2,400 research outputs found
Surface Plasmon Excitation of Second Harmonic light: Emission and Absorption
We aim to clarify the role that absorption plays in nonlinear optical
processes in a variety of metallic nanostructures and show how it relates to
emission and conversion efficiency. We define a figure of merit that
establishes the structure's ability to either favor or impede second harmonic
generation. Our findings suggest that, despite the best efforts embarked upon
to enhance local fields and light coupling via plasmon excitation, nearly
always the absorbed harmonic energy far surpasses the harmonic energy emitted
in the far field. Qualitative and quantitative understanding of absorption
processes is crucial in the evaluation of practical designs of plasmonic
nanostructures for the purpose of frequency mixing
Spontaneous and Stimulated Raman Scattering near Metal Nanostructures in the Ultrafast, High-Intensity regime
The inclusion of atomic inversion in Raman scattering can significantly alter
field dynamics in plasmonic settings. Our calculations show that large local
fields and femtosecond pulses combine to yield: (i) population inversion within
hot spots; (ii) gain saturation; and (iii) conversion efficiencies
characterized by a switch-like transition to the stimulated regime that spans
twelve orders of magnitude. While in Raman scattering atomic inversion is
usually neglected, we demonstrate that in some circumstances full accounting of
the dynamics of the Bloch vector is required
Harmonic generation and energy transport in dielectric and semiconductors at visible and UV wavelengths: the case of GaP
We study inhibition of absorption, transparency, energy and momentum
transport of the inhomogeneous component of harmonic pulses in dielectrics and
semiconductors, at visible and UV wavelengths, focusing on materials like GaP.
In these spectral regions GaP is characterized by large absorption, metallic
behavior or a combination of both. We show that phase locking causes the
generated inhomogeneous signals to propagate through a bulk metallic medium
without being absorbed, that is occurs even in centrosymmetric materials via
the magnetic Lorentz force, and that the transport of energy and momentum is
quite peculiar and seemingly anomalous. These results make it clear that there
are new opportunities in ultrafast nonlinear optics and nano-plasmonics in new
wavelength ranges.Comment: 16 pages, 5 figures, 1 vide
Accelerated Extraction and Analysis of Ethyl Glucuronide in Hair by Means of Pressurized Liquid Extraction Followed by Liquid Chromatography-Tandem Mass Spectrometry Determination
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