STRATAQ: A three-dimensional Chemical Transport Model of the stratosphere

International audienceA three-dimensional (3-D) Chemical Transport Model (CTM) of the stratosphere has been developed and used for a test study of the evolution of chemical species in the arctic lower stratosphere during winter 1996/97. This particular winter has been chosen for testing the model's capabilities for its remarkable dynamical situation (very cold and strong polar vortex) along with the availability of sparse chlorine, HNO3 and O3 data, showing also very low O3 values in late March/April. Due to those unusual features, the winter 1996/97 can be considered an excellent example of the impact of both dynamics and heterogeneous reactions on the chemistry of the stratosphere. Model integration has been performed from January to March 1997 and the resulting long-lived and short-lived tracer fields compared with available measurements. The model includes a detailed gas phase chemical scheme and a parameterization of the heterogeneous reactions occurring on liquid aerosol and polar stratospheric cloud (PSC) surfaces. The transport is calculated using a semi-lagrangian flux scheme, forced by meteorological analyses. In such form, the STRATAQ CTM model is suitable for short-term integrations to study transport and chemical evolution related to "real" meteorological situations. Model simulation during the chosen winter shows intense PSC formation, with noticeable local HNO3 capture by PSCs, and the activation of vortex air leading to chlorine production and subsequent O3 destruction. The resulting model fields show generally good agreement with satellite data (MLS and TOMS), although the available observations, due to their limited number and time/space sparse nature, are not enough to effectively constraint the model. In particular, the model seems to perform well in reproducing the rapid processing of air inside the polar vortex on PSC converting reservoir species in active chlorine. In addition, it satisfactorily reproduces the morphology of the continuous O3 decline as shown by the satellite during the investigated period, with a tendency, however, to underestimate the total column values inside the polar vortex during late winter. As possible causes of this model/observation difference we suggest an incorrect estimation of the vertical transport and of the tropospheric contribution

Assimilation of stratospheric ozone in the chemical transport model STRATAQ

International audienceWe describe a sequential assimilation approach useful for assimilating tracer measurements into a three-dimensional chemical transport model (CTM) of the stratosphere. The numerical code, developed largely according to Kha00, uses parameterizations and simplifications allowing assimilation of sparse observations and the simultaneous evaluation of analysis errors, with reasonable computational requirements. Assimilation parameters are set by using ?2 and OmF (Observation minus Forecast) statistics. The CTM used here is a high resolution three-dimensional model. It includes a detailed chemical package and is driven by UKMO (United Kingdom Meteorological Office) analyses. We illustrate the method using assimilation of Upper Atmosphere Research Satellite/Microwave Limb Sounder (UARS/MLS) ozone observations for three weeks during the 1996 antarctic spring. The comparison of results from the simulations with TOMS (Total Ozone Mapping Spectrometer) measurements shows improved total ozone fields due to assimilation of MLS observations. Moreover, the assimilation gives indications on a possible model weakness in reproducing polar ozone values during springtime

Validation and analysis of regional present-day climate and climate change simulations over Europe

In the European Commission (EC) project "Regionalization of Anthropogenic Climate Change Simulations, RACCS, recently terminated, 11 European institutions have carried out tests of dynamical and statistical regionalization techniques. The outcome of the "dynamical part" of the project, utilizing a series of high resolution LAMs and a variable resolution global model (all of which we shall refer to as RCMs, Regional Climate Models), is presented here. The per- formance of the dqterent LAMs had first, in a preceding EC project, been tested with "perfect" boundary forcing fields (ECMWF analyses) and also multi-year present-day climate simula- tions with AMIP "perfect ocean " or mixed layer ocean GCM boundary conditions had been validated against available climatological data. The present report involves results of vali- dation and analysis of RCM present-day climate simulations and anthropogenic climate change experiments. Multi-year (5 - 30 years) present-day climate simulations have been per- formed with resolutions between 19 and 70 km (grid lengths) and with boundary conditions from the newest CGCM simulations. The climate change experiments involve various 2xCO2 - ]xCO2 transient greenhouse gas experiments and in one case also changing sulphur aerosols. A common validation and inter-comparison was made at the coordinating institution, MPIfor Meteorology. The validation of the present-day climate simulations shows the importance of systematic errors in the low level general circulation. Such errors seem to induce large errors in precipitation and surface air temperature in the RCMs as well as in the CGCMs providing boundary conditions. Over Europe the field of systematic errors in the mean sea level pressure (MSLP) usually involve an area of too low pressure, often in the form of an east-west trough across Europe with too high pressure to the north and south. New storm-track analyses confirm that the areas of too low pressure are caused by enhanced cyclonic activity and similarly that the areas of too high pressure are caused by reduced such activity. The precise location and strength of the extremes in the MSLP error field seems to be dependent on the physical param- eterization package used. In model pairs sharing the same package the area of too low pressure is deepened further in the RCM compared to the corresponding CGCM, indicating an increase of the excessive cyclonic activity with increasing resolution. From the experiments performed it seems not possible to decide to what extent the systematic errors in the general circulation are the result of local errors in the physical parameterization schemes or remote errors trans- mitted to the European region via the boundary conditions. Additional errors in precipitation and temperature seems to be due to direct local effects of errors in certain parameterization schemes and errors in the SSTs taken from the CGCMs. For all seasons many biases are fOund to be statistically significant compared to estimates of the internal model variability of the time- slice mean values. In the climate change experiments statistically significant European mean temperature changes which are large compared to the corresponding biases are found. How- ever, the changes in the deviations from the European mean temperature as well as the changes in precipitation are only partly sign wcan ce and are of the same order of magnitude or smaller than the corresponding biases found in the present-day climate simulations. Cases of an inter- action between the systematic model errors and the radiative forcing show that generally the errors are not canceling out when the changes are computed. Therefore, reliable regional cli- mate changes can only be achieved after model improvements which reduce their systematic errors sufficiently. Also in future RCM experiments sujiciently long time-slices must be used in order to obtain statistically sign ijicant climate changes on the sub-continental scale aimed at with the present regionalization technique

Coupling a distributed grid based hydrological model and MM5 meteorological model for flooding alert mapping

International audienceThe increased number of extreme rainfall events seems to be one of the common feature of climate change signal all over the world (Easterlin et al., 2000; Meehl et al., 2000). In the last few years a large number of floods caused by extreme meteorological events has been observed over the river basins of Mediterranean area and they mainly affected small basins (few hundreds until few thousands of square kilometres of drainage area) . A strategic goal of applied meteorology is now to try to predict with high spatial resolution the segments of drainage network where floods may occur. A possible way to reach this aim is the coupling of meteorological mesoscale model with high resolution hydrological model. In this work few case studies of observed floods in the Italian Mediterranean area will be presented. It is shown how a distributed hydrological model, using the precipitation fields predicted by MM5 meteorological model, is able to highlight the area where the major floods may occur

Thermally driven circulation in a region of complex topography: comparison of wind-profiling radar measurements and MM5 numerical predictions

The diurnal variation of regional wind patterns in the complex terrain of Central Italy was investigated for summer fair-weather conditions and winter time periods using a radar wind profiler. The profiler is located on a site where interaction between the complex topography and land-surface produces a variety of thermally and dynamically driven wind systems. The observational data set, collected for a period of one year, was used first to describe the diurnal evolution of thermal driven winds, second to validate the Mesoscale Model 5 (MM5) that is a three-dimensional numerical model. This type of analysis was focused on the near-surface wind observation, since thermally driven winds occur in the lower atmosphere. According to the valley wind theory expectations, the site – located on the left sidewall of the valley (looking up valley) – experiences a clockwise turning with time. Same characteristics in the behavior were established in both the experimental and numerical results. <P style="line-height: 20px;"> Because the thermally driven flows can have some depth and may be influenced mainly by model errors, as a third step the analysis focuses on a subset of cases to explore four different MM5 Planetary Boundary Layer (PBL) parameterizations. The reason is to test how the results are sensitive to the selected PBL parameterization, and to identify the better parameterization if it is possible. For this purpose we analysed the MM5 output for the whole PBL levels. The chosen PBL parameterizations are: 1) Gayno-Seaman; 2) Medium-Range Forecast; 3) Mellor-Yamada scheme as used in the ETA model; and 4) Blackadar

Aircraft based four-channel thermal dissociation laser induced fluorescence instrument for simultaneous measurements of NO2, total peroxy nitrate, total alkyl nitrate, and HNO3

A four-channel thermal dissociation laser induced fluorescence (TD-LIF) instrument has been developed for simultaneous measurements of nitrogen dioxide (NO2), total peroxy nitrate (∑PNs), total alkyl nitrate (∑ANs) and nitric acid (HNO3). NO2 is measured directly by LIF at 532 nm, whereas organic nitrates and nitric acid are thermally dissociated at distinct temperatures in the inlet to form NO2, which is then measured by LIF. The concentrations of each dissociated species are derived by the differences in measured NO2 relative to the reference colder inlet channel. The TD-LIF was adapted to fly on board the UK Facility for Airborne Atmospheric Measurements (FAAM) BAe 146-301 atmospheric research aircraft in summer 2010, and to date has successfully flown in five field campaigns. This paper reports novel improvements in the TD-LIF instrumentations, including (1) the use of a single wavelength laser, which makes the system compact and relatively cheap; (2) the use of a single beam laser that allows easy alignment and optical stability against the vibrational aircraft environment; and (3) the optical assembly of four detection cells that allow simultaneous and fast (time resolution up to 0.1 s) measurements of NO2, ∑PNs, ∑ANs and HNO3. Laboratory-generated mixtures of PNs, ANs and HNO3 in zero air are converted into NO2 and used to fix the dissociation temperatures of each heated inlet to test the selectivity of the instrument and potential interferences due to recombination reactions of the dissociated products. The effectiveness of the TD-LIF was demonstrated during the RONOCO aircraft campaign (summer 2010). A chemiluminescence system that was measuring NO2 and a broadband cavity enhanced absorption spectrometer (BBCEAS) that was measuring one of the PNs (N2O5) were installed on the same aircraft during the campaign. The in-flight intercomparison of the new TD-LIF with the chemiluminescence system for NO2 measurements and the intercomparison between ∑PNs measured by the TD-LIF and N2O5 by the BBCEAS are used to assess the performance of the TD-LIF

Mixing and reaction efficiency in closed domains

We present a numerical study of mixing and reaction efficiency in closed domains. In particular we focus our attention on laminar flows. In the case of inert transport the mixing properties of the flows strongly depend on the details of the Lagrangian transport. We also study the reaction efficiency. Starting with a little spot of product we compute the time needed to complete the reaction in the container. We found that the reaction efficiency is not strictly related to the mixing properties of the flow. In particular, reaction acts as a "dynamical regulator".Comment: 11 pages, 10 figure

Solar-Powered Deep Learning-Based Recognition System of Daily Used Objects and Human Faces for Assistance of the Visually Impaired

This paper introduces a novel low-cost solar-powered wearable assistive technology (AT) device, whose aim is to provide continuous, real-time object recognition to ease the finding of the objects for visually impaired (VI) people in daily life. The system consists of three major components: a miniature low-cost camera, a system on module (SoM) computing unit, and an ultrasonic sensor. The first is worn on the user’s eyeglasses and acquires real-time video of the nearby space. The second is worn as a belt and runs deep learning-based methods and spatial algorithms which process the video coming from the camera performing objects’ detection and recognition. The third assists on positioning the objects found in the surrounding space. The developed device provides audible descriptive sentences as feedback to the user involving the objects recognized and their position referenced to the user gaze. After a proper power consumption analysis, a wearable solar harvesting system, integrated with the developed AT device, has been designed and tested to extend the energy autonomy in the dierent operating modes and scenarios. Experimental results obtained with the developed low-cost AT device have demonstrated an accurate and reliable real-time object identification with an 86% correct recognition rate and 215 ms average time interval (in case of high-speed SoM operating mode) for the image processing. The proposed system is capable of recognizing the 91 objects oered by the Microsoft Common Objects in Context (COCO) dataset plus several custom objects and human faces. In addition, a simple and scalable methodology for using image datasets and training of Convolutional Neural Networks (CNNs) is introduced to add objects to the system and increase its repertory. It is also demonstrated that comprehensive trainings involving 100 images per targeted object achieve 89% recognition rates, while fast trainings with only 12 images achieve acceptable recognition rates of 55%

Facial Asymmetry Detected with 3D Methods in Orthodontics: A Systematic Review

Background: Historically, the development of two-dimensional (2D) imaging techniques forerun that of three-dimensional (3D) ones. Some 2D methods are still considered valid and effective to diagnose facial asymmetry but 3D techniques may provide more precise and accurate measurements. Objective: The aim of this work is to analyze the accuracy and reliability of the imaging techniques available for the diagnosis of facial asymmetry in orthodontics and find the most reliable. Methods: A search strategy was implemented using PubMed (National Library of Medicine, NCBI). Results: A total of 3201 papers were identified in electronic searches. 90 articles, available in full text, were included in the qualitative synthesis consisting of 8 reviews on the diagnosis of facial asymmetry, 22 in vivo and in vitro studies on 2D methods and 60 in vivo and in vitro studies on 3D methods to quantify the asymmetry. Conclusion: 2D techniques include X-ray techniques such as posterior-anterior cephalogram, which still represents the first level exam in the diagnosis of facial asymmetry. 3D techniques represent the second level exam in the diagnosis of facial asymmetry. The most current used techniques are CBCT, stereophotogrammetry, laser scanning, 3D optical sensors and contact digitization. The comparison between bilateral parameters (linear distances, angles, areas, volumes and contours) and the calculation of an asymmetry index represent the best choices for clinicians who use CBCT. The creation of a color-coded distance map seems to represent the most accurate, reliable and validated methods for clinicians who use stereophotogrammetry, laser scanning and 3D optical sensors