Current-driven magnetization decrease in single crystalline ferromagnetic manganese oxide

The electrical and magnetic response to a bias current has been investigated in a singlecrystalline ferromagnetic manganese oxide $\Pr_{0.8}$Ca$_{0.2}$MnO$_3$ . A significant decrease of the magnetization is observed at the same threshold current where a non-linearity of V-I characteristics appears. Such a behavior cannot be understood in the framework of the filamentary picture usually invoked for the non linearity of the other manganese oxides. Instead, an analogy with spintronic features might be useful and experimental signatures seem to be in agreement with excitations of spin waves by an electric current. This provides an example of a bulk system in which the spin polarized current induces a macroscopic change in the magnetization.Comment: 3 pages, 4 figure

Control of the colossal magnetoresistance by strain effect in Nd0.5_{0.5}Ca0.5_{0.5}MnO3_{3} thin films

Thin films of Nd$_{0.5}$Ca$_{0.5}$MnO$_{3}$ manganites with colossal magnetoresistance (CMR) properties have been synthesized by the Pulsed Laser Deposition technique on (100)-SrTiO$_{3}$. The lattice parameters of these manganites and correlatively their CMR properties can be controlled by the substrate temperature $T_{S}$. The maximum CMR effect at 75K, calculated as the ratio $\rho (H=0T)/\rho (H=7T)$ is 10$^4$ for a deposition temperature of $T_{S}=680$ degC. Structural studies show that the Nd$_{0.5}$Ca$_{0.5}$MnO$_{3}$ film is single phase, [010]-oriented and has a pseudocubic symmetry of the perovskite subcell with a=3.77$\AA$ at room temperature. We suggest that correlation between lattice parameters, CMR and substrate temperature $T_{S}$ result mainly from substrate-induced strains which can weaken the charge-ordered state at low temperature.Comment: 9 pages, 4 figures. To be published in Applied Physics Letter

Microphase separation in Pr0.67Ca0.33MnO3 by small angle neutron scattering

We have evidenced by small angle neutron scattering at low temperature the coexistence of ferromagnetism (F) and antiferromagnetism (AF) in Pr0.67Ca0.33MnO3. The results are compared to those obtained in Pr0.80Ca0.20MnO3 and Pr0.63Ca0.37MnO3, which are F and AF respectively. Quantitative analysis shows that the small angle scattering is not due to a mesoscopic mixing but to a nanoscopic electronic and magnetic ''red cabbage'' structure, in which the ferromagnetic phase exists in form of thin layers in the AF matrix (stripes or 2D ''sheets'').Comment: 4 figure

Enhanced electrical and magnetic properties in La0.7Sr0.3MnO3 thin films deposited on CaTiO3-buffered silicon substrates

We investigate the suitability of an epitaxial CaTiO3 buffer layer deposited onto (100) Si by reactive molecular-beam epitaxy (MBE) for the epitaxial integration of the colossal magnetoresistive material La0.7Sr0.3MnO3 with silicon. The magnetic and electrical properties of La0.7Sr0.3MnO3 films deposited by MBE on CaTiO3-buffered silicon (CaTiO3/Si) are compared with those deposited on SrTiO3-buffered silicon (SrTiO3/Si). In addition to possessing a higher Curie temperature and a higher metal-to-insulator transition temperature, the electrical resistivity and 1/f noise level at 300 K are reduced by a factor of two in the heterostructure with the CaTiO3 buffer layer. These results are relevant to device applications of La0.7Sr0.3MnO3 thin films on silicon substrates

Non-linear electrical response in a charge/orbital ordered Pr⁡0.63\Pr_{0.63}Ca0.37_{0.37}MnO3_3 crystal : the charge density wave analogy

Non-linear conduction in a charge-ordered manganese oxide Pr$_{0.63}$Ca$_{0.37}$MnO$_3$ is reported. To interpret such a feature, it is usually proposed that a breakdown of the charge or orbitally ordered state is induced by the current. The system behaves in such a way that the bias current may generate metallic paths giving rise to resistivity drop. One can describe this feature by considering the coexistence of localized and delocalized electron states with independent paths of conduction. This situation is reminiscent of what occurs in charge density wave systems where a similar non-linear conduction is also observed. In the light of recent experimental results suggesting the development of charge density waves in charge and orbitally ordered manganese oxides, a phenomenological model for charge density waves motion is used to describe the non-linear conduction in Pr$_{0.63}$Ca$_{0.37}$MnO$_3$. In such a framework, the non-linear conduction arises from the motion of the charge density waves condensate which carries a net electrical current.Comment: 13 pages, 6 figure

Non-linear electrical response in a non-charge-ordered manganite: Pr0.8Ca0.2MnO3

Up to now, electric field induced non-linear conduction in the Pr(1-x)CaxMnO3 system has been ascribed to a current-induced destabilization of the charge ordered phase. However, for x<0.25, a ferromagnetic insulator state is observed and charge-ordering is absent whatever the temperature. A systematic investigation of the non-linear transport in the ferromagnetic insulator Pr0.8Ca0.2MnO3 shows rather similar results to those obtained in charge ordered systems. However, the experimental features observed in Pr0.8Ca0.2MnO3 are distinct in that the collapse of the CO energy gap can not be invoked as usually done in the other members of the PCMO system. We propose interpretations in which the effectiveness of the DE is restored upon application of electric field.Comment: 6 pages, 5 figure

Anomaly in the dielectric response at the charge orbital ordering transition of crystalline Pr0.67Ca0.33MnO3

The complex impedance of a Pr0.67Ca0.33MnO3 crystal has been measured. The frequency dependence is studied for a wide range of temperatures (50K-403K) and is found to be characteristic of relaxation process with a single Debye time relaxation constant, which is interpreted as a dielectric constant of the material. A strong peak is observed in this dielectric constant (up to two millions) at the charge ordering transition suggesting an interpretation in terms of ordering of electric dipoles at TCO or in term of phase separation. Comparison with Pr0.63Ca0.37MnO3 - in which the phase separation is much smaller and the peak in the dielectric constant is absent - suggests an interpretation in term of phase separation between insulating and metallic states.Comment: pdf fil

Colossal dielectric constants in transition-metal oxides

Many transition-metal oxides show very large ("colossal") magnitudes of the dielectric constant and thus have immense potential for applications in modern microelectronics and for the development of new capacitance-based energy-storage devices. In the present work, we thoroughly discuss the mechanisms that can lead to colossal values of the dielectric constant, especially emphasising effects generated by external and internal interfaces, including electronic phase separation. In addition, we provide a detailed overview and discussion of the dielectric properties of CaCu3Ti4O12 and related systems, which is today's most investigated material with colossal dielectric constant. Also a variety of further transition-metal oxides with large dielectric constants are treated in detail, among them the system La2-xSrxNiO4 where electronic phase separation may play a role in the generation of a colossal dielectric constant.Comment: 31 pages, 18 figures, submitted to Eur. Phys. J. for publication in the Special Topics volume "Cooperative Phenomena in Solids: Metal-Insulator Transitions and Ordering of Microscopic Degrees of Freedom