscopy (PEEM) experiments. The interpretation of photoemission data, in particular of dichroism effects in ARPES, requires the precise knowledge of the exact polarization state. Numerical simulations show that the first harmonics of the EPU at MAESTRO provides soft X-rays of almost 100% on axis polarization. However, the higher harmonics as well as the downstream optical elements of the beamline, have a considerable impact on the polarization of the light delivered to the experimental end-station. Employing a simple reflective polarimeter, the polarization is characterized for variable EPU and beamline settings and the overall degree of polarization in the MAESTRO end-stations is estimated to be on the order of 83%
High resolution angle resolved photoemission studies on quasi-particle dynamics in graphite
We obtained the spectral function of the graphite H point using high
resolution angle resolved photoelectron spectroscopy (ARPES). The extracted
width of the spectral function (inverse of the photo-hole lifetime) near the H
point is approximately proportional to the energy as expected from the linearly
increasing density of states (DOS) near the Fermi energy. This is well
accounted by our electron-phonon coupling theory considering the peculiar
electronic DOS near the Fermi level. And we also investigated the temperature
dependence of the peak widths both experimentally and theoretically. The upper
bound for the electron-phonon coupling parameter is ~0.23, nearly the same
value as previously reported at the K point. Our analysis of temperature
dependent ARPES data at K shows that the energy of phonon mode of graphite has
much higher energy scale than 125K which is dominant in electron-phonon
coupling.Comment: 9 pages, 8 figures, accepted for publication in Phys. Rev.
Band structure of SnTe studied by Photoemission Spectroscopy
We present an angle-resolved photoemission spectroscopy study of the
electronic structure of SnTe, and compare the experimental results to ab initio
band structure calculations as well as a simplified tight-binding model of the
p-bands. Our study reveals the conjectured complex Fermi surface structure near
the L-points showing topological changes in the bands from disconnected
pockets, to open tubes, and then to cuboids as the binding energy increases,
resolving lingering issues about the electronic structure. The chemical
potential at the crystal surface is found to be 0.5eV below the gap,
corresponding to a carrier density of p =1.14x10^{21} cm^{-3} or 7.2x10^{-2}
holes per unit cell. At a temperature below the cubic-rhombohedral structural
transition a small shift in spectral energy of the valance band is found, in
agreement with model predictions.Comment: 4 figure
Penetration of alkali atoms throughout graphene membrane: theoretical modeling
Theoretical studies of penetration of various alkali atoms (Li, Na, Rb, Cs)
throughout graphene membrane grown on silicon carbide substrate are reported
and compared with recent experimental results. Results of first principles
modeling demonstrate rather low (about 0.8 eV) energy barrier for the formation
of temporary defects in carbon layer required for the penetration of Li at high
concentration of adatoms, higher (about 2 eV) barrier for Na, and barriers
above 4 eV for Rb and Cs. Experiments prove migration of lithium adatoms from
graphene surface to the buffer layer and SiC substrate at room temperature,
sodium at 100{\deg}C and impenetrability of graphene membrane for Rb and Cs.
Differences between epitaxial and free standing graphene for the penetration of
alkali ions are also discussed.Comment: 16 pages, 3 figure, accepted to Nanoscal
Risk of prostate cancer after isolated high-grade prostatic intraepithelial neoplasia (HGPIN) detected on extended core needle biopsy : a UK hospital experience.
Background High-grade prostatic intraepithelial neoplasia (HGPIN) is a precursor lesion to prostate cancer (CaP). UK-based studies examining the occurrence of isolated HGPIN and subsequent risk of CaP are lacking. Our aim was to assess the occurrence of HGPIN in a regional UK population and to determine whether in a retrievable cohort of such patients that had repeat extended core biopsies, there was an elevated risk of CaP. Methods A retrospective analysis of the pathology database was conducted at our institution (Lancashire Teaching Hospitals NHS Foundation Trust) for prostate biopsies recorded between January 2001 and December 2005 (all extended core biopsies). Those patients with isolated HGPIN on 1st set of biopsies were identified and, their clinical characteristics and pathological findings from subsequent biopsies (if any) were determined. The risk of CaP on subsequent biopsies based on presenting baseline PSA was stratified. Results Of 2,192 biopsied patients, there were 88 cases of isolated HGPIN of which 67 patients underwent one or more repeat biopsies. In this repeat-biopsy group, 28 CaP diagnoses were made. Age at first biopsy (P 20 ng/ml – 87.5%. Conclusion Based on our results, we recommend delaying the 1st repeat biopsy at low PSA range but to have a shorter interval to repeat biopsies at intermediate and higher PSA ranges
Surface states and Rashba-type spin polarization in antiferromagnetic MnBiTe
The layered van der Waals antiferromagnet MnBiTe has been predicted
to combine the band ordering of archetypical topological insulators such as
BiTe with the magnetism of Mn, making this material a viable candidate
for the realization of various magnetic topological states. We have
systematically investigated the surface electronic structure of
MnBiTe(0001) single crystals by use of spin- and angle-resolved
photoelectron spectroscopy experiments. In line with theoretical predictions,
the results reveal a surface state in the bulk band gap and they provide
evidence for the influence of exchange interaction and spin-orbit coupling on
the surface electronic structure.Comment: Revised versio
Angle-resolved photoemission spectra of graphene from first-principles calculations
Angle-resolved photoemission spectroscopy (ARPES) is a powerful experimental
technique for directly probing electron dynamics in solids. The energy vs.
momentum dispersion relations and the associated spectral broadenings measured
by ARPES provide a wealth of information on quantum many-body interaction
effects. In particular, ARPES allows studies of the Coulomb interaction among
electrons (electron-electron interactions) and the interaction between
electrons and lattice vibrations (electron-phonon interactions). Here, we
report ab initio simulations of the ARPES spectra of graphene including both
electron-electron and electron-phonon interactions on the same footing. Our
calculations reproduce some of the key experimental observations related to
many-body effects, including the indication of a mismatch between the upper and
lower halves of the Dirac cone
Extraordinary epitaxial alignment of graphene islands on Au(111)
Pristine, single-crystalline graphene displays a unique collection of
remarkable electronic properties that arise from its two-dimensional, honeycomb
structure. Using in-situ low-energy electron microscopy, we show that when
deposited on the (111) surface of Au carbon forms such a structure. The
resulting monolayer, epitaxial film is formed by the coalescence of dendritic
graphene islands that nucleate at a high density. Over 95% of these islands can
be identically aligned with respect to each other and to the Au substrate.
Remarkably, the dominant island orientation is not the better lattice-matched
30^{\circ} rotated orientation but instead one in which the graphene [01] and
Au [011] in-plane directions are parallel. The epitaxial graphene film is only
weakly coupled to the Au surface, which maintains its reconstruction under the
slightly p-type doped graphene. The linear electronic dispersion characteristic
of free-standing graphene is retained regardless of orientation. That a weakly
interacting, non-lattice matched substrate is able to lock graphene into a
particular orientation is surprising. This ability, however, makes Au(111) a
promising substrate for the growth of single crystalline graphene films
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