Broken time-reversal symmetry in cubic skutterudite-like superconductor Y3_3Ru4_4Ge13_{13}

The microscopic properties of superconducting cubic skutterudite-like material Y$_3$Ru$_4$Ge$_{13}$ are investigated using muon spin relaxation and rotation ($\mu$SR) measurements. Zero-field $\mu$SR measurements reveal the presence of a spontaneous internal field with a magnitude of $\approx$ 0.18~mT below the superconducting transition temperature, indicating broken time-reversal symmetry in the ground state. In line with previous experiments, transverse-field $\mu$SR measurements are consistent with a fully developed superconductivity gap in Y$_3$Ru$_4$Ge$_{13}$. Our observations point towards the relevance of electronic correlations beyond electron-phonon coupling as origin and indicate that spin-orbit coupling is likely not the key driving force behind the spontaneous breaking of time-reversal symmetry in this system.Comment: 7 pages, 3 figure

Time-reversal symmetry breaking in superconducting low-carrier-density quasi-skutterudite Lu3Os4Ge13

The complex structure of the Remeika phases, the intriguing quantum states they display, and their low carrier concentrations are a strong motivation to study the nature of their superconducting phases. In this work, the microscopic properties of the superconducting phase of single-crystalline Lu$_3$Os$_4$Ge$_{13}$ are investigated by muon-spin relaxation and rotation ($\mu$SR) measurements. The zero-field $\mu$SR data reveal the presence of spontaneous static or quasi-static magnetic fields in the superconducting state, breaking time-reversal symmetry; the associated internal magnetic field scale is found to be exceptionally large ($\approx$ 0.18~mT). Furthermore, transverse-field $\mu$SR measurements in the vortex state of Lu$_3$Os$_4$Ge$_{13}$ imply a complex gap function with significantly different strengths on different parts of the Fermi surface. While our measurements do not completely determine the order parameter, they strongly indicate that electron-electron interactions are essential to stabilizing pairing in the system, thus, demonstrating its unconventional nature.Comment: 7 pages, 2 figure

Enhanced skyrmion metastability under applied strain in FeGe

Mechanical straining of skyrmion hosting materials has previously demonstrated increased phase stability through the expansion of the skyrmion equilibrium pocket. Additionally, metastable skyrmions can be generated via rapid field cooling to form significant skyrmion populations at low temperatures. Using small-angle x-ray scattering and x-ray holographic imaging on a thermally strained 200-nm-thick FeGe lamella, we observe temperature-induced strain effects on the structure and metastability of the skyrmion lattice. We find that in this sample orientation ( H ∥ [ ¯ 1 1 0 ] ) with no strain, metastable skyrmions produced by field cooling through the equilibrium skyrmion pocket vanish from the sample upon dropping below the well-known helical reorientation temperature. However, when strain is applied along the [ 1 1 0 ] axis, and this procedure is repeated, a substantial volume fraction of metastable skyrmions persist upon cooling below this temperature down to 100 K. Additionally, we observe a large number of skyrmions retained after a complete magnetic field polarity reversal, implying that the metastable energy barrier protecting skyrmions from decay is enhanced

Real-space imaging of confined magnetic skyrmion tubes

Abstract: Magnetic skyrmions are topologically nontrivial particles with a potential application as information elements in future spintronic device architectures. While they are commonly portrayed as two dimensional objects, in reality magnetic skyrmions are thought to exist as elongated, tube-like objects extending through the thickness of the host material. The study of this skyrmion tube state (SkT) is vital for furthering the understanding of skyrmion formation and dynamics for future applications. However, direct experimental imaging of skyrmion tubes has yet to be reported. Here, we demonstrate the real-space observation of skyrmion tubes in a lamella of FeGe using resonant magnetic x-ray imaging and comparative micromagnetic simulations, confirming their extended structure. The formation of these structures at the edge of the sample highlights the importance of confinement and edge effects in the stabilisation of the SkT state, opening the door to further investigation into this unexplored dimension of the skyrmion spin texture

Phonons in an aperiodic alkane/urea composite crystal studied by inelastic x-ray scattering

International audienceAperiodic composite crystals belong to a new state of matter that possesses long-range order without translational symmetry. We report measurements of low-lying phonon branches in a n-alkane/urea compound that provide a new insight to the urea sub-lattice and the commensurate basal plane dynamics. Focusing on the thoroughly studied n-nonadecane/urea compound makes a comparison with other inelastic scattering results possible, allowing the observation of a new aperiodic elastic signature. Using three techniques, slight but reproducible difference in sound velocities is observed between the transverse mode propagating along the aperiodic direction and polarized in the commensurate basal plane, and the one polarized along the aperiodic direction propagating in the basal plane

Probing spin fluctuations in NaOsO3 by muon spin rotation and NMR spectroscopy

We have used muon spin rotation and relaxation (μSR) and 23Na nuclear magnetic resonance (NMR) spectroscopic methods in the NaOsO3 antiferromagnetic phase to determine the temperature evolution of the magnetic order parameter and the role of the magnetic fluctuations at the Néel temperature. Additionally, we performed muon spin relaxation measurements in the vicinity of TA = 30 K, where the appearance of an anomaly in the electrical resistivity was suggested to be due to a progressive reduction of the Os magnetic moment associated with spin fluctuation. Our measurements suggest the absence of prominent change in the spin fluctuations frequency at TA, within the muon probing time scale and the absence of a reduction of the localized Os magnetic moment reflected by the stability within few permille of the local magnetic field strength sensed by the muons below 50 K

Real-space imaging of confined magnetic skyrmion tubes

Magnetic skyrmions are topologically nontrivial particles with a potential application as information elements in future spintronic device architectures. While they are commonly portrayed as two dimensional objects, in reality magnetic skyrmions are thought to exist as elongated, tube-like objects extending through the thickness of the host material. The study of this skyrmion tube state (SkT) is vital for furthering the understanding of skyrmion formation and dynamics for future applications. However, direct experimental imaging of skyrmion tubes has yet to be reported. Here, we demonstrate the real-space observation of skyrmion tubes in a lamella of FeGe using resonant magnetic x-ray imaging and comparative micromagnetic simulations, confirming their extended structure. The formation of these structures at the edge of the sample highlights the importance of confinement and edge effects in the stabilisation of the SkT state, opening the door to further investigations into this unexplored dimension of the skyrmion spin texture