216 research outputs found
Size-dependent electronic-transport mechanism and sign reversal of magnetoresistance in Nd0.5Sr0.5CoO3
A detailed investigation of electronic-transport properties of Nd0.5Sr0.5CoO3
has been carried out as a function of grain size ranging from micrometer order
down to an average size of 28 nm. Interestingly, we observe a size induced
metal-insulator transition in the lowest grain size sample while the bulk-like
sample is metallic in the whole measured temperature regime. An analysis of the
temperature dependent resistivity in the metallic regime reveals that the
electron-electron interaction is the dominating mechanism while other processes
like electron-magnon and electron-phonon scatterings are also likely to be
present. The fascinating observation of enhanced low temperature upturn and
minimum in resistivity on reduction of grain size is found due to
electron-electron interaction (quantum interference effect). This effect is
attributed to enhanced disorder on reduction of grain size. Interestingly, we
observed a cross over from positive to negative magnetoresistance in the low
temperature regime as the grain size is reduced. This observed sign reversal is
attributed to enhanced phase separation on decreasing the grain size of the
cobaltite
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Hygroscopic growth and activation of HULIS particles: Experimental data and a new iterative parameterization scheme for complex aerosol particles
The hygroscopic growth and activation of two HULIS (HUmic LIke Substance) and one Aerosol-Water-Extract sample, prepared from urban-type aerosol, were investigated. All samples were extracted from filters, redissolved in water and atomized for the investigations presented here. The hygroscopic growth measurements were done using LACIS (Leipzig Aerosol Cloud Interaction Simulator) together with a HH-TDMA (High Humidity Tandem Differential Mobility Analyzer). Hygroscopic growth was determined for relative humidities (RHs) up to 99.75%. The critical diameters for activation were measured for supersaturations between 0.2 and 1%. All three samples showed a similar hygroscopic growth behavior, and the two HULIS samples also were similar in their activation behavior, while the Aerosol-Water-Extract turned out to be more CCN active than the HULIS samples. The experimental data was used to derive parameterizations for the hygroscopic growth and activation of HULIS particles. The concept of ρion (Wex et al., 2007a) and the Szyszkowski-equation (Szyszkowski, 1908; Facchini, 1999) were used for parameterizing the Raoult and the Kelvin (surface tension) terms of the Köhler equation, respectively. This concept proved to be very successful for the HULIS samples in the saturation range from RHs larger than 98% up to activation. It was also shown to work well with data on HULIS taken from literature. Here, different atmospheric life-times and/or different sources for the different samples showed up in different coefficients for the parameterization. However, the parameterization did not work out well for the Aerosol-Water-Extract
Hygroscopic growth and activation of HULIS particles: experimental data and a new iterative parameterization scheme for complex aerosol particles
International audienceThe hygroscopic growth and activation of two HULIS and one Aerosol-Water-Extract sample, prepared from urban-type aerosol, were investigated. All samples were extracted from filters, redissolved in water and atomized for the investigations presented here. The hygroscopic growth measurements were done using LACIS (Leipzig Aerosol Cloud Interaction Simulator) together with a HH-TDMA (High Humidity Tandem Differential Mobility Analyzer). Hygroscopic growth was determined for relative humidities up to 99.75%. The critical diameters for activation were measured using LACIS for supersaturations between 2 and 10 per mill. All three samples showed a similar hygroscopic growth behaviour, and the two HULIS samples also were similar in their activation behavior, while the Aerosol-Water-Extract turned out to be more CCN active than the HULIS samples. The experimental data was used to derive parameterizations for the hygroscopic growth and activation of HULIS particles. The concept of ?ion (Wex et al., 2007a) and the Szyszkowski-equation (Szyszkowski, 1908; Facchini et al., 1999) were used for parameterizing the Raoult and the Kelvin (surface tension) terms of the Köhler equation, respectively. This concept proved to be very successful for the HULIS samples in the saturation range from relative humidities larger than 98% up to activation. However it failed for the Aerosol-Water extract
Calculations of giant magnetoresistance in Fe/Cr trilayers using layer potentials determined from {\it ab-initio} methods
The ab initio full-potential linearized augmented plane-wave method
explicitly designed for the slab geometry was employed to elucidate the
physical origin of the layer potentials for the trilayers nFe/3Cr/nFe(001),
where n is the number of Fe monolayers. The thickness of the transition-metal
ferromagnet has been ranged from up to n=8 while the spacer thickness was
fixed to 3 monolayers. The calculated potentials were inserted in the
Fuchs-Sondheimer formalism in order to calculate the giant magnetoresistance
(GMR) ratio. The predicted GMR ratio was compared with the experiment and the
oscillatory behavior of the GMR as a function of the ferromagnetic layer
thickness was discussed in the context of the layer potentials. The reported
results confirm that the interface monolayers play a dominant role in the
intrinsic GMR.Comment: 17 pages, 7 figures, 3 tables. accepted in J. Phys.: Cond. Matte
Large voltage from spin pumping in magnetic tunnel junctions
We studied the response of a ferromagnet-insulator-normal metal tunnel
structure under an external oscillating radio frequency (R.F.) magnetic field.
The D. C. voltage across the junction is calculated and is found not to
decrease despite the high resistance of the junction; instead, it is of the
order of to , much larger than the experimentally observed
value (100 nano-V) in the "strong coupled" ohmic ferromagnet-normal metal
bilayers. This is consistent with recent experimental results in tunnel
structures, where the voltage is larger than s. The damping and loss of
an external RF field in this structure is calculated
Intrinsic Superconductivity at 25 K in Highly Oriented Pyrolytic Graphite
High resolution magnetoresistance data in highly oriented pyrolytic graphite
thin samples manifest non-homogenous superconductivity with critical
temperature K. These data exhibit: i) hysteretic loops of
resistance versus magnetic field similar to Josephson-coupled grains, ii)
quantum Andreev's resonances and iii) absence of the Schubnikov-de Haas
oscillations. The results indicate that graphite is a system with
non-percolative superconducting domains immersed in a semiconducting-like
matrix. As possible origin of the superconductivity in graphite we discuss
interior-gap superconductivity when two very different electronic masses are
present.Comment: 5 pages, 3 figure
Low frequency 1/f noise in doped manganite grain-boundary junctions
We have performed a systematic analysis of the low frequency 1/f-noise in
single grain boundary junctions in the colossal magnetoresistance material
La_{2/3}Ca_{1/3}MnO_{3-delta}. The grain boundary junctions were formed in
epitaxial La_{2/3}Ca_{1/3}MnO_{3-delta} films deposited on SrTiO_3 bicrystal
substrates and show a large tunneling magnetoresistance of up to 300% at 4.2 K
as well as ideal, rectangular shaped resistance versus applied magnetic field
curves. Below the Curie temperature T_C the measured 1/f noise is dominated by
the grain boundary. The dependence of the noise on bias current, temperature
and applied magnetic field gives clear evidence that the large amount of low
frequency noise is caused by localized sites with fluctuating magnetic moments
in a heavily disordered grain boundary region. At 4.2 K additional temporally
unstable Lorentzian components show up in the noise spectra that are most
likely caused by fluctuating clusters of interacting magnetic moments. Noise
due to fluctuating domains in the junction electrodes is found to play no
significant role.Comment: 9 pages, 7 figure
Ambipolar gate effect and low temperature magnetoresistance of ultrathin La0.8Ca0.2MnO3 Films
Ultrathin La0.8Ca0.2MnO3 films have been measured in a field-effect geometry.
The electric field due to the gate produces a large ambipolar decrease in
resistance at low temperatures. This is attributed to the development of a
pseudogap in the density of states and the couple of localized charge to
strain. The gate effect and mangetoresistance are interpreted in a consistent
framework. The implications for the low temperature behavior of a manganite
film in the two dimensional limit are discussed.Comment: 4 pages, 3 figure
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