Absolute frequency measurements for hyperfine structure determination of the R(26) 62-0 transition at 501.7 nm in molecular iodine

The absolute frequencies of the hyperfine components of the R(26) 62-0 transition in molecular iodine at 501.7 nm are measured for the first time with an optical clockwork based on a femtosecond laser frequency comb generator. The set-up is composed of an Ar+ laser locked to a hyperfine component of the R(26) 62-0 transition detected in a continuously pumped low-pressure cell (0.33 Pa). The detected resonances show a linewidth of 45 kHz (half-width at half-maximum). The uncertainty of the frequency measurement is estimated to be 250 Hz

Fully stabilized mid-infrared frequency comb for high-precision molecular spectroscopy

A fully stabilized mid-infrared optical frequency comb spanning from 2.9 to 3.4 mu m is described in this article. The comb is based on half-harmonic generation in a femtosecond optical parametric oscillator, which transfers the high phase coherence of a fully stabilized near-infrared Er-doped fiber laser comb to the mid-infrared region. The method is simple, as no phase-locked loops or reference lasers are needed. Precise locking of optical frequencies of the mid-infrared comb to the pump comb is experimentally verified at sub-20 mHz level, which corresponds to a fractional statistical uncertainty of 2 x 10(-16) at the center frequency of the mid-infrared comb. The fully stabilized mid-infrared comb is an ideal tool for high-precision molecular spectroscopy, as well as for optical frequency metrology in the mid-infrared region, which is difficult to access with other stabilized frequency comb techniques. (C) 2017 Optical Society of AmericaPeer reviewe

Absolute frequency measurement of molecular transitions by a direct link to a comb generated around 3-µm

A 3-microm continuous-wave difference-frequency source is directly referenced to a mid-infrared optical frequency comb synthesizer by measuring their beat-note signal by a fast HgCdTe detector. Absolute frequency metrology of molecular vibration spectra is demonstrated by locking the 3-microm coherent radiation to the nearest comb tooth and tuning the comb mode spacing across the Doppler-broadened absorption profile of a CH(4) ro-vibrational transition

Development and characterisation of a near-infrared femtosecond optical parametric oscillator frequency comb

This thesis describes a 280 MHz MgO:PPLN-based optical parametric oscillator (OPO) synchronously pumped by a 50 fs Ti:sapphire laser to produce ultrafast pulses in the near-infrared. The OPO tuned over a wavelength range from 1450 - 1550 nm and 1624 - 1750 nm for the signal and idler respectively. The carrier-envelope-offset (CEO) frequency of the signal pulses was stabilised to a 10 MHz reference frequency without f-2f self-referencing, with an RMS phase variation of 0.56 rad over an observation time of 1 second. The relative intensity noise was measured for the CEO-stabilised OPO over an observation time of 64 seconds as 0.04%. The repetition frequency of the OPO was stabilised to 280 MHz using a frequency synthesiser at the eighth harmonic (2.24 GHz). This locking loop had an RMS phase variation of 0.98 mrad over a 1 second observation time. The CEO- and repetition frequencies were then locked simultaneously to a synthesiser referenced to a Rb-disciplined source, to generate a fully stabilised 1.5 μm frequency comb with an absolute uncertainty in comb mode position of 110 Hz. The upper limit for the fractional instability for a comb mode at 200 THz was found to be 2 x 10-11, limited by the stability of the Rb reference. A five-fold increase in comb mode spacing to 1.4 GHz was demonstrated with the stabilised frequency comb. This was achieved using a passive filter cavity, stabilised to a transmission peak via dither locking. The FWHM bandwidth of the optical spectrum for the filtered frequency comb was reduced to 8 nm, however no increase in comb linewidth was observed. An additional experiment was carried out where an external cavity diode laser was frequency-stabilised to a saturated absorption peak in Rb at 780.2 nm using dither locking, providing an optical frequency reference for future OPO frequency combs

Carrier-Envelope Offset Stabilized Ultrafast Diode-Pumped Solid-State Lasers

Optical frequency combs have been revolutionizing many research areas and are finding a growing number of real-world applications. While initially dominated by Ti:Sapphire and fiber lasers, optical frequency combs from modelocked diode-pumped solid-state lasers (DPSSLs) have become an attractive alternative with state-of-the-art performance. In this article, we review the main achievements in ultrafast DPSSLs for frequency combs. We present the current status of carrier-envelope offset (CEO) frequency-stabilized DPSSLs based on various approaches and operating in different wavelength regimes. Feedback to the pump current provides a reliable scheme for frequency comb CEO stabilization, but also other methods with faster feedback not limited by the lifetime of the gain material have been applied. Pumping DPSSLs with high power multi-transverse-mode diodes enabled a new class of high power oscillators and gigahertz repetition rate lasers, which were initially not believed to be suitable for CEO stabilization due to the pump noise. However, this challenge has been overcome, and recently both high power and gigahertz DPSSL combs have been demonstrated. Thin disk lasers have demonstrated the highest pulse energy and average power emitted from any ultrafast oscillator and present a high potential for the future generation of stabilized frequency combs with hundreds of watts average output power

Frequency comb assisted two-photon vibrational spectroscopy

We report a setup for high-resolution two-photon spectroscopy using a mid-infrared continuous wave optical parametric oscillator (CW-OPO) and a near-infrared diode laser as the excitation sources, both of which are locked to fully stabilized optical frequency combs. The diode laser is directly locked to a commercial near-infrared optical frequency comb using an optical phase-locked loop. The near-infrared frequency comb is also used to synchronously pump a degenerate femtosecond optical parametric oscillator to produce a fully stabilized mid-infrared frequency comb. The beat frequency between the mid-infrared comb and the CW-OPO is then stabilized through frequency locking. We used the setup to measure a double resonant two-photon transition to a symmetric vibrational state of acetylene with a sub-Doppler resolution and high signal-to-noise ratio. (C) 2017 Optical Society of AmericaPeer reviewe

Coherent terahertz radiation with 2.8-octave tunability through chip-scale photomixed microresonator optical parametric oscillation

High spectral purity frequency agile room temperature sources in the terahertz spectrum are foundational elements for imaging, sensing, metrology, and communications. Here we present a chip scale optical parametric oscillator based on an integrated nonlinear microresonator that provides broadly tunable single frequency and multi frequency oscillators in the terahertz regime. Through optical to terahertz down conversion using a plasmonic nanoantenna array, coherent terahertz radiation spanning 2.8 octaves is achieved from 330 GHz to 2.3 THz, with 20 GHz cavity mode limited frequency tuning step and 10 MHz intracavity mode continuous frequency tuning range at each step. By controlling the microresonator intracavity power and pump resonance detuning, tunable multi frequency terahertz oscillators are also realized. Furthermore, by stabilizing the microresonator pump power and wavelength, sub 100 Hz linewidth of the terahertz radiation with 10-15 residual frequency instability is demonstrated. The room temperature generation of both single frequency, frequency agile terahertz radiation and multi frequency terahertz oscillators in the chip scale platform offers unique capabilities in metrology, sensing, imaging and communications

High Sensitivity Terahertz Receivers Based on Plasmonic Photoconductors.

Terahertz radiation has unique properties that enable new functionalities for various imaging and sensing applications, such as security screening, bio sensing, medical imaging, and astronomical studies, etc. Despite great benefits that terahertz radiation can offer to these applications, high-power terahertz transmitters and sensitive terahertz receivers are still in demand to realize practical terahertz systems. This PhD research focuses on high sensitivity terahertz receivers based on plasmonic photoconductors. Two types of terahertz receivers have been studied to achieve high terahertz detection sensitivity levels. The first type is photoconductive terahertz receivers, which are widely used for detecting terahertz pulses in time-domain terahertz spectroscopy systems. By utilizing plasmonic contact electrodes in photoconductive terahertz receivers, significantly higher detection sensitivities can be achieved compared to conventional photoconductive terahertz receivers that do not use plasmonic contact electrodes. The second type of terahertz receivers that have been studied is plasmonic heterodyne terahertz receivers, which can be used to detect continuous wave (CW) terahertz radiation and provide accurate intensity and frequency information simultaneously. A novel scheme for heterodyne terahertz receivers based on plasmonic photomixers is presented, which replaces the terahertz local oscillator of conventional heterodyne receivers with two wavelength tunable lasers to provide large dynamic range and broadband operation at room temperature.PhDElectrical EngineeringUniversity of Michigan, Horace H. Rackham School of Graduate Studieshttp://deepblue.lib.umich.edu/bitstream/2027.42/133342/1/niwa_1.pd