Optical vortex mode generation by nanoarrays with a tailored geometry

Light generated with orbital angular momentum, commonly known as an optical vortex, is widely achieved by modifying the phase structure of a conventional laser beam through the utilization of a suitable optical element. In recent research, a process has been introduced that can produce electromagnetic radiation with a helical wave-front directly from a source. The chirally driven optical emission originates from a hierarchy of tailored nanoscale chromophore arrays arranged with a specific propeller-like geometry and symmetry. In particular, a nanoarray composed of n particles requires each component to be held in a configuration with a rotation and associated phase shift of 2 π/n radians with respect to its neighbor. Following initial electronic excitation, each such array is capable of supporting delocalized doubly degenerate excitons, whose azimuthal phase progression is responsible for the helical wave-front. Under identified conditions, the relaxation of the electronically-excited nanoarray produces structured light in a spontaneous manner. Nanoarrays of escalating order, i.e. those containing an increasing number of components, enable access to a set of topological charges of higher order. Practical considerations for the development of this technique are discussed, and potential new applications are identified. © (2014) COPYRIGHT Society of Photo-Optical Instrumentation Engineers (SPIE)

Expanded horizons for generating and exploring optical angular momentum in vortex structures

Spin provides for a well-known extension to the information capacity of nanometer-scale electronic devices. Spin transfer can be effected with high fidelity between quantum dots, this type of emission being primarily associated with emission dipoles. However, in seeking to extend the more common spectroscopic connection of dipole transitions with orbital angular momentum, it has been shown impossible to securely transmit information on any other multipolar basis – partly because point detectors are confined to polarization measurement. Standard polarization methods in optics provide for only two independent degrees of freedom, such as the circular states of opposing handedness associated with photon spin. Complex light beams with structured wave-fronts or vector polarization do, however, offer a basis for additional degrees of freedom, enabling individual photons to convey far more information content. A familiar example is afforded by Laguerre-Gaussian modes, whose helically twisted wave-front and vortex fields are associated with orbital angular momentum. Each individual photon in such a beam has been shown to carry the entire spatial helical-mode information, supporting an experimental basis for sorting beams of different angular momentum content. One very recent development is a scheme for such optical vortices to be directly generated through electronic relaxation processes in structured molecular chromophore arrays. © (2013) COPYRIGHT Society of Photo-Optical Instrumentation Engineers (SPIE)

Extraterrestrial applications of solar optics for interior illumination

Solar optics is a terrestrial technology that has potential extraterrestrial applications. Active solar optics (ASO) and passive solar optics (PSO) are two approaches to the transmission of sunlight to remote interior spaces. Active solar optics is most appropriate for task illumination, while PSO is most appropriate for general illumination. Research into solar optics, motivated by energy conservation, has produced lightweight and low-cost materials, products that have applications to NASA's Controlled Ecological Life Support System (CELSS) program and its lunar base studies. Specifically, prism light guides have great potential in these contexts. Several applications of solar optics to lunar base concepts are illustrated

Encoding of low-quality DNA profiles as genotype probability matrices for improved profile comparisons, relatedness evaluation and database searches

Many DNA profiles recovered from crime scene samples are of a quality that does not allow them to be searched against, nor entered into, databases. We propose a method for the comparison of profiles arising from two DNA samples, one or both of which can have multiple donors and be affected by low DNA template or degraded DNA. We compute likelihood ratios to evaluate the hypothesis that the two samples have a common DNA donor, and hypotheses specifying the relatedness of two donors. Our method uses a probability distribution for the genotype of the donor of interest in each sample. This distribution can be obtained from a statistical model, or we can exploit the ability of trained human experts to assess genotype probabilities, thus extracting much information that would be discarded by standard interpretation rules. Our method is compatible with established methods in simple settings, but is more widely applicable and can make better use of information than many current methods for the analysis of mixed-source, low-template DNA profiles. It can accommodate uncertainty arising from relatedness instead of or in addition to uncertainty arising from noisy genotyping. We describe a computer program GPMDNA, available under an open source license, to calculate LRs using the method presented in this paper.Comment: 28 pages. Accepted for publication 2-Sep-2016 - Forensic Science International: Genetic

Hyper-Rayleigh scattering in centrosymmetric systems

Hyper-Rayleigh scattering (HRS) is an incoherent mechanism for optical second harmonic generation. The frequency-doubled light that emerges from this mechanism is not emitted in a laser-like manner, in the forward direction; it is scattered in all directions. The underlying theory for this effect involves terms that are quadratic in the incident field and involves an even-order optical susceptibility (for a molecule, its associated hyperpolarizability). In consequence, HRS is often regarded as formally forbidden in centrosymmetric media. However, for the fundamental three-photon interaction, theory based on the standard electric dipole approximation, representable as E13, does not account for all experimental observations. The relevant results emerge upon extending the theory to include E12M1 and E12E2 contributions, incorporating one magnetic dipolar or electric quadrupolar interaction, respectively, to a consistent level of multipolar expansion. Both additional interactions require the deployment of higher orders in the multipole expansion, with the E12E2 interaction analogous in rank and parity to a four-wave susceptibility. To elicit the correct form of response from fluid or disordered media invites a tensor representation which does not oversimplify the molecular components, yet which can produce results to facilitate the interpretation of experimental observations. The detailed derivation in this work leads to results which are summarized for the following: perpendicular detection of polarization components both parallel and perpendicular to the pump radiation, leading to distinct polarization ratio results, as well as a reversal ratio for forward scattered circular polarizations. The results provide a route to handling data with direct physical interpretation, to enable the more sophisticated design of molecules with sought nonlinear optical properties

Nanoarrays for the generation of complex optical wave-forms

Light beams with unusual forms of wavefront offer a host of useful features to extend the repertoire of those developing new optical techniques. Complex, non-uniform wavefront structures offer a wide range of optomechanical applications, from microparticle rotation, traction and sorting, through to contactless microfluidic motors. Beams combining transverse nodal structures with orbital angular momentum, or vector beams with novel polarization profiles, also present new opportunities for imaging and the optical transmission of information, including quantum entanglement effects. Whilst there are numerous well-proven methods for generating light with complex wave-forms, most current methods work on the basis of modifying a conventional Hermite-Gaussian beam, by passage through suitably tailored optical elements. It has generally been considered impossible to directly generate wave-front structured beams either by spontaneous or stimulated emission from individual atoms, ions or molecules. However, newly emerged principles have shown that emitter arrays, cast in an appropriately specified geometry, can overcome the obstacles: one possibility is a construct based on the electronic excitation of nanofabricated circular arrays. Recent experimental work has extended this concept to a phase-imprinted ring of apertures holographically encoded in a diffractive mask, generated by a programmed spatial light modulator. These latest advances are potentially paving the way for creating new sources of structured light