Femtosecond combs for optical frequency metrology

This thesis is dedicated to femtosecond combs as a tool for optical frequency metrology and as an integral part of an optical clock. After an overview of optical frequency measurement techniques, the design of two frequency combs based on mode-locked femtosecond lasers as they were at the beginning of my project is described. The first comb is based on an Er:fibre laser operating at a central wavelength of 1550 nm with a repetition rate of 100 MHz. The second is a Ti:sapphire-laser-based comb operating at a central wavelength of 810 nm with a repetition rate of 87 MHz. Improvements to the original design of the Ti:sapphire comb are detailed in the next chapter. A novel f-to-2f self-referencing scheme based on a pair of Wollaston prisms and employing a PPKTP crystal for SHG results in up to 20 dB enhancement of the signal to noise ratio in the carrier-envelope offset frequency beat signal f0 and in up to 15 dB lower phase noise in the f0 beat signal compared to a Michelson interferometer based system. Next, the factors influencing the stability and accuracy of the microwave reference signal and the performance of two synthesisers used for the stabilisation of the frequency combs were investigated. It is shown that stability of the maser reference signal is reduced by the distribution system by factor of 1.5. A fractional frequency change of 4.1(0.7) × 10−16 (K/h)−1 was measured for the better of the two synthesisers (an IFR 2023A) indicating that for accurate frequency measurements the synthesiser signal should be monitored to enable systematic frequency corrections to be made. Finally, an absolute frequency measurement of the electric quadrupole clock transition in a frequency standard based on a single 171Yb+ trapped ion is described. The result f = 688 358 979 309 310 ± 9 Hz agrees with an independent measurement made by the PTB group within the uncertainty of the measurements

Phase-stabilized Ultrashort Laser Systems for Spectroscopy

The investigation of laser-matter interactions calls for ever shorter pulses as new effects can thus be explored. With laser pulses consisting of only a few cycles of the electric field, the phase of these electric field oscillations becomes important for many applications. In this thesis ultrafast laser sources are presented that provide few-cycle laser pulses with controlled evolution of the electric field waveform. Firstly, a technique for phasestabilizing ultra-broadband oscillators is discussed. With a simple setup it improves the reproducibility of the phase by an order of magnitude compared to previously existing methods. In a further step, such a phase-stabilized oscillator was integrated into a chirped-pulse amplifier. The preservation of phase-stability during amplification is ensured by secondary phase detection. The phase-stabilized intense laser pulses from this system were employed in a series of experiments that studied strong-field phenomena in a time-resolved manner. For instance, the laser-induced tunneling of electrons from atoms was studied on a sub-femtosecond timescale. Additional evidence for the reproducibility of the electric field waveform of the laser pulses is presented here: individual signatures of the electric field half-cycles were found in photoelectron spectra from above-threshold ionization. Frequency conversion of intense laser pulses by high-order harmonic generation is a common way of producing coherent light in the extreme ultraviolet (XUV) spectral region. Many attempts have been made to increase the low efficiency of this nonlinear process, e.g. by quasi phase-matching. Here, high-harmonic generation from solid surfaces under grazing incidence instead from a gas target is studied as higher efficiencies are expected in this configuration. Another approach to increasing the efficiency of high-harmonic generation is the placing of the gas target in an enhancement resonator. Additionally, the production of XUV photons happens at the full repetition rate of the seeding laser, i.e. in the region of several tens to hundreds of megahertz. This high repetition rate enables the use of the XUV light for high-precision optical frequency metrology with the frequency comb technique. With such an arrangement, harmonics up to 15th order were produced. A build-up cavity that stacks femtosecond laser pulses in a coherent manner to produce intra-cavity pulse energies of more than ten microjoules at a repetition rate of ten megahertz is presented here. With this high average power measuring hitherto uninvestigated optical transition frequencies in the XUV, such as the 1S-2S transition in singly charged helium ions may become a reality

Stable and ultra-stable laser systems for a mobile strontium optical clock

This thesis presents a realisation of the most demanding laser systems for a mobile strontium optical clock. First, stable 689 nm cooling lasers are presented: an amplified semiconductor diode laser and a prototype of the semiconductor disc laser (SDL/VECSEL). The first was stabilised to a novel miniaturised multi-laser frequency stabilisation system that allows to stabilise all the six lasers used in the strontium optical clock. The latter was used for the first time in the second-stage cooling of strontium to obtain a cold cloud of trapped atoms. An atomic optical clock requires a laser oscillator for interrogating the clock transition. This thesis presents the construction and discusses the performance of the cutting-edge ultra-stable interrogation lasers at 698 nm. One of the systems is a stationary system based at the University of Birmingham, with the instability of $5\times10^{-15}$. A mobile version of the interrogation laser is also presented and characterised in this work. The laser reaches instability of $8\times10^{-16}$, which is one of the best results for a mobile system. The mobile laser is a part of the space optical clock project (SOC2), in which a record-low instability for the bosonic strontium was observed of $<4\times10^{-16}/\sqrt{\tau}$

Understanding Quantum Technologies 2022

Understanding Quantum Technologies 2022 is a creative-commons ebook that provides a unique 360 degrees overview of quantum technologies from science and technology to geopolitical and societal issues. It covers quantum physics history, quantum physics 101, gate-based quantum computing, quantum computing engineering (including quantum error corrections and quantum computing energetics), quantum computing hardware (all qubit types, including quantum annealing and quantum simulation paradigms, history, science, research, implementation and vendors), quantum enabling technologies (cryogenics, control electronics, photonics, components fabs, raw materials), quantum computing algorithms, software development tools and use cases, unconventional computing (potential alternatives to quantum and classical computing), quantum telecommunications and cryptography, quantum sensing, quantum technologies around the world, quantum technologies societal impact and even quantum fake sciences. The main audience are computer science engineers, developers and IT specialists as well as quantum scientists and students who want to acquire a global view of how quantum technologies work, and particularly quantum computing. This version is an extensive update to the 2021 edition published in October 2021.Comment: 1132 pages, 920 figures, Letter forma