Cold SO_2 molecules by Stark deceleration

We produce SO_2 molecules with a centre of mass velocity near zero using a Stark decelerator. Since the initial kinetic energy of the supersonic SO_2 molecular beam is high, and the removed kinetic energy per stage is small, 326 deceleration stages are necessary to bring SO_2 to a complete standstill, significantly more than in other experiments. We show that in such a decelerator possible loss due to coupling between the motional degrees of freedom must be considered. Experimental results are compared with 3D Monte-Carlo simulations and the quantum state selectivity of the Stark decelerator is demonstrated.Comment: 7 pages, 5 figure

Efficient Stark deceleration of cold polar molecules

Stark deceleration has been utilized for slowing and trapping several species of neutral, ground-state polar molecules generated in a supersonic beam expansion. Due to the finite physical dimension of the electrode array and practical limitations of the applicable electric fields, only molecules within a specific range of velocities and positions can be efficiently slowed and trapped. These constraints result in a restricted phase space acceptance of the decelerator in directions both transverse and parallel to the molecular beam axis; hence, careful modeling is required for understanding and achieving efficient Stark decelerator operation. We present work on slowing of the hydroxyl radical (OH) elucidating the physics controlling the evolution of the molecular phase space packets both with experimental results and model calculations. From these results we deduce experimental conditions necessary for efficient operation of a Stark decelerator.Comment: 8 pages, 9 figure

Stark deceleration of CaF molecules in strong- and weak-field seeking states

We report the Stark deceleration of CaF molecules in the strong-field seeking ground state and in a weak-field seeking component of a rotationally-excited state. We use two types of decelerator, a conventional Stark decelerator for the weak-field seekers, and an alternating gradient decelerator for the strong-field seekers, and we compare their relative merits. We also consider the application of laser cooling to increase the phase-space density of decelerated molecules.Comment: 10 pages, 8 figure

On deflection fields, weak-focusing and strong-focusing storage rings for polar molecules

In this paper, we analyze electric deflection fields for polar molecules in terms of a multipole expansion and derive a simple but rather insightful expression for the force on the molecules. Ideally, a deflection field exerts a strong, constant force in one direction, while the force in the other directions is zero. We show how, by a proper choice of the expansion coefficients, this ideal can be best approximated. We present a design for a practical electrode geometry based on this analysis. By bending such a deflection field into a circle, a simple storage ring can be created; the direct analog of a weak-focusing cyclotron for charged particles. We show that for realistic parameters a weak-focusing ring is only stable for molecules with a very low velocity. A strong-focusing (alternating-gradient) storage ring can be created by arranging many straight deflection fields in a circle and by alternating the sign of the hexapole term between adjacent deflection fields. The acceptance of this ring is numerically calculated for realistic parameters. Such a storage might prove useful in experiments looking for an EDM of elementary particles.Comment: 8 pages, 5 figure

Feasibility of a storage ring for polar molecules in strong-field-seeking states

We show, through modeling and simulation, that it is feasible to construct a storage ring that will store dense bunches of strong-field-seeking polar molecules at 30 m/s (kinetic energy of 2K) and hold them, for several minutes, against losses due to defocusing, oscillations, and diffusion. The ring, 3 m in diameter, has straight sections that afford access to the stored molecules and a lattice structure that may be adapted for evaporative cooling. Simulation is done using a newly-developed code that tracks the particles, in time, through 400 turns; it accounts for longitudinal velocity changes as a function of external electric field, focusing and deflection nonlinearities, and the effects of gravity. An injector, decelerator, and source are included and intensities are calculated.Comment: 6 pages 5 figures, 3 table

Ramsey-type microwave spectroscopy on CO (a3Πa^3\Pi)

Using a Ramsey-type setup, the lambda-doublet transition in the $J=1,\, \Omega=1$ level of the $a^3\Pi$ state of CO was measured to be 394 064 870(10) Hz. In our molecular beam apparatus, a beam of metastable CO is prepared in a single quantum level by expanding CO into vacuum and exciting the molecules using a narrow-band UV laser system. After passing two microwave zones that are separated by 50 cm, the molecules are state-selectively deflected and detected 1 meter downstream on a position sensitive detector. In order to keep the molecules in a single $m_J^B$ level, a magnetic bias field is applied. We find the field-free transition frequency by taking the average of the $m_J^B = +1 \rightarrow m_J^B = +1$ and $m_J^B = -1 \rightarrow m_J^B = -1$ transitions, which have an almost equal but opposite Zeeman shift. The accuracy of this proof-of-principle experiment is a factor of 100 more accurate than the previous best value obtained for this transition

Economic Analysis of Western Corn Rootworm Injury to Continuous Corn in Northeast Nebraska.

The most economically significant corn pest in the US Corn Belt is the Western Corn Rootworm (WCR), Diabrotica virgifera virgifera LeConte. This study compares a field experiment outcome of 4 different treatments against WCR, which consist of a rootworm Bt corn pyramid (SmartStax®) and non-rootworm Bt trait hybrid (VT2P), with or without the addition of the rootworm soil insecticide (Aztec®) to identify the risk-reward trade-off for each one of them. Observed prices were used for the years in the study (2020, 2021, and 2022), and low and high price scenarios were simulated for the period, to incorporate different dynamic relations between years. Also, different WCR Bt resistance levels and rootworm densities were accounted for: fields were classified into four groups based on susceptibility (corrected survival ³ 0.5 and \u3c 0.5) and population pressure (root injury for the control treatment ³ 1 and \u3c 1). This study also addresses how crop insurance plays a role in offsetting revenue to farmers from the fields most affected by WCR, at two insurance coverage levels: 70% coverage level – a commonly used level - and 85% coverage level - as a specific strategy with moral hazard implications. We identified that SmartStax® was the most profitable option although adding the insecticide reduces production risk exposure. Also, crop insurance gives an advantage to non-rootworm Bt traits and the 85% coverage level for fields that presented low resistance but high population pressure. Advisor: Cory Walter

Sensitivity of rotational transitions in CH and CD to a possible variation of fundamental constants

The sensitivity of rotational transitions in CH and CD to a possible variation of fundamental constants has been investigated. Largely enhanced sensitivity coefficients are found for specific transitions which are due to accidental degeneracies between the different fine-structure manifolds. These degeneracies occur when the spin-orbit coupling constant is close to four times the rotational constant. CH and particularly CD match this condition closely. Unfortunately, an analysis of the transition strengths shows that the same condition that leads to an enhanced sensitivity suppresses the transition strength, making these transitions too weak to be of relevance for testing the variation of fundamental constants over cosmological time scales. We propose a test in CH based on the comparison between the rotational transitions between the e and f components of the Omega'=1/2,J=1/2 and Omega'=3/2,J=3/2 levels at 532 and 536 GHz and other rotational or Lambda-doublet transitions in CH involving the same absorbing ground levels. Such a test, to be performed by radioastronomy of highly redshifted objects, is robust against systematic effects

Preparation of an ultra-cold sample of ammonia molecules for precision measurements

We present experiments in which an ultra-cold sample of ammonia molecules is released from an electrostatic trap and recaptured after a variable time. It is shown that, by performing adiabatic cooling before releasing the molecules and adiabatic re-compression after they are recaptured, we are able to observe molecules even after more than 10 ms of free expansion. A coherent measurement performed during this time will have a statistical uncertainty that decreases approximately as the inverse of the square root of the expansion time. This offers interesting prospects for high-resolution spectroscopy and precision tests of fundamental physics theories