High intensity x-ray diffraction in transmission mode employing an analog of Poisson's spot

Poisson’s spot is a diffraction phenomenon producing an intensity maximum at the center of the geometric shadow of circular opaque objects. In an analog of the Poisson spot experiment, we show that a tubular cone of x-rays incident upon a crystalline sample produces diffraction spots or foci, corresponding to Bragg maxima within a transmission shadow. We discuss the beam geometry and the intensity gain recorded at the foci in transmission mode. We describe the geometric growth and decay of the foci over a linear axis with the aid of a movie sequence synchronized with the plotting of a diffractogram. The mean signal of a small central area in each successive camera image provides the intensity data for the diffractogram

Probing the size and density of silicon nanocrystals in nanocrystal memory device applications

Structural characterization via transmission electron microscopy and atomic force microscopy of arrays of small Si nanocrystals embedded in SiO2, important to many device applications, is usually difficult and fails to correctly resolve nanocrystal size and density. We demonstrate that scanning tunneling microscopy (STM) imaging enables a much more accurate measurement of the ensemble size distribution and array density for small Si nanocrystals in SiO2, estimated to be 2-3 nm and 4 x 10^(12) - 3 x 10^(13) cm^(-2), respectively, in this study. The reflection high energy electron diffraction pattern further verifies the existence of nanocrystallites in SiO2. The present STM results enable nanocrystal charging characteristics to be more clearly understood: we find the nanocrystal charging measurements to be consistent with single charge storage on individual Si nanocrystals. Both electron tunneling and hole tunneling processes are suggested to explain the asymmetric charging/ discharging processes as a function of bias

Electrooptic Modulation in Thin Film Barium Titanate Plasmonic Interferometers

We demonstrate control of the surface plasmon polariton wavevector in an active metal−dielectric plasmonic interferometer by utilizing electrooptic barium titanate as the dielectric layer. Arrays of subwavelength interferometers were fabricated from pairs of parallel slits milled in silver on barium titanate thin films. Plasmon-mediated transmission of incident light through the subwavelength slits is modulated by an external voltage applied across the barium titanate thin film. Transmitted light modulation is ascribed to two effects, electrically induced domain switching and electrooptic modulation of the barium titanate index

HST and Spitzer point source detection and optical extinction in powerful narrow-line radio galaxies

We present the analysis of infrared HST and Spitzer data for a sample of 13 FRII radio galaxies at 0.03<z<0.11 that are classified as narrow-line radio galaxies (NLRG). In the context of the unified schemes for active galactic nuclei (AGN), our direct view of the AGN in NLRG is impeded by a parsec-scale dusty torus structure. Our high resolution infrared observations provide new information about the degree of extinction induced by the torus, and the incidence of obscured AGN in NLRG. We find that the point-like nucleus detection rate increases from 25 per cent at 1.025$\mu$m, to 80 per cent at 2.05$\mu$m, and to 100 per cent at 8.0$\mu$m. This supports the idea that most NLRG host an obscured AGN in their centre. We estimate the extinction from the obscuring structures using X-ray, near-IR and mid-IR data. We find that the optical extinction derived from the 9.7$\mu$m silicate absorption feature is consistently lower than the extinction derived using other techniques. This discrepancy challenges the assumption that all the mid-infrared emission of NLRG is extinguished by a simple screen of dust at larger radii. This disagreement can be explained in terms of either weakening of the silicate absorption feature by (i) thermal mid-IR emission from the narrow-line region, (ii) non-thermal emission from the base of the radio jets, or (iii) by direct warm dust emission that leaks through a clumpy torus without suffering major attenuation.Comment: 18 pages, 7 figures, 8 tables, accepted for publication in MNRA

X-ray absorption tomography employing a conical shell beam

We demonstrate depth-resolved absorption imaging by scanning an object through a conical shell of X-rays. We measure ring shaped projections and apply tomosynthesis to extract optical sections at different axial focal plane positions. Three-dimensional objects have been imaged to validate our theoretical treatment. The novel principle of our method is scalable with respect to both scan size and X-ray energy. A driver for this work is to complement previously reported methods concerning the measurement of diffracted X-rays for structural analysis. The prospect of employing conical shell beams to combine both absorption and diffraction modalities would provide enhanced analytical utility and has many potential applications in security screening, process control and diagnostic imaging

Study of orientation effect on nanoscale polarization in BaTiO3 thin films using piezoresponse force microscopy

We have investigated the effect of texture on in-plane (IPP) and out- of plane (OPP) polarizations of pulsed-laser-deposited BaTiO3 thin films grown on Pt and La0.5Sr0.5CoO3 (LSCO) buffered Pt electrodes. The OPP and IPP polarizations were observed by piezoresponse force microscopy (PFM) for three-dimensional polarization analyses in conjunction with conventional diffraction methods using x-ray diffraction and reflection high energy electron diffraction measurements. BaTiO3 films grown on Pt electrodes exhibited highly (101) preferred orientation with higher IPP component whereas BaTiO3 film grown on LSCO/Pt electrodes showed (001) and (101) orientations with higher OPP component. Measured effective d(33) values of BaTiO3 films deposited on Pt and LSCO/ Pt electrodes were 14.3 and 54.0 pm/ V, respectively. Local piezoelectric strain loops obtained by OPP and IPP-PFM showed that piezoelectric properties were strongly related to film orientation

Single-Supply Pre-Biasing Circuit for Low-Amplitude Energy Harvesting Applications

Published versio

Clear detection of dusty torus signatures in a Weak-Line Radio Galaxy: the case of PKS 0043-42

We report the clearest detection to date of dusty torus signatures in a Weak-Line Radio Galaxy (WLRG). The deep Spitzer InfraRed Spectrograph (IRS) rest-frame mid-infrared (MIR) spectrum of the WLRG PKS 0043-42 (z=0.116) shows a clear spectral turnover at wavelengths longer than ~20 micron suggestive of warm dust, as well as a 9.7 micron silicate absorption feature. In addition, the hard X-ray results, based on Chandra data, strongly support a picture in which PKS 0043-42 has a torus and accretion disc more typical of Strong-Line Radio Galaxies (SLRGs). The MIR and X-ray spectra are markedly different from those of other WLRGs at similar redshifts, and here we show that the former can be successfully fitted with clumpy torus models with parameters characteristic of Type-2 AGN tori: close to edge-on (i=74 deg) and relatively broad (torus angular width=60 deg), with an outer radius of 2 pc, hydrogen column density ~1.6x10^(23) cm^(-2), and AGN bolometric luminosity ~1.6x10^(44) erg s^(-1). The presence of a compact torus in PKS 0043-42 provides evidence that this WLRG is fuelled by cold, rather than hot, gas accretion. We suggest that WLRGs are a diverse population, and PKS 0043-42 may represent a type of radio galaxy in which the AGN activity has been recently re-triggered as a consequence of intermittent gas supply, or in which the covering factor of the Narrow-Line Region (NLR) clouds is relatively low.Comment: 7 pages, 6 figures, 1 table. Accepted by MNRA

Active plasmonic devices and optical metamaterials

We studied active near-infrared metamaterials based on phase transition of vanadium oxide thin films, asymmetrically coupled split-ring resonators for narrowing resonance line-widths , field effect modulation of plasmon propagation and 3D single layer, plasmonic negative-index metamaterials

A Phase Diagram of Low Temperature Epitaxial Silicon Grown by Hot-wire Chemical Vapor Deposition for Photovoltaic Devices

We have investigated the low-temperature epitaxial growth of thin silicon films by hot-wire chemical vapor deposition (HWCVD). Using reflection high energy electron diffraction (RHEED) and transmission electron microscopy (TEM), we have found conditions for epitaxial growth at low temperatures achieving twinned epitaxial growth up to 6.8 µm on Si(100) substrates at a substrate temperature of 230°C. This opens the possibility of growing high quality films on low cost substrates. The H_2:SiH_4 dilution ratio was set to 50:1 for all growths. Consistent with previous results, the epitaxial thickness is found to decrease with an increase in the substrate temperature