527 research outputs found

    Magnetic excitations in vanadium spinels

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    We study magnetic excitations in vanadium spinel oxides AV2_2O4_4 (A=Zn, Mg, Cd) using two models: first one is a superexchange model for vanadium S=1 spins, second one includes in addition spin-orbit coupling, and crystal anisotropy. We show that the experimentally observed magnetic ordering can be obtained in both models, however the orbital ordering is different with and without spin-orbit coupling and crystal anisotropy. We demonstrate that this difference strongly affects the spin-wave excitation spectrum above the magnetically ordered state, and argue that the neutron measurement of such dispersion is a way to distinguish between the two possible orbital orderings in AV2_2O4_4.Comment: accepted in Phys. Rev.

    A possible phase dependent absorption feature in the transient X-ray pulsar SAX J2103.5+4545

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    We present an X-ray spectral and timing analysis of two NuSTARNuSTAR observations of the transient Be X-ray binary SAX J2103.5+4545 during its April 2016 outburst, which was characterized by the highest flux since NuSTARNuSTAR's launch. These observations provide detailed hard X-ray spectra of this source during its bright precursor flare and subsequent fainter regular outburst for the first time. In this work, we model the phase-averaged spectra for these observations with a negative and positive power law with an exponential cut-off (NPEX) model and compare the pulse profiles at different flux states. We found that the broad-band pulse profile changes from a three peaked pulse in the first observation to a two peaked pulse in the second observation, and that each of the pulse peaks has some energy dependence. We also perform pulse-phase spectroscopy and fit phase-resolved spectra with NPEX to evaluate how spectral parameters change with pulse phase. We find that while the continuum parameters are mostly constant with pulse phase, a weak absorption feature at ~12 keV that might, with further study, be classified as a cyclotron line, does show strong pulse phase dependence.Comment: 10 pages, 7 figures, accepted by ApJ, acknowledgements update

    Mimicking climate warming effects on Alaskan soil microbial communities via gradual temperature increase

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    Climate change can trigger shifts in community structure and may therefore pose a severe threat to soil microbial communities, especially in high northern latitudes such as the Arctic. Arctic soils are covered by snow and ice throughout most of the year. This insulation shields them from high temperature variability and low surface temperatures. If this protective layer thaws, these soils are predicted to warm up at 1.5x to 4x the rate of other terrestrial biomes. In this study, we sampled arctic soils from sites with different elevations in Alaska, incubated them for 5 months with a simulated, gradual or abrupt temperature increase of +5 °C, and compared bacterial and fungal community compositions after the incubation. We hypothesized that the microbial communities would not significantly change with a gradual temperature treatment, whereas an abrupt temperature increase would decrease microbial diversity and shift community composition. The only differences in community composition that we observed were, however, related to the two elevations. The abrupt and gradual temperature increase treatments did not change the microbial community composition as compared to the control indicating resistance of the microbial community to changes in temperature. This points to the potential importance of microbial dormancy and resting stages in the formation of a “buffer” against elevated temperatures. Microbial resting stages might heavily contribute to microbial biomass and thus drive the responsiveness of arctic ecosystems to climate change

    Non-resonant inelastic x-ray scattering involving excitonic excitations

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    In a recent publication Larson \textit{et al.} reported remarkably clear dd-dd excitations for NiO and CoO measured with x-ray energies well below the transition metal KK edge. In this letter we demonstrate that we can obtain an accurate quantitative description based on a local many body approach. We find that the magnitude of q\vec{q} can be tuned for maximum sensitivity for dipole, quadrupole, etc. excitations. We also find that the direction of q\vec{q} with respect to the crystal axes can be used as an equivalent to polarization similar to electron energy loss spectroscopy, allowing for a determination of the local symmetry of the initial and final state based on selection rules. This method is more generally applicable and combined with the high resolution available, could be a powerful tool for the study of local distortions and symmetries in transition metal compounds including also buried interfaces

    Evidence for a temperature-induced spin-state transition of Co3+ in La2-xSrxCoO4

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    We study the magnetic susceptibility of mixed-valent La2-xSrxCoO4 single crystals in the doping range of 0.5<= x <= 0.8 for temperatures up to 1000 K. The magnetism below room temperature is described by paramagnetic Co2+ in the high-spin state and by Co3+ in the non-magnetic low-spin state. Above room temperature, an increase in susceptibility compared to the behavior expected from Co2+ is seen, which we attribute to a spin-state transition of Co3+. The susceptibility is analyzed by comparison to full-multiplet calculations for the thermal population of the high- and intermediate-spin states of Co3+

    Magnetic properties of 3d-impurities substituted in GaAs

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    We have calculated the magnetic properties of substituted 3d-impurities (Cr-Ni) in a GaAs host by means of first principles electronic structure calculations. We provide a novel model explaining the ferromagnetic long rang order of III-V dilute magnetic semiconductors. The origin of the ferromagnetism is shown to be due to delocalized spin-uncompensated As dangling bond electrons. Besides the quantitative prediction of the magnetic moments, our model provides an understanding of the halfmetallicity, and the raise of the critical temperature with the impurity concentration

    Fungal response to abruptly or gradually delivered antifungal agent amphotericin B is growth stage dependent

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    Anthropogenic disturbances pose a multitude of novel challenges to ecosystems. While many experiments have tested effects using abrupt treatment applications, most environmental changes in fact are gradual. Since ecosystem responses might be highly dependent on the temporal nature of stressors, it is crucial to differentiate the effects of abrupt vs gradual treatment application. Antifungal agents, which are widely used in disease control both for humans and in agriculture, are becoming a new class of environmental contaminants. In this study, we examined the effect of a sub-lethal application of one antifungal agent, amphotericin B. We applied different rates of delivery, e.g. gradual and abrupt, and monitored biomass and sporulation of the model fungus Neurospora crassa in a batch culture. Our results demonstrate that: (i) the effect size difference between abrupt and gradual treatments is fungal growth stage dependent and (ii) the gradual treatment clearly had a higher sporulation level compared with all types of abrupt treatments. Our findings highlight the importance of considering the rate of change in environmental change research and point to a new research direction for future global change studies. Furthermore, our results also have important implications for avoiding treatment-induced spore production in agriculture and medical practise

    Critical Phenomena in Continuous Dimension

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    We present a calculation of critical phenomena directly in continuous dimension d employing an exact renormalization group equation for the effective average action. For an Ising-type scalar field theory we calculate the critical exponents nu(d) and eta(d) both from a lowest--order and a complete first--order derivative expansion of the effective average action. In particular, this can be used to study critical behavior as a function of dimensionality at fixed temperature.Comment: 5 pages, 1 figure, PLB version, references adde

    Local electronic structure of Fe2+^{2+} impurities in MgO thin films: Temperature-dependent soft x-ray absorption spectroscopy study

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    We report on the local electronic structure of Fe impurities in MgO thin films. Using soft x-ray absorption spectroscopy (XAS) we verified that the Fe impurities are all in the 2+ valence state. The fine details in the line shape of the Fe L2,3L_{2,3} edges provide direct evidence for the presence of a dynamical Jahn-Teller distortion. We are able to determine the magnitude of the effective D4hD_{4h} crystal field energies. We also observed a strong temperature dependence in the spectra which we can attribute to the thermal population of low-lying excited states that are present due to the spin-orbit coupling in the Fe 3d. Using this Fe2+^{2+} impurity system as an example, we show that an accurate measurement of the orbital moment in Fe3_3O4_4 will provide a direct estimate for the effective local low-symmetry crystal fields on the Fe2+^{2+} sites, important for the theoretical modeling of the formation of orbital ordering
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