54,618 research outputs found
Proposal for the determination of nuclear masses by high-precision spectroscopy of Rydberg states
The theoretical treatment of Rydberg states in one-electron ions is
facilitated by the virtual absence of the nuclear-size correction, and
fundamental constants like the Rydberg constant may be in the reach of planned
high-precision spectroscopic experiments. The dominant nuclear effect that
shifts transition energies among Rydberg states therefore is due to the nuclear
mass. As a consequence, spectroscopic measurements of Rydberg transitions can
be used in order to precisely deduce nuclear masses. A possible application of
this approach to the hydrogen and deuterium, and hydrogen-like lithium and
carbon is explored in detail. In order to complete the analysis, numerical and
analytic calculations of the quantum electrodynamic (QED) self-energy remainder
function for states with principal quantum number n=5,...,8 and with angular
momentum L=n-1 and L=n-2 are described (j = L +/- 1/2).Comment: 21 pages; LaTe
Maple procedures for the coupling of angular momenta. VI. LS-jj transformations
Transformation matrices between different coupling schemes are required, if a
reliable classification of the level structure is to be obtained for open-shell
atoms and ions. While, for instance, relativistic computations are
traditionally carried out in jj-coupling, a LSJ coupling notation often occurs
much more appropriate for classifying the valence-shell structure of atoms.
Apart from the (known) transformation of single open shells, however, further
demand on proper transformation coefficients has recently arose from the study
of open d- and f-shell elements, the analysis of multiple--excited levels, or
the investigation on inner-shell phenomena. Therefore, in order to facilitate a
simple access to LS jj transformation matrices, here we present an
extension to the Racah program for the set-up and the transformation of
symmetry-adapted functions. A flexible notation is introduced for defining and
for manipulating open-shell configurations at different level of complexity
which can be extended also to other coupling schemes and, hence, may help
determine an optimum classification of atomic levels and processes in the
future
Helium 2 3S - 2 1S metrology at 1557 nm
An experiment is proposed to excite the 'forbidden' 1s2s 3S1 - 1s2s 1S0
magnetic dipole (M1) transition at 1557 nm in a collimated and slow atomic beam
of metastable helium atoms. It is demonstrated that an excitation rate of 5000
/s can be realised with the beam of a 2W narrowband telecom fiber laser
intersecting the atomic beam perpendicularly. A Doppler-limited sub-MHz
spectroscopic linewidth is anticipated. Doppler-free excitation of 2% of
trapped and cooled atoms may be realised in a one-dimensional optical lattice
geometry, using the 2W laser both for trapping and spectroscopy. The very small
(8 Hz) natural linewidth of this transition presents an opportunity for
accurate tests of atomic structure calculations of the helium atom. A
measurement of the 3He - 4He isotope shift allows for accurate determination of
the difference in nuclear charge radius of both isotopes.Comment: accepted for publication in Europhysics Letter
Accumulation of chromium metastable atoms into an Optical Trap
We report the fast accumulation of a large number of metastable 52Cr atoms in
a mixed trap, formed by the superposition of a strongly confining optical trap
and a quadrupolar magnetic trap. The steady state is reached after about 400
ms, providing a cloud of more than one million metastable atoms at a
temperature of about 100 microK, with a peak density of 10^{18} atoms.m^{-3}.
We have optimized the loading procedure, and measured the light shift of the
5D4 state by analyzing how the trapped atoms respond to a parametric
excitation. We compare this result to a theoretical evaluation based on the
available spectroscopic data for chromium atoms.Comment: 7 pages, 5 Figure
Resonance ionization spectroscopy of thorium isotopes - towards a laser spectroscopic identification of the low-lying 7.6 eV isomer of Th-229
In-source resonance ionization spectroscopy was used to identify an efficient
and selective three step excitation/ionization scheme of thorium, suitable for
titanium:sapphire (Ti:sa) lasers. The measurements were carried out in
preparation of laser spectroscopic investigations for an identification of the
low-lying Th-229m isomer predicted at 7.6 +- 0.5 eV above the nuclear ground
state. Using a sample of Th-232, a multitude of optical transitions leading to
over 20 previously unknown intermediate states of even parity as well as
numerous high-lying odd parity auto-ionizing states were identified. Level
energies were determined with an accuracy of 0.06 cm-1 for intermediate and
0.15 cm-1 for auto-ionizing states. Using different excitation pathways an
assignment of total angular momenta for several energy levels was possible. One
particularly efficient ionization scheme of thorium, exhibiting saturation in
all three optical transitions, was studied in detail. For all three levels in
this scheme, the isotope shifts of the isotopes Th-228, Th-229, and Th-230
relative to Th-232 were measured. An overall efficiency including ionization,
transport and detection of 0.6 was determined, which was predominantly limited
by the transmission of the mass spectrometer ion optics
Highly charged ions: optical clocks and applications in fundamental physics
Recent developments in frequency metrology and optical clocks have been based
on electronic transitions in atoms and singly charged ions as references. These
systems have enabled relative frequency uncertainties at a level of a few parts
in . This accomplishment not only allows for extremely accurate time
and frequency measurements, but also to probe our understanding of fundamental
physics, such as variation of fundamental constants, violation of the local
Lorentz invariance, and forces beyond the Standard Model of Physics. In
addition, novel clocks are driving the development of sophisticated technical
applications. Crucial for applications of clocks in fundamental physics are a
high sensitivity to effects beyond the Standard Model and Einstein's Theory of
Relativity and a small frequency uncertainty of the clock. Highly charged ions
offer both. They have been proposed as highly accurate clocks, since they
possess optical transitions which can be extremely narrow and less sensitive to
external perturbations compared to current atomic clock species. The selection
of highly charged ions in different charge states offers narrow transitions
that are among the most sensitive ones for a change in the fine-structure
constant and the electron-to-proton mass ratio, as well as other new physics
effects. Recent advances in trapping and sympathetic cooling of highly charged
ions will in the future enable high accuracy optical spectroscopy. Progress in
calculating the properties of selected highly charged ions has allowed the
evaluation of systematic shifts and the prediction of the sensitivity to the
"new physics" effects. This article reviews the current status of theory and
experiment in the field.Comment: 53 pages, 16 figures, submitted to RM
Spectroscopy of the a^3\Sigma_u^+ state and the coupling to the X^1\Sigma_g^+ state of K_2
We report on high resolution Fourier-transform spectroscopy of fluorescence
to the a^3\Sigma_u^+ state excited by two-photon or two-step excitation from
the X^1\Sigma_g^+ state to the 2^3\Pi_g state in the molecule K_2. These
spectroscopic data are combined with recent results of Feshbach resonances and
two-color photoassociation spectra for deriving the potential curves of
X^1\Sigma_g^+ and a^3\Sigma_u^+ up to the asymptote. The precise relative
position of the triplet levels with respect of the singlet levels was achieved
by including the excitation energies from the X^1\Sigma_g^+ state to the
2^3\Pi_g state and down to the a^3\Sigma_u^+ state in the simultaneous fit of
both potentials. The derived precise potential curves allow for reliable
modeling of cold collisions of pairs of potassium atoms in their ^2S ground
state
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