109 research outputs found
Feasibility of isotope harvesting at a projectile fragmentation facility: ⁶⁷Cu
The work presented here describes a proof-of-principle experiment for the chemical extraction of (67)Cu from an aqueous beam stop at the National Superconducting Cyclotron Laboratory (NSCL). A 76 MeV/A (67)Cu beam was stopped in water, successfully isolated from the aqueous solution through a series of chemical separations involving a chelating disk and anion exchange chromatography, then bound to NOTA-conjugated Herceptin antibodies, and the bound activity was validated using instant thin-layer chromatography (ITLC). The chemical extraction efficiency was found to be 88 ± 3% and the radiochemical yield was ≥95%. These results show that extraction of radioisotopes from an aqueous projectile-fragment beam dump is a feasible method for obtaining radiochemically pure isotopes
Ground-state proton decay of 69Br and implications for the rp-process 68Se waiting-point
The first direct measurement of the proton separation energy, Sp, for the
proton-unbound nucleus 69Br is reported. Of interest is the exponential
dependence of the 2p-capture rate on Sp which can bypass the 68Se waiting-point
in the astrophysical rp process. An analysis of the observed proton decay
spectrum is given in terms of the 69Se mirror nucleus and the influence of Sp
is explored within the context of a single-zone X-ray burst model.Comment: 6 pages, 6 figures, INPC 2010 conference proceeding
Investigations of three, four, and five-particle exit channels of levels in light nuclei created using a 9C beam
The interactions of a E/A=70-MeV 9C beam with a Be target was used to
populate levels in Be, B, and C isotopes which undergo decay into many-particle
exit channels. The decay products were detected in the HiRA array and the level
energies were identified from their invariant mass. Correlations between the
decay products were examined to deduce the nature of the decays, specifically
to what extent all the fragments were created in one prompt step or whether the
disintegration proceeded in a sequential fashion through long-lived
intermediate states. In the latter case, information on the spin of the level
was also obtained. Of particular interest is the 5-body decay of the 8C ground
state which was found to disintegrate in two steps of two-proton decay passing
through the 6Beg.s. intermediate state. The isobaric analog of 8Cg.s. in 8B was
also found to undergo two-proton decay to the isobaric analog of 6Beg.s. in
6Li. A 9.69-MeV state in 10C was found to undergo prompt 4-body decay to the
2p+2alpha exit channel. The two protons were found to have a strong
enhancementin the diproton region and the relative energies of all four p-alpha
pairs were consistent with the 5Lig.s. resonance
Angular Dependence in Proton-Proton Correlation Functions in Central and Reactions
The angular dependence of proton-proton correlation functions is studied in
central and nuclear reactions at E=80
MeV/A. Measurements were performed with the HiRA detector complemented by the
4 Array at NSCL. A striking angular dependence in the laboratory frame is
found within p-p correlation functions for both systems that greatly exceeds
the measured and expected isospin dependent difference between the neutron-rich
and neutron-deficient systems. Sources measured at backward angles reflect the
participant zone of the reaction, while much larger sources observed at forward
angles reflect the expanding, fragmenting and evaporating projectile remnants.
The decrease of the size of the source with increasing momentum is observed at
backward angles while a weaker trend in the opposite direction is observed at
forward angles. The results are compared to the theoretical calculations using
the BUU transport model.Comment: 8 pages, 3 figures, submitted to PR
Heated nuclear matter, condensation phenomena and the hadronic equation of state
The thermodynamic properties of heated nuclear matter are explored using an
exactly solvable canonical ensemble model. This model reduces to the results of
an ideal Fermi gas at low temperatures. At higher temperatures, the
fragmentation of the nuclear matter into clusters of nucleons leads to features
that resemble a Bose gas. Some parallels of this model with the phenomena of
Bose condensation and with percolation phenomena are discussed. A simple
expression for the hadronic equation of state is obtained from the model.Comment: 12 pages, revtex, 1 ps file appended (figure 1
Spin alignment of excited projectiles due to target spin-flip interactions
The sequential breakup of E/A=65.5-MeVBe7 and E/A=36.6-MeVLi6 projectiles excited through inelastic interactions with Be9 target nuclei has been studied. For events where the target nucleus remained in its ground state, significant alignment of the excited projectile\u27s spin axis parallel or antiparallel to the beam direction was observed. This unusual spin alignment was found to be largely independent of the projectile\u27s scattering angle and it was deduced that the target nucleus has a significant probability of changing its spin orientation during the interaction. It is proposed that the unusual spin alignment is a consequence of the molecular structure of the Be9 nucleus
Extended Hauser-Feshbach Method for Statistical Binary-Decay of Light-Mass Systems
An Extended Hauser-Feshbach Method (EHFM) is developed for light heavy-ion
fusion reactions in order to provide a detailed analysis of all the possible
decay channels by including explicitly the fusion-fission phase-space in the
description of the cascade chain. The mass-asymmetric fission component is
considered as a complex-fragment binary-decay which can be treated in the same
way as the light-particle evaporation from the compound nucleus in
statistical-model calculations. The method of the phase-space integrations for
the binary-decay is an extension of the usual Hauser-Feshbach formalism to be
applied to the mass-symmetric fission part. The EHFM calculations include
ground-state binding energies and discrete levels in the low excitation-energy
regions which are essential for an accurate evaluation of the phase-space
integrations of the complex-fragment emission (fission). In the present
calculations, EHFM is applied to the first-chance binary-decay by assuming that
the second-chance fission decay is negligible. In a similar manner to the
description of the fusion-evaporation process, the usual cascade calculation of
light-particle emission from the highly excited complex fragments is applied.
This complete calculation is then defined as EHFM+CASCADE. Calculated
quantities such as charge-, mass- and kinetic-energy distributions are compared
with inclusive and/or exclusive data for the S+Mg and
Cl+C reactions which have been selected as typical examples.
Finally, the missing charge distributions extracted from exclusive measurements
are also successfully compared with the EHFM+CASCADE predictions.Comment: 34 pages, 6 Figures available upon request, Phys. Rev. C (to be
published
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