Publisher Correction: Coherent diffractive imaging of single helium nanodroplets with a high harmonic generation source

In the original version of this Article, the affiliation for Luca Poletto was incorrectly given as ‘European XFEL GmbH, Holzkoppel 4, 22869 Schenefeld, Hamburg, Germany’, instead of the correct ‘CNR, Istituto di Fotonica e Nanotecnologie Padova, Via Trasea 7, 35131 Padova, Italy’. This has now been corrected in both the PDF and HTML versions of the Article

Three-Dimensional Shapes of Spinning Helium Nanodroplets

A significant fraction of superfluid helium nanodroplets produced in a free-jet expansion have been observed to gain high angular momentum resulting in large centrifugal deformation. We measured single-shot diffraction patterns of individual rotating helium nanodroplets up to large scattering angles using intense extreme ultraviolet light pulses from the FERMI free-electron laser. Distinct asymmetric features in the wide-angle diffraction patterns enable the unique and systematic identification of the three-dimensional droplet shapes. The analysis of a large dataset allows us to follow the evolution from axisymmetric oblate to triaxial prolate and two-lobed droplets. We find that the shapes of spinning superfluid helium droplets exhibit the same stages as classical rotating droplets while the previously reported metastable, oblate shapes of quantum droplets are not observed. Our three-dimensional analysis represents a valuable landmark for clarifying the interrelation between morphology and superfluidity on the nanometer scale

Deep neural networks for classifying complex features in diffraction images

Intense short-wavelength pulses from free-electron lasers and high-harmonic-generation sources enable diffractive imaging of individual nano-sized objects with a single x-ray laser shot. The enormous data sets with up to several million diffraction patterns represent a severe problem for data analysis, due to the high dimensionality of imaging data. Feature recognition and selection is a crucial step to reduce the dimensionality. Usually, custom-made algorithms are developed at a considerable effort to approximate the particular features connected to an individual specimen, but facing different experimental conditions, these approaches do not generalize well. On the other hand, deep neural networks are the principal instrument for today's revolution in automated image recognition, a development that has not been adapted to its full potential for data analysis in science. We recently published in Langbehn et al. (Phys. Rev. Lett. 121, 255301 (2018)) the first application of a deep neural network as a feature extractor for wide-angle diffraction images of helium nanodroplets. Here we present the setup, our modifications and the training process of the deep neural network for diffraction image classification and its systematic benchmarking. We find that deep neural networks significantly outperform previous attempts for sorting and classifying complex diffraction patterns and are a significant improvement for the much-needed assistance during post-processing of large amounts of experimental coherent diffraction imaging data.Comment: Published Version. Github code available at: https://github.com/julian-carpenter/airyne

The Low Density Matter (LDM) beamline at FERMI: Optical layout and first commissioning

The Low Density Matter (LDM) beamline has been built as part of the FERMI free-electron laser (FEL) facility to serve the atomic, molecular and cluster physics community. After the commissioning phase, it received the first external users at the end of 2012. The design and characterization of the LDM photon transport system is described, detailing the optical components of the beamline

Ultrafast Nuclear Dynamics in Double-Core Ionized Water Molecules

Double-core-hole (DCH) states in isolated water and heavy water molecules, resulting from the sequential absorption of two x-ray photons, have been investigated. A comparison of the subsequent Auger emission spectra from the two isotopes provides direct evidence of ultrafast nuclear motion during the 1.5 fs lifetime of these DCH states. Our numerical results align well with the experimental data, providing for various DCH states an in-depth study of the dynamics responsible of the observed isotope effect

Resonance-Enhanced Multiphoton Ionization in the X-Ray Regime

Here, we report on the nonlinear ionization of argon atoms in the short wavelength regime using ultraintense x rays from the European XFEL. After sequential multiphoton ionization, high charge states are obtained. For photon energies that are insufficient to directly ionize a 1s electron, a different mechanism is required to obtain ionization to Ar17+. We propose this occurs through a two-color process where the second harmonic of the FEL pulse resonantly excites the system via a 1s -> 2p transition followed by ionization by the fundamental FEL pulse, which is a type of x-ray resonance-enhanced multiphoton ionization (REMPI). This resonant phenomenon occurs not only for Ar16+, but also through lower charge states, where multiple ionization competes with decay lifetimes, making x-ray REMPI distinctive from conventional REMPI. With the aid of state-of-the-art theoretical calculations, we explain the effects of x-ray REMPI on the relevant ion yields and spectral profile

The Small Quantum Systems - SQS Instrument at the European X-Ray Free Electron Laser

This contribution will present the Small Quantum System (SQS) scientific instrument, which is one of six experimental end stations at the European XFEL planned to open for user operation in autumn 2017. This experimental platform is designed for investigations of atomic and molecular systems, as well as clusters, nano-particles and small bio-molecules. It is located behind the SASE 3 soft x-ray undulator, which will provide horizontally polarized FEL radiation in a photon energy range between 260 eV and 3000 eV (4.8 nm to 0.4 nm) with 0.1 to 2 × 10e14 photons per pulse and up to 27000 pulses per second. Two high-quality elliptical mirrors in Kirkpatrick-Baez configuration will focus the FEL beam to a FWHM spot size of approximately 1 µm diameter. This is going to result in an intensity of more than 10e18 W/cm2 within the interaction region, which will allow for studying non-linear multi-photon processes. Furthermore, the short FEL pulse duration between 2 fs and 100 fs in combination with a synchronized optical femtosecond laser will enable time-resolved studies of dynamic processes, thus capturing the motion of electrons and nuclei with unprecedented resolution in space on ultrafast time scales

The Small Quantum Systems - SQS Instrument at the European XFEL

This contribution will present the Small Quantum System (SQS) scientific instrument, which is one of six experimental end stations at the European XFEL planned to open for user operation in autumn 2017. This experimental platform is designed for investigations of atomic and molecular systems, as well as clusters, nano-particles and small bio-molecules. It is located behind the SASE 3 soft x-ray undulator, which will provide horizontally polarized FEL radiation in a photon energy range between 260 and 3000 (4.8 to 0.4) with 0.1 to 2 × 10e14 photons per pulse and up to 27000 pulses per second. Two high-quality elliptical mirrors in Kirkpatrick-Baez configuration will focus the FEL beam to a FWHM spot size of approximately 1 diameter. This is going to result in an intensity of more than 10e18/2 within the interaction region, which will allow for studying non-linear multi-photon processes. Furthermore, the short FEL pulse duration between 2 and 100 in combination with a synchronized optical femtosecond laser will enable time-resolved studies of dynamic processes, thus capturing the motion of electrons and nuclei with unprecedented resolution in space on ultrafast time scales

The beam transport system for the Small Quantum Systems instrument at the European XFEL: optical layout and first commissioning results

The Small Quantum Systems instrument is one of the six operating instruments of the European XFEL, dedicated to the atomic, molecular and cluster physics communities. The instrument started its user operation at the end of 2018 after a commissioning phase. The design and characterization of the beam transport system are described here. The X-ray optical components of the beamline are detailed, and the beamline performances, transmission and focusing capabilities are reported. It is shown that the X-ray beam can be effectively focused as predicted by ray-tracing simulations. The impact of non-ideal X-ray source conditions on the focusing performances is discussed.Deutsche Forschungsgemeinschaft https://doi.org/10.13039/501100001659Volkswagen Foundation https://doi.org/10.13039/501100001663Horizon 2020 Framework Programme, European Metrology Programme for Innovation and Research https://doi.org/10.13039/100014132Deutsche Forschungsgemeinschaft https://doi.org/10.13039/50110000165