Evidence of nitric acid uptake in warm cirrus anvil clouds during the NASA TC4 campaign

Uptake of HNO3 onto cirrus ice may play an important role in tropospheric NOx cycling. Discrepancies between modeled and in situ measurements of gas-phase HNO3 in the troposphere suggest that redistribution and removal mechanisms by cirrus ice have been poorly constrained. Limited in situ measurements have provided somewhat differing results and are not fully compatible with theory developed from laboratory studies. We present new airborne measurements of HNO3 in cirrus clouds from anvil outflow made during the Tropical Composition, Cloud, and Climate Coupling Experiment (TC4). Upper tropospheric (\u3e9 km) measurements made during three flights while repeatedly traversing the same cloud region revealed depletions of gas-phase HNO3 in regions characterized by higher ice water content and surface area. We hypothesize that adsorption of HNO3 onto cirrus ice surfaces could explain this. Using measurements of cirrus ice surface area density and some assumptions about background mixing ratios of gas-phase HNO3, we estimate molecular coverages of HNO 3 on cirrus ice surface in the tropical upper troposphere during the TC4 racetracks to be about 1 × 1013 molecules cm-2. This likely reflects an upper limit because potential dilution by recently convected, scavenged air is ignored. Also presented is an observation of considerably enhanced gas-phase HNO3 at the base of a cirrus anvil suggesting vertical redistribution of HNO3 by sedimenting cirrus particles and subsequent particle sublimation and HNO3 evaporation. The impact of released HNO3, however, appears to be restricted to a very thin layer just below the cloud. Copyright 2010 by the American Geophysical Union

Lidar cloud studies for FIRE and ECLIPS

Optical remote sensing measurements of cirrus cloud properties were collected by one airborne and four ground-based lidar systems over a 32 h period during this case study from the First ISCCP (International Satellite Cloud Climatology Program) Regional Experiment (FIRE) Intensive Field Observation (IFO) program. The lidar systems were variously equipped to collect linear depolarization, intrinsically calibrated backscatter, and Doppler velocity information. Data presented describe the temporal evolution and spatial distribution of cirrus clouds over an area encompassing southern and central Wisconsin. The cirrus cloud types include: dissipating subvisual and thin fibrous cirrus cloud bands, an isolated mesoscale uncinus complex (MUC), a large-scale deep cloud that developed into an organized cirrus structure within the lidar array, and a series of intensifying mesoscale cirrus cloud masses. Although the cirrus frequently developed in the vertical from particle fall-streaks emanating from generating regions at or near cloud tops, glaciating supercooled (-30 to -35 C) altocumulus clouds contributed to the production of ice mass at the base of the deep cirrus cloud, apparently even through riming, and other mechanisms involving evaporation, wave motions, and radiative effects are indicated. The generating regions ranged in scale from approximately 1.0 km cirrus uncinus cells, to organized MUC structures up to approximately 120 km across

Microphysical fundamentals governing cirrus cloud growth: Modeling studies

For application to Global Climate Models, large scale numerical models of cirrus cloud formation and maintenance need to be refined to more reliably simulate the effects and feedbacks of high level clouds. A key aspect is how ice crystal growth is initiated in cirrus, which has started a cloud microphysical controversy between camps either believing that heterogeneous or homogeneous drop freezing is predominantly responsible for cold cirrus ice crystal nucleation. In view of convincing evidence for the existence of highly supercooled cloud droplets in the middle and upper troposphere, however, it is concluded that active ice nuclei are rather scarce at cirrus cloud altitudes, and so a new understanding of cirrus cloud formation is needed. This understanding is sought through an examination of cirrus cloud growth models

Cirrus microphysics and radiative transfer: Cloud field study on October 28, 1986

The radiative properties of cirrus clouds present one of the unresolved problems in weather and climate research. Uncertainties in ice particle amount and size and, also, the general inability to model the single scattering properties of their usually complex particle shapes, prevent accurate model predictions. For an improved understanding of cirrus radiative effects, field experiments, as those of the Cirrus IFO of FIRE, are necessary. Simultaneous measurements of radiative fluxes and cirrus microphysics at multiple cirrus cloud altitudes allows the pitting of calculated versus measured vertical flux profiles; with the potential to judge current cirrus cloud modeling. Most of the problems in this study are linked to the inhomogeneity of the cloud field. Thus, only studies on more homogeneous cirrus cloud cases promises a possibility to improve current cirrus parameterizations. Still, the current inability to detect small ice particles will remain as a considerable handicap

ETO lidar studies of cirrostratus altocumulogenitus: Another role for supercooled liquid water in cirrus cloud formation

Cirrus clouds have traditionally been viewed as cold, wispy, or stratiform ice clouds, typically displaying optical phenomena such as haloes. A composition entirely of hexagonal ice crystals, of one habit or another could only have a transitory existence in cirrus, since the concentrations of ice nuclei (IN) measured by various techniques (at the surface or in the lower troposphere) indicate an enormous number of IN that should be active at cirrus cloud temperatures. In light of recent instrumental aircraft and polarization lidar studies of cirrus clouds, it is clear that highly supercooled cloud droplets can sometimes be a component of cirrus clouds. It remains to be determined if supercooled liquid water (SLW) is present abundantly enough in cirrus to play a significant role in earth's radiance balance, or is merely a curious, infrequent occurrence. To help evaluate this issue, the UH polarization lidar FIRE Extended Time Observation (ETO) of cirrus clouds are being utilized to compile, among other parameters, a climatological record of SLW clouds associated with and within cirrus

Direct Estimate of Cirrus Noise in Herschel Hi-GAL Images

In Herschel images of the Galactic plane and many star forming regions, a major factor limiting our ability to extract faint compact sources is cirrus confusion noise, operationally defined as the "statistical error to be expected in photometric measurements due to confusion in a background of fluctuating surface brightness". The histogram of the flux densities of extracted sources shows a distinctive faint-end cutoff below which the catalog suffers from incompleteness and the flux densities become unreliable. This empirical cutoff should be closely related to the estimated cirrus noise and we show that this is the case. We compute the cirrus noise directly, both on Herschel images from which the bright sources have been removed and on simulated images of cirrus with statistically similar fluctuations. We connect these direct estimates with those from power spectrum analysis, which has been used extensively to predict the cirrus noise and provides insight into how it depends on various statistical properties and photometric operational parameters. We report multi-wavelength power spectra of diffuse Galactic dust emission from Hi-GAL observations at 70 to 500 microns within Galactic plane fields at l= 30 degrees and l= 59 degrees. We find that the exponent of the power spectrum is about -3. At 250 microns, the amplitude of the power spectrum increases roughly as the square of the median brightness of the map and so the expected cirrus noise scales linearly with the median brightness. Generally, the confusion noise will be a worse problem at longer wavelengths, because of the combination of lower angular resolution and the rising power spectrum of cirrus toward lower spatial frequencies, but the photometric signal to noise will also depend on the relative spectral energy distribution of the source compared to the cirrus.Comment: 4 pages (in journal), 3 figures, Astronomy and Astrophysics, accepted for publication 13 May 201

Use of high-resolution measurements for the retrieval of temperature and gas-concentration profiles from outgoing infrared spectra in the presence of cirrus clouds

We explore ways in which high-spectral-resolution measurements can aid in the retrieval of atmospheric temperature and gas-concentration profiles from outgoing infrared spectra when optically thin cirrus clouds are present. Simulated outgoing spectra that contain cirrus are fitted with spectra that do not contain cirrus, and the residuals are examined. For those lines with weighting functions that peak near the same altitude as the thin cirrus, unique features are observed in the residuals. These unique features are highly sensitive to the resolution of the instrumental line shape. For thin cirrus these residual features are narrow (≤0.1 cm-1), so high spectral resolution is required for unambiguous observation. The magnitudes of these unique features are larger than the noise of modern instruments. The sensitivities of these features to cloud height and cloud optical depth are also discussed. Our sensitivity studies show that, when the errors in the estimation of temperature profiles are not large, the dominant contribution to the residuals is the misinterpretation of cirrus. An analysis that focuses on information content is also presented. An understanding of the magnitude of the effect and of its dependence on spectral resolution as well as on spectral region is important for retrieving spacecraft data and for the design of future infrared instruments for forecasting weather and monitoring greenhouse gases

Starburst and cirrus models for submillimeter galaxies

We present radiative transfer models for submillimeter galaxies with spectroscopic redshifts and mid-infrared spectroscopy from Spitzer/IRS and analyze available Spitzer/MIPS 24, 70 and 160mu data. We use two types of starburst models, a cirrus model and a model for the emission of an AGN torus in order to investigate the nature of these objects. We find that for three of the objects (25%) cirrus emission alone can account for the mid-infrared spectrum and the MIPS and submillimeter data. For the remaining objects we find that we need a combination of starburst and cirrus in order to fit simultaneously the multi--wavelength data. We find that the typical submillimeter galaxy has comparable luminosity in the starburst (median L=10^12.5 Lo) and cirrus (median L=10^12.4 Lo) components. This could arise if the galaxies have been forming stars continuously for the last 250Myr with the star formation occurring in the last 5Myr being shrouded by high-optical-depth molecular cloud dust, whereas the rest of the starlight is attenuated by diffuse dust or cirrus with an Av of about 1mag.Comment: 9 pages, AA accepte

FIRE Cirrus on October 28, 1986: LANDSAT; ER-2; King Air; theory

A simultaneous examination was conducted of cirrus clouds in the FIRE Cirrus IFO-I on 10/28/86 using a multitude of remote sensing and in-situ measurements. The focus is cirrus cloud radiative properties and their relationship to cloud microphysics. A key element is the comparison of radiative transfer model calculations and varying measured cirrus radiative properties (emissivity, reflectance vs. wavelength, reflectance vs. viewing angle). As the number of simultaneously measured cloud radiative properties and physical properties increases, more sharply focused tests of theoretical models are possible

Comparison between microphysical model simulation and observed cirrus clouds formation within a volcanic aerosol layer in the Tropical Tropopause Layer

In order to know the formation process of cirrus clouds in tropical tropopause layer, we used a microphysical numerical model to calculate nucleation and growing process of cirrus cloud particles, and compared the results of the model simulations with observed results. The observations compared had been performed at Biak, Indonesia in January 2011. Formation of cirrus clouds was observed by lidar in an aerosol layer at the altitude from 17.5 to 19 km. The backscatter coefficient of cirrus clouds was 10-8~10-7/m/str and number concentration was estimated less than 105/m3. Calculated results by model assumed only heterogeneous nucleation or only homogeneous nucleation (cooling rate \u3c 0.1K/h) show agreements with the observed values. However, if there are solid and liquid aerosol particles, the simulations with heterogeneous nucleation show better agreement with the observation