447 research outputs found

    Magnetic phase diagram of the quantum spin chain compound SrCo2_{2}V2_{2}O8_{8}: a single-crystal neutron diffraction study in magnetic field

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    We explore the spin states in the quantum spin chain compound SrCo2_{2}V2_{2}O8_{8} up to 14.9 T and down to 50 mK, using single-crystal neutron diffraction. Upon cooling in zero-field, antiferromagnetic (AFM) order of N\'eel type develops at TNT_\mathrm{{N}} ≃\simeq 5.0 K. Applying an external magnetic field (HH ∥\parallel cc-axis) destabilizes the N\'eel order, leading to an order-disorder transition when applying a field between TNT_\mathrm{{N}} and ∼\sim 1.5 K. Below 1.5 K, we observe a N\'eel to longitudinal spin density wave (LSDW) order transition at 3.9 T, and a LSDW to emergent AFM order transition at 7.0 T. Our results also reveal several unique signatures for the states of the spins that are not present in the isostructural counterpart BaCo2_{2}V2_{2}O8_{8}.Comment: 9 pages, 9 figures. Accepted manuscrip

    Effect of long-range Coulomb interaction on shot-noise suppression in ballistic transport

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    We present a microscopic analysis of shot-noise suppression due to long-range Coulomb interaction in semiconductor devices under ballistic transport conditions. An ensemble Monte Carlo simulator self-consistently coupled with a Poisson solver is used for the calculations. A wide range of injection-rate densities leading to different degrees of suppression is investigated. A sharp tendency of noise suppression at increasing injection densities is found to scale with a dimensionless Debye length related to the importance of space-charge effects in the structure.Comment: RevTex, 4 pages, 4 figures, minor correction

    A simulational study of the indirect geometry neutron spectrometer, BIFROST at the European Spallation Source, from neutron source position to detector position

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    The European Spallation Source (ESS) is intended to become the most powerful spallation neutron source in the world and the flagship of neutron science in the upcoming decades. The exceptionally high neutron flux will provide unique opportunities for scientific experiments, but also set high requirements for the detectors. One of the most challenging aspects is the rate capability and in particular the peak instantaneous rate capability, i.e. the number of neutrons hitting the detector per channel or cm2^2 at the peak of the neutron pulse. The primary purpose of this paper is to estimate the incident rates that are anticipated for the BIFROST instrument planned for ESS, and also to demonstrate the use of powerful simulation tools for the correct interpretation of neutron transport in crystalline materials. A full simulation model of the instrument from source to detector position, implemented with the use of multiple simulation software packages is presented. For a single detector tube instantaneous incident rates with a maximum of 1.7 GHz for a Bragg peak from a single crystal, and 0.3 MHz for a vanadium sample are found. This paper also includes the first application of a new pyrolytic graphite model, and a comparison of different simulation tools to highlight their strengths and weaknesses.Comment: 45 pages, 20 figure

    Magnetic ground state and magnon-phonon interaction in multiferroic h-YMnO3_3

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    Inelastic neutron scattering has been used to study the magneto-elastic excitations in the multiferroic manganite hexagonal YMnO3_3. An avoided crossing is found between magnon and phonon modes close to the Brillouin zone boundary in the (a,b)(a,b)-plane. Neutron polarization analysis reveals that this mode has mixed magnon-phonon character. An external magnetic field along the cc-axis is observed to cause a linear field-induced splitting of one of the spin wave branches. A theoretical description is performed, using a Heisenberg model of localized spins, acoustic phonon modes and a magneto-elastic coupling via the single-ion magnetostriction. The model quantitatively reproduces the dispersion and intensities of all modes in the full Brillouin zone, describes the observed magnon-phonon hybridized modes, and quantifies the magneto-elastic coupling. The combined information, including the field-induced magnon splitting, allows us to exclude several of the earlier proposed models and point to the correct magnetic ground state symmetry, and provides an effective dynamic model relevant for the multiferroic hexagonal manganites.Comment: 12 pages, 10 figure

    Design and Performance of a Pilot Scale High-Gradient Magnetic Filter Using a Mandhala Magnet and Its Application for Soy-Whey Protein Purification

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    The scalability of economic high-gradient magnetic separation (HGMS) technology is essential in order to demonstrate the feasibility of the concept. One of the means is the application of a permanent magnet with a hollow cylindrical volume made from identical magnetic blocks (e.g., Mandhala), another is the development of a High-Gradient Magnetic Filter (HGMF) with a new backwashing concept. The Mandhala (Magnetic Arrangement for Novel Discrete Halbach Layout) magnet produces a dipolar transversal magnetic field in the center of the bore and its usable volume is easily adaptable to the separation device\u27s extensions. The chapter presents the pilot scale design of the Mandhala magnet and the HGMF as well as experimental performance tests using a water-magnetic beads model system. Subsequently, experiments using soy-whey as a real feedstock demonstrate the purification of the protein Bowman-Birk inhibitor (BBI), an agent against cancer and multiples sclerosis

    Shot noise of a quantum dot with non-Fermi liquid correlations

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    The shot noise of a one-dimensional wire interrupted by two barriers shows interesting features related to the interplay between Coulomb blockade effects, Luttinger correlations and discrete excitations. At small bias the Fano factor reaches the lowest attainable value, 1/2, irrespective of the ratio of the two junction resistances. At larger voltages this asymmetry is power-law renormalized by the interaction strength. We discuss how the measurement of current and these features of the noise allow to extract the Luttinger liquid parameter.Comment: 4 pages, 3 figures,to be published in Phys. Rev. B. For high resolution image of Fig.1 see http://server1.fisica.unige.it/~braggio/doc.ht

    HCl and ClO in activated Arctic air; first retrieved vertical profiles from TELIS submillimetre limb spectra

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    The first profile retrieval results of the Terahertz and submillimeter Limb Sounder (TELIS) balloon instrument are presented. The spectra are recorded during a 13-h balloon flight on 24 January 2010 from Kiruna, Sweden. The TELIS instrument was mounted on the MIPAS-B2 gondola and shared this platform with the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) and the mini- Differential Optical Absorption Spectroscopy (mini-DOAS) instruments. The flight took place within the Arctic vortex at an altitude of ≈34 km in chlorine activated air, and both active (ClO) and inactive chlorine (HCl) were measured over an altitude range of respectively ≈16–32 km and ≈10– 32 km. In this altitude range, the increase of ClO concentration levels during sunrise has been recorded with a temporal resolution of one minute. During the daytime equilibrium, a maximum ClO level of 2.1±0.3 ppbv has been observed at an altitude of 23.5 km. This equilibrium profile is validated against the ClO profile by the satellite instrument Microwave Limb Sounder (MLS) aboard EOS Aura. HCl profiles have been determined from two different isotopes – H35Cl and H37Cl – and are also validated againstMLS. The precision of all profiles is well below 0.01 ppbv and the overall accuracy is therefore governed by systematic effects. The total uncertainty of these effects is estimated to be maximal 0.3 ppbv for ClO around its peak value at 23.5 km during the daytime equilibrium, and for HCl it ranges from 0.05 to 0.4 ppbv, depending on altitude. In both cases the main uncertainty stems from a largely unknown non-linear response in the detector

    Microscopic analysis of shot-noise suppression in nondegenerate diffusive conductors

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    We present a theoretical investigation of shot-noise suppression due to long-range Coulomb interaction in nondegenerate diffusive conductors. Calculations make use of an ensemble Monte Carlo simulator self-consistently coupled with a one-dimensional Poisson solver. We analyze the noise in a lightly doped active region surrounded by two contacts acting as thermal reservoirs. By taking the doping of the injecting contacts and the applied voltage as variable parameters, the influence of elastic and inelastic scattering in the active region is investigated. The transition from ballistic to diffusive transport regimes under different contact injecting statistics is analyzed and discussed. Provided significant space-charge effects take place inside the active region, long-range Coulomb interaction is found to play an essential role in suppressing the shot noise at qU≫kBTqU \gg k_BT. In the elastic diffusive regime, momentum space dimensionality is found to modify the suppression factor γ\gamma, which within numerical uncertainty takes values respectively of about 1/3, 1/2 and 0.7 in the 3D, 2D and 1D cases. In the inelastic diffusive regime, shot noise is suppressed to the thermal value.Comment: 11 pages, 13 figure

    Making waves. Bridging theory and practice towards multiple stressor management in freshwater ecosystems

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    Embargo until February 26, 2023Despite advances in conceptual understanding, single-stressor abatement approaches remain common in the management of fresh waters, even though they can produce unexpected ecological responses when multiple stressors interact. Here we identify limitations restricting the development of multiple-stressor management strategies and address these, bridging theory and practice, within a novel empirical framework. Those critical limitations include that (i) monitoring schemes fall short of accounting for theory on relationships between multiple-stressor interactions and ecological responses, (ii) current empirical modelling approaches neglect the prevalence and intensity of multiple-stressor interactions, and (iii) mechanisms of stressor interactions are often poorly understood. We offer practical recommendations for the use of empirical models and experiments to predict the effects of freshwater degradation in response to changes in multiple stressors, demonstrating this approach in a case study. Drawing on our framework, we offer practical recommendations to support the development of effective management strategies in three general multiple-stressor scenarios.acceptedVersio

    Surveillance biopsies in children post-kidney transplant

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    Surveillance biopsies are increasingly used in the post-transplant monitoring of pediatric renal allograft recipients. The main justification for this procedure is to diagnose early and presumably modifiable acute and chronic renal allograft injury. Pediatric recipients are theoretically at increased risk for subclinical renal allograft injury due to their relatively large adult-sized kidneys and their higher degree of immunological responsiveness. The safety profile of this procedure has been well investigated. Patient morbidity is low, with macroscopic hematuria being the most common adverse event. No patient deaths have been attributed to this procedure. Longitudinal surveillance biopsy studies have revealed a substantial burden of subclinical immunological and non-immunological injury, including acute cellular rejection, interstitial fibrosis and tubular atrophy, microvascular lesions and transplant glomerulopathy. The main impediment to the implementation of surveillance biopsies as the standard of care is the lack of demonstrable benefit of early histological detection on long-term outcome. The considerable debate surrounding this issue highlights the need for multicenter, prospective, and randomized studies
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