1,738 research outputs found
Transport and recombination through weakly coupled localized spin pairs in semiconductors during coherent spin excitation
Semi-analytical predictions for the transients of spin-dependent transport
and recombination rates through localized states in semiconductors during
coherent electron spin excitation are made for the case of weakly spin-coupled
charge carrier ensembles. The results show that the on-resonant Rabi frequency
of electrically or optically detected spin-oscillation doubles abruptly as the
strength of the resonant microwave field gamma B_1 exceeds the Larmor frequency
separation within the pair of charge carrier states between which the transport
or recombination transition takes place. For the case of a Larmor frequency
separation of the order of gamma B_1 and arbitrary excitation frequencies, the
charge carrier pairs exhibit four different nutation frequencies. From the
calculations, a simple set of equations for the prediction of these frequencies
is derived
Effect of exchange coupling on coherently controlled spin-dependent transition rates
Journal ArticleThe effect of exchange interactions within spin pairs on spin-dependent transport and recombination rates through localized states in semiconductors during coherent electron-spin resonant excitation is studied theoretically. It is shown that for identical spin systems, significant quantitative differences are to be expected between the results of pulsed electrically/optically detected magnetic resonance (pEDMR/pODMR) experiments, where permutation symmetry is the observable, and the results of pulsed electron-spin resonance (pESR) experiments, with polarization in the x-y plane of the rotating frame as the observable. It is predicted that beat oscillations of the spin nutations and not the nutations themselves dominate the transport or recombination rates when the exchange coupling strength or the field strength of the exciting radiation exceed the difference between the Zeeman energies within the spin pair. Furthermore, while the intensities of the rate oscillations decrease with increasing exchange within the spin pairs, the singlet and triplet signals retain their relative strengths. This means that pEDMR and pODMR experiments allow experimental access to ESR forbidden singlet transitions
Electrical detection of 31P spin quantum states
In recent years, a variety of solid-state qubits has been realized, including
quantum dots, superconducting tunnel junctions and point defects. Due to its
potential compatibility with existing microelectronics, the proposal by Kane
based on phosphorus donors in Si has also been pursued intensively. A key issue
of this concept is the readout of the P quantum state. While electrical
measurements of magnetic resonance have been performed on single spins, the
statistical nature of these experiments based on random telegraph noise
measurements has impeded the readout of single spin states. In this letter, we
demonstrate the measurement of the spin state of P donor electrons in silicon
and the observation of Rabi flops by purely electric means, accomplished by
coherent manipulation of spin-dependent charge carrier recombination between
the P donor and paramagnetic localized states at the Si/SiO2 interface via
pulsed electrically detected magnetic resonance. The electron spin information
is shown to be coupled through the hyperfine interaction with the P nucleus,
which demonstrates the feasibility of a recombination-based readout of nuclear
spins
- and -spin relaxation time limitations of phosphorous donor electrons near crystalline silicon to silicon dioxide interface defects
A study of donor electron spins and spin--dependent electronic transitions
involving phosphorous (P) atoms in proximity of the (111) oriented
crystalline silicon (c-Si) to silicon dioxide (SiO) interface is
presented for [P] = 10 and [P] =
10 at about liquid He temperatures (
). Using pulsed electrically detected magnetic
resonance (pEDMR), spin--dependent transitions between the \Phos donor state
and two distinguishable interface states are observed, namely (i) \Pb centers
which can be identified by their characteristic anisotropy and (ii) a more
isotropic center which is attributed to E defects of the \sio bulk
close to the interface. Correlation measurements of the dynamics of
spin--dependent recombination confirm that previously proposed transitions
between \Phos and the interface defects take place. The influence of these
electronic near--interface transitions on the \Phos donor spin coherence time
as well as the donor spin--lattice relaxation time is then
investigated by comparison of spin Hahn--echo decay measurements obtained from
conventional bulk sensitive pulsed electron paramagnetic resonance and surface
sensitive pEDMR, as well as surface sensitive electrically detected inversion
recovery experiments. The measurements reveal that both and of
\Phos donor electrons spins in proximity of energetically lower interface
states at K are reduced by several orders of magnitude
In vivo Neutralization of Pro-inflammatory Cytokines During Secondary Streptococcus pneumoniae Infection Post Influenza A Virus Infection
An overt pro-inflammatory immune response is a key factor contributing to lethal pneumococcal infection in an influenza pre-infected host and represents a potential target for therapeutic intervention. However, there is a paucity of knowledge about the level of contribution of individual cytokines. Based on the predictions of our previous mathematical modeling approach, the potential benefit of IFN-γ- and/or IL-6-specific antibody-mediated cytokine neutralization was explored in C57BL/6 mice infected with the influenza A/PR/8/34 strain, which were subsequently infected with the Streptococcus pneumoniae strain TIGR4 on day 7 post influenza. While single IL-6 neutralization had no effect on respiratory bacterial clearance, single IFN-γ neutralization enhanced local bacterial clearance in the lungs. Concomitant neutralization of IFN-γ and IL-6 significantly reduced the degree of pneumonia as well as bacteremia compared to the control group, indicating a positive effect for the host during secondary bacterial infection. The results of our model-driven experimental study reveal that the predicted therapeutic value of IFN-γ and IL-6 neutralization in secondary pneumococcal infection following influenza infection is tightly dependent on the experimental protocol while at the same time paving the way toward the development of effective immune therapies
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