1,003 research outputs found
Edge Dynamics in a Quantum Spin Hall State: Effects from Rashba Spin-Orbit Interaction
We analyze the dynamics of the helical edge modes of a quantum spin Hall
state in the presence of a spatially non-uniform Rashba spin-orbit (SO)
interaction. A randomly fluctuating Rashba SO coupling is found to open a
scattering channel which causes localization of the edge modes for a weakly
screened electron-electron (e-e) interaction. A periodic modulation of the SO
coupling, with a wave number commensurate with the Fermi momentum, makes the
edge insulating already at intermediate strengths of the e-e interaction. We
discuss implications for experiments on edge state transport in a HgTe quantum
well.Comment: 4 pages, 2 figures; published versio
Single particle analysis of the accumulation mode aerosol over the northeast Amazonian tropical rain forest, Surinam, South America
International audienceSingle particle analysis of aerosols particles larger than 0.2 ?m diameter was performed on 24 samples collected over Surinam tropical rain forest and in the adjacent marine boundary layer (MBL) during the LBA-CLAIRE 98 campaign in March 1998. Elemental composition and morphology of 2308 particles was determined using SEM-EDX. The aerosol particles were divided into seven groups according to their chemical composition: organic particles, mineral dust, aged mineral dust, sea salt, aged sea salt, Ca-rich, and biogenic aerosol. However the organic material in aerosol particles cannot be identified directly by SEM-EDX, we present indirect method of detection of organic material using this technique. Samples were further divided with respect to the distinct atmospheric layers present in the tropical troposphere including MBL, continental mixed layer, cloud convective layer, free troposphere and region of deep convection outflow. The organic and mineral dust particles are two major groups observed over the rainforest. In the MBL also sea salt particles represented a large fraction between 15 and 27%. The organic particles control much of the chemical characteristic of the aerosol in the continental tropical troposphere. Their abundance ranged from less than 20% in the MBL to more than 90% in the free troposphere between 4.5- and 12.6-km altitude. During the transport of the air masses from the MBL over the rain forest, fraction of organic aerosol particles more than doubled, reaching 40?60% in the continental boundary layer. This increase was attributed to direct emissions of biogenic aerosols from the tropical vegetation. The high fraction of the organic accumulation mode particles in the upper tropical troposphere could be a good indicator for the air masses originated over the tropical rain forest
A review of sea-spray aerosol source functions using a large global set of sea salt aerosol concentration measurements
Sea-spray aerosols (SSA) are an important part of the climate system because
of their effects on the global radiative budget – both directly as scatterers and
absorbers of solar and terrestrial radiation, and indirectly as cloud
condensation nuclei (CCN) influencing cloud formation, lifetime, and
precipitation. In terms of their global mass, SSA have the largest
uncertainty of all aerosols. In this study we review 21 SSA source functions
from the literature, several of which are used in current climate models. In
addition, we propose a~new function. Even excluding outliers, the global annual
SSA mass produced spans roughly 3–70 Pg yr<sup>−1</sup> for the different
source functions, for particles with dry diameter <i>D</i><sub>p</sub> < 10 μm,
with relatively little interannual variability for a given
function. The FLEXPART Lagrangian particle dispersion model was run in
backward mode for a large global set of observed SSA concentrations,
comprised of several station networks and ship cruise measurement campaigns.
FLEXPART backward calculations produce gridded emission sensitivity fields,
which can subsequently be multiplied with gridded SSA production fluxes in order to
obtain modeled SSA concentrations. This allowed us to efficiently and simultaneously evaluate all
21 source functions against the measurements. Another
advantage of this method is that source-region information on wind speed and
sea surface temperatures (SSTs) could be stored and used for improving the
SSA source function parameterizations. The best source functions reproduced
as much as 70% of the observed SSA concentration variability at
several stations, which is comparable with "state of the art" aerosol
models. The main driver of SSA production is wind, and we found that the best
fit to the observation data could be obtained when the SSA production is
proportional to <i>U</i><sub>10</sub><sup>3.5</sup>, where
<i>U</i><sub>10</sub> is the source region averaged
10 m wind speed. A strong influence of SST on SSA production, with
higher temperatures leading to higher production, could be detected as well,
although the underlying physical mechanisms of the SST influence remains
unclear. Our new source function with wind speed and temperature dependence
gives a global SSA production for particles smaller than
<i>D</i><sub>p</sub> < 10 μm of 9 Pg yr<sup>−1</sup>, and is the best fit to the observed
concentrations
Changes in aerosol properties during spring-summer period in the Arctic troposphere
The change in aerosol properties during the transition from the more polluted spring to the clean summer in the Arctic troposphere was studied. A six-year data set of observations from Ny-Ã…lesund on Svalbard, covering the months April through June, serve as the basis for the characterisation of this time period. In addition four-day-back trajectories were used to describe air mass histories. The observed transition in aerosol properties from an accumulation-mode dominated distribution to an Aitken-mode dominated distribution is discussed with respect to long-range transport and influences from natural and anthropogenic sources of aerosols and pertinent trace gases. Our study shows that the air-mass transport is an important factor modulating the physical and chemical properties observed. However, the air-mass transport cannot alone explain the annually repeated systematic and rather rapid change in aerosol properties, occurring within a limited time window of approximately 10 days. With a simplified phenomenological model, which delivers the nucleation potential for new-particle formation, we suggest that the rapid shift in aerosol microphysical properties between the Arctic spring and summer is mainly driven by the incoming solar radiation in concert with transport of precursor gases and changes in condensational sink
Sputtering of polished EUROFER97 steel: Surface structure modification and enrichment with tungsten and tantalum
Arctic smoke - aerosol characteristics during a record smoke event in the European Arctic and its radiative impact
In early May 2006 a record high air pollution event was observed at Ny-Ålesund, Spitsbergen. An atypical weather pattern established a pathway for the rapid transport of biomass burning aerosols from agricultural fires in Eastern Europe to the Arctic. Atmospheric stability was such that the smoke was constrained to low levels, within 2 km of the surface during the transport. A description of this smoke event in terms of transport and main aerosol characteristics can be found in Stohl et al. (2007). This study puts emphasis on the radiative effect of the smoke. The aerosol number size distribution was characterised by lognormal parameters as having an accumulation mode centered around 165–185 nm and almost 1.6 for geometric standard deviation of the mode. Nucleation and small Aitken mode particles were almost completely suppressed within the smoke plume measured at Ny-Ålesund. Chemical and microphysical aerosol information obtained at Mt. Zeppelin (474 m a.s.l) was used to derive input parameters for a one-dimensional radiation transfer model to explore the radiative effects of the smoke. The daily mean heating rate calculated on 2 May 2006 for the average size distribution and measured chemical composition reached 0.55 K day−1 at 0.5 km altitude for the assumed external mixture of the aerosols but showing much higher heating rates for an internal mixture (1.7 K day−1). In comparison a case study for March 2000 showed that the local climatic effects due to Arctic haze, using a regional climate model, HIRHAM, amounts to a maximum of 0.3 K day−1 of heating at 2 km altitude (Treffeisen et al., 2005)
Electrical control of the Kondo effect in a helical edge liquid
Magnetic impurities affect the transport properties of the helical edge
states of quantum spin Hall insulators by causing single-electron
backscattering. We study such a system in the presence of a Rashba spin-orbit
interaction induced by an external electric field, showing that this can be
used to control the Kondo temperature, as well as the correction to the
conductance due to the impurity. Surprisingly, for a strongly anisotropic
electron-impurity spin exchange, Kondo screening may get obstructed by the
presence of a non-collinear spin interaction mediated by the Rashba coupling.
This challenges the expectation that the Kondo effect is stable against
time-reversal invariant perturbations.Comment: 7 pages, 2 figures. Expression for the current operator corrected.
(Conclusions unaffected.) Erratum to be publishe
Effects of relative humidity on aerosol light scattering in the Arctic
Aerosol particles experience hygroscopic growth in the ambient atmosphere. Their optical properties – especially the aerosol light scattering – are therefore strongly dependent on the ambient relative humidity (RH). In-situ light scattering measurements of long-term observations are usually performed under dry conditions (RH&gt;30–40%). The knowledge of this RH effect is of eminent importance for climate forcing calculations or for the comparison of remote sensing with in-situ measurements. This study combines measurements and model calculations to describe the RH effect on aerosol light scattering for the first time for aerosol particles present in summer and fall in the high Arctic. For this purpose, a field campaign was carried out from July to October 2008 at the Zeppelin station in Ny-Ålesund, Svalbard. The aerosol light scattering coefficient &sigma;<sub>sp</sub>(&lambda;) was measured at three distinct wavelengths (λ=450, 550, and 700 nm) at dry and at various, predefined RH conditions between 20% and 95% with a recently developed humidified nephelometer (WetNeph) and with a second nephelometer measuring at dry conditions with an average RH&lt;10% (DryNeph). In addition, the aerosol size distribution and the aerosol absorption coefficient were measured. The scattering enhancement factor <i>f</i>(RH, &lambda;) is the key parameter to describe the RH effect on &sigma;<sub>sp</sub>(&lambda;) and is defined as the RH dependent &sigma;<sub>sp</sub>(RH, &lambda;) divided by the corresponding dry &sigma;<sub>sp</sub>(RH<sub>dry</sub>, &lambda;). During our campaign the average <i>f</i>(RH=85%, λ=550 nm) was 3.24&plusmn;0.63 (mean &plusmn; standard deviation), and no clear wavelength dependence of <i>f</i>(RH, &lambda;) was observed. This means that the ambient scattering coefficients at RH=85% were on average about three times higher than the dry measured in-situ scattering coefficients. The RH dependency of the recorded <i>f</i>(RH, &lambda;) can be well described by an empirical one-parameter equation. We used a simplified method to retrieve an apparent hygroscopic growth factor <i>g</i>(RH), defined as the aerosol particle diameter at a certain RH divided by the dry diameter, using the WetNeph, the DryNeph, the aerosol size distribution measurements and Mie theory. With this approach we found, on average, <i>g</i>(RH=85%) values to be 1.61&plusmn;0.12 (mean&plusmn;standard deviation). No clear seasonal shift of <i>f</i>(RH, &lambda;) was observed during the 3-month period, while aerosol properties (size and chemical composition) clearly changed with time. While the beginning of the campaign was mainly characterized by smaller and less hygroscopic particles, the end was dominated by larger and more hygroscopic particles. This suggests that compensating effects of hygroscopicity and size determined the temporal stability of <i>f</i>(RH, &lambda;). During sea salt influenced periods, distinct deliquescence transitions were observed. At the end we present a method on how to transfer the dry in-situ measured aerosol scattering coefficients to ambient values for the aerosol measured during summer and fall at this location
Spatial and temporal distribution of atmospheric aerosols in the lowermost troposphere over the Amazonian tropical rainforest
International audienceWe present measurements of aerosol physico-chemical properties below 5 km altitude over the tropical rain forest and the marine boundary layer (MBL) obtained during the LBA-CLAIRE 1998 project. The MBL aerosol size distribution some 50-100km of the coast of French Guyana and Suriname showed a bi-modal shape typical of aged and cloud processed aerosol. The average particle number density in the MBL was 383cm-3. The daytime mixed layer height over the rain forest for undisturbed conditions was estimated to be between 1200-1500m. During the morning hours the height of the mixed layer increased by 144-180mh-1. The median daytime aerosol number density in the mixed layer increased from 450cm-3 in the morning to almost 800cm-3 in the late afternoon. The evolution of the aerosol size distribution in the daytime mixed layer over the rain forest showed two distinct patterns. Between dawn and midday, the Aitken mode particle concentrations increased, whereas later during the day, a sharp increase of the accumulation mode aerosol number densities was observed, resulting in a doubling of the morning accumulation mode concentrations from 150cm-3 to 300cm-3. Potential sources of the Aitken mode particles are discussed here including the rapid growth of ultrafine aerosol particles formed aloft and subsequently entrained into the mixed layer, as well as the contribution of emissions from the tropical vegetation to Aitken mode number densities. The observed increase of the accumulation mode aerosol number densities is attributed to the combined effect of: the direct emissions of primary biogenic particles from the rain forest and aerosol in-cloud processing by shallow convective clouds. Based on the similarities among the number densities, the size distributions and the composition of the aerosol in the MBL and the nocturnal residual layer we propose that the air originating in the MBL is transported above the nocturnal mixed layer up to 300-400km inland over the rain forest by night without significant processing
- …