120 research outputs found
Study of the hydrogen stability in evaporated amorphous Si 1− x Sn x :H (0≤ x ≤0.2) alloys by neutron scattering and exodiffusion measurements
International audienc
Spin-Waves in the Mid-Infrared Spectrum of Antiferromagnetic YBaCuO
The mid-infrared spin-wave spectrum of antiferromagnetic
YBaCuO\ was determined by infrared transmission and reflection
measurements (\bbox{k} \!\! \parallel c) at ~K.\@ Excitation of
single magnons of the optical branch was observed at
~meV.\@ Two further peaks at ~meV
() and ~meV
() both belong to the two-magnon spectrum. Linear
spin wave theory is in good agreement with the measured two-magnon spectrum,
and allows to determine the exchange constant to be about ~meV,
whereas the intrabilayer coupling is approximately .Comment: 3 figures in uuencoded for
Specific heat of Ce_{0.8}La_{0.2}Al_{3} in magnetic fields: a test of the anisotropic Kondo picture
The specific heat C of Ce_{0.8}La_{0.2}Al_{3} has been measured as a function
of temperature T in magnetic fields up to 14 T. A large peak in C at 2.3 K has
recently been ascribed to an anisotropic Kondo effect in this compound. A 14-T
field depresses the temperature of the peak by only 0.2 K, but strongly reduces
its height. The corresponding peak in C/T shifts from 2.1 K at zero field to
1.7 K at 14 T. The extrapolated specific heat coefficient C/T(T->0) increases
with field over the range studied. We show that these trends are inconsistent
with the anisotropic Kondo model.Comment: 4 pages, 5 figures, ReVTeX + eps
Satellite holmium M-edge spectra from the magnetic phase via resonant x-ray scattering
Developing an expression of resonant x-ray scattering (RXS) amplitude which
is convenient for investigating the contributions from the higher rank tensor
on the basis of a localized electron picture, we analyze the RXS spectra from
the magnetic phases of Ho near the absorption edges. At the
edge in the uniform helical phase, the calculated spectra of the absorption
coefficient, the RXS intensities at the first and second satellite spots
capture the properties the experimental data possess, such as the spectral
shapes and the peak positions. This demonstrates the plausibility of the
adoption of the localized picture in this material and the effectiveness of the
spectral shape analysis. The latter point is markedly valuable since the
azimuthal angle dependence, which is one of the most useful informations RXS
can provides, is lacking in the experimental conditions. Then, by focusing on
the temperature dependence of the spectral shape at the second satellite spot,
we expect that the spectrum is the contribution of the pure rank two profile in
the uniform helical and the conical phases while that is dominated by the rank
one profile in the intermediate temperature phase, so-called spin slip phase.
The change of the spectral shape as a function of temperature indicates a
direct evidence of the change of magnetic structures undergoing. Furthermore,
we predict that the intensity, which is the same order observed at the second
satellite spot, is expected at the fourth satellite spot from the conical phase
in the electric dipolar transition.Comment: 24 pages, 5 figure
High energy spin excitations in YBa_2 Cu_3 O_{6.5}
Inelastic neutron scattering has been used to obtain a comprehensive
description of the absolute dynamical spin susceptibility
of the underdoped superconducting cuprate YBa_2 Cu_3 O_{6.5} ()
over a wide range of energies and temperatures ( and ). Spin excitations of two different
symmetries (even and odd under exchange of two adjacent CuO_2 layers) are
observed which, surprisingly, are characterized by different temperature
dependences. The excitations show dispersive behavior at high energies.Comment: 15 pages, 5 figure
Resonant x-ray diffraction study of the magnetoresistant perovskite Pr0.6Ca0.4MnO3
We report a x-ray resonant diffraction study of the perovskite
Pr0.6Ca0.4MnO3. At the Mn K-edge, this technique is sensitive to details of the
electronic structure of the Mn atoms. We discuss the resonant x-ray spectra
measured above and below the charge and orbital ordering phase transition
temperature (TCOO = 232 K), and present a detailed analysis of the energy and
polarization dependence of the resonant scattering. The analysis confirms that
the structural transition is a transition to an orbitally ordered phase in
which inequivalent Mn atoms are ordered in a CE-type pattern. The Mn atoms
differ mostly by their 3d orbital occupation. We find that the charge
disproportionation is incomplete, 3d^{3.5-\delta} and 3d^{3.5+\delta} with
\delta\ll0.5 . A revised CE-type model is considered in which there are two Mn
sublattices, each with partial e_{g} occupancy. One sublattice consists of Mn
atoms with the 3x^{2}-r^{2} or 3y^{2}-r^{2} orbitals partially occupied, the
other sublattice with the x^{2}-y^{2} orbital partially occupied.Comment: 15 pages, 15 figure
N2-H2 capacitively coupled radio-frequency discharges at low pressure. Part I. Experimental results: Effect of the H2 amount on electrons, positive ions and ammonia formation
The mixing of N2 with H2 leads to very different plasmas from pure N2 and H2 plasma discharges. Numerous issues are therefore raised involving the processes leading to ammonia (NH3) formation. The aim of this work is to better characterize capacitively-coupled radiofrequency plasma discharges in N2 with few percents of H2 (up to 5%), at low pressure (0.3-1 mbar) and low coupled power (3-13 W). Both experimental measurements and numerical simulations are performed. For clarity, we separated the results in two complementary parts. The actual one (first part), presents the details on the experimental measurements, while the second focuses on the simulation, a hybrid model combining a 2D fluid module and a 0D kinetic module. Electron density is measured by a resonant cavity method. It varies from 0.4 to 5 109 cm-3, corresponding to ionization degrees from 2 10-8 to 4 10-7. Ammonia density is quantified by combining IR absorption and mass spectrometry. It increases linearly with the amount of H2 (up to 3 1013 cm-3 at 5% H2). On the contrary, it is constant with pressure, which suggests the dominance of surface processes on the formation of ammonia. Positive ions are measured by mass spectrometry. Nitrogen-bearing ions are hydrogenated by the injection of H2, N2H+ being the major ion as soon as the amount of H2 is >1%. The increase of pressure leads to an increase of secondary ions formed by ion/radical-neutral collisions (ex: N2H+, NH4 +, H3 +), while an increase of the coupled power favours ions formed by direct ionization (ex: N2 +, NH3 +, H2 +).N. Carrasco acknowledges the financial support of the European Research Council (ERC Starting Grant
PRIMCHEM, Grant agreement no. 636829).
A. Chatain acknowledges ENS Paris-Saclay Doctoral Program. A. Chatain is grateful to Gilles Cartry and
Thomas Gautier for fruitful discussions on the MS calibration.
L.L. Alves acknowledges the financial support of the Portuguese Foundation for Science and Technology (FCT) through the project UID/FIS/50010/2019.
L. Marques and M. J. Redondo acknowledge the financial support of the Portuguese Foundation for Science
and Technology (FCT) in the framework of the Strategic Funding UIDB/04650/2019
The neutron and its role in cosmology and particle physics
Experiments with cold and ultracold neutrons have reached a level of
precision such that problems far beyond the scale of the present Standard Model
of particle physics become accessible to experimental investigation. Due to the
close links between particle physics and cosmology, these studies also permit a
deep look into the very first instances of our universe. First addressed in
this article, both in theory and experiment, is the problem of baryogenesis ...
The question how baryogenesis could have happened is open to experimental
tests, and it turns out that this problem can be curbed by the very stringent
limits on an electric dipole moment of the neutron, a quantity that also has
deep implications for particle physics. Then we discuss the recent spectacular
observation of neutron quantization in the earth's gravitational field and of
resonance transitions between such gravitational energy states. These
measurements, together with new evaluations of neutron scattering data, set new
constraints on deviations from Newton's gravitational law at the picometer
scale. Such deviations are predicted in modern theories with extra-dimensions
that propose unification of the Planck scale with the scale of the Standard
Model ... Another main topic is the weak-interaction parameters in various
fields of physics and astrophysics that must all be derived from measured
neutron decay data. Up to now, about 10 different neutron decay observables
have been measured, much more than needed in the electroweak Standard Model.
This allows various precise tests for new physics beyond the Standard Model,
competing with or surpassing similar tests at high-energy. The review ends with
a discussion of neutron and nuclear data required in the synthesis of the
elements during the "first three minutes" and later on in stellar
nucleosynthesis.Comment: 91 pages, 30 figures, accepted by Reviews of Modern Physic
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