Two-color-laser-driven direct electron acceleration in infinite vacuum

We propose a direct electron acceleration scheme that uses a two-color pulsed radially polarized laser beam. The two-color scheme achieves electron acceleration exceeding 90% of the theoretical energy gain limit, over twice of what is possible with a one-color pulsed beam of equal total energy and pulse duration. The scheme succeeds by exploiting the Gouy phase shift to cause an acceleration-favoring interference of fields only as the electron enters its effectively final accelerating cycle. Optimization conditions and power scaling characteristics are discussed.National Science Foundation (U.S.) (NSF grant NSF-018899-001)Singapore. Agency for Science, Technology and Researc

On the theory of quantum measurement

Many so called paradoxes of quantum mechanics are clarified when the measurement equipment is treated as a quantized system. Every measurement involves nonlinear processes. Self consistent formulations of nonlinear quantum optics are relatively simple. Hence optical measurements, such as the quantum nondemolition (QND) measurement of photon number, are particularly well suited for such a treatment. It shows that the so called 'collapse of the wave function' is not needed for the interpretation of the measurement process. Coherence of the density matrix of the signal is progressively reduced with increasing accuracy of the photon number determination. If the QND measurement is incorporated into the double slit experiment, the contrast ratio of the fringes is found to decrease with increasing information on the photon number in one of the two paths

Impact of the Electronic Band Structure in High-Harmonic Generation Spectra of Solids

An accurate analytic model describing the microscopic mechanism of high-harmonic generation (HHG) in solids is derived. Extensive first-principles simulations within a time-dependent density-functional framework corroborate the conclusions of the model. Our results reveal that (i) the emitted HHG spectra are highly anisotropic and laser-polarization dependent even for cubic crystals; (ii) the harmonic emission is enhanced by the inhomogeneity of the electron-nuclei potential; the yield is increased for heavier atoms; and (iii) the cutoff photon energy is driver-wavelength independent. Moreover, we show that it is possible to predict the laser polarization for optimal HHG in bulk crystals solely from the knowledge of their electronic band structure. Our results pave the way to better control and optimize HHG in solids by engineering their band structure.European Research Council (Grant ERC-2015-AdG-694097)European Cooperation in the Field of Scientific and Technical Research (Organization) (Action Grant MP1306)German Science Foundation. Hamburg Centre for Ultrafast Imaging-Structure, Dynamics and Control of Matter at the Atromic ScaleGerman Science Foundation (Grant SPP1840 SOLSTICE

Cascaded Parametric Amplification for Highly Efficient Terahertz Generation

A highly efficient, practical approach to high-energy terahertz (THz) generation based on spectrally cascaded optical parametric amplification (THz-COPA) is introduced. The THz wave initially generated by difference frequency generation between a strong narrowband optical pump and optical seed (0.1-10% of pump energy) kick-starts a repeated or cascaded energy down-conversion of pump photons. This helps to greatly surpass the quantum-defect efficiency and results in exponential growth of THz energy over crystal length. In cryogenically cooled periodically poled lithium niobate, energy conversion efficiencies >8% for 100 ps pulses are predicted. The calculations account for cascading effects, absorption, dispersion and laser-induced damage. Due to the coupled nonlinear interaction of multiple triplets of waves, THz-COPA exhibits physics distinct from conventional three-wave mixing parametric amplifiers. This in turn governs optimal phase-matching conditions, evolution of optical spectra as well as limitations of the nonlinear process.Comment: 5 pages, double colum

Direct carrier–envelope phase stabilization of a soliton-effect compressed sub-two-cycle pulse source through nonlinear mixing of solitonic and dispersive waves

We present a carrier–envelope phase (CEP) stabilized sub-two-cycle 5.2 fs pulse source based on soliton-effect self-compression of femtosecond laser pulses in millimetre-long highly nonlinear photonic crystal fibres. We employ a simple and efficient scheme to generate a strong (40–60 dB, configuration dependent) CEP beat signal directly from the pulse source via f-to-2f interferometry where the second harmonic of the main soliton pulse is mixed with the isolated dispersive blue/green radiation peak that is also generated in the compression process, obviating the need for additional spectral broadening mechanisms.Fundação para a Ciência e a Tecnologia (Portugal)Fonds Europeen de Developpement Economique et Regional (Grant PTDC/FIS/115102/2009

AXSIS: Exploring the frontiers in attosecond X-ray science, imaging and spectroscopy

X-ray crystallography is one of the main methods to determine atomic-resolution 3D images of the whole spectrum of molecules ranging from small inorganic clusters to large protein complexes consisting of hundred-thousands of atoms that constitute the macromolecular machinery of life. Life is not static, and unravelling the structure and dynamics of the most important reactions in chemistry and biology is essential to uncover their mechanism. Many of these reactions, including photosynthesis which drives our biosphere, are light induced and occur on ultrafast timescales. These have been studied with high time resolution primarily by optical spectroscopy, enabled by ultrafast laser technology, but they reduce the vast complexity of the process to a few reaction coordinates. In the AXSIS project at CFEL in Hamburg, funded by the European Research Council, we develop the new method of attosecond serial X-ray crystallography and spectroscopy, to give a full description of ultrafast processes atomically resolved in real space and on the electronic energy landscape, from co-measurement of X-ray and optical spectra, and X-ray diffraction. This technique will revolutionize our understanding of structure and function at the atomic and molecular level and thereby unravel fundamental processes in chemistry and biology like energy conversion processes. For that purpose, we develop a compact, fully coherent, THz-driven attosecond X-ray source based on coherent inverse Compton scattering off a free-electron crystal, to outrun radiation damage effects due to the necessary high X-ray irradiance required to acquire diffraction signals. This highly synergistic project starts from a completely clean slate rather than conforming to the specifications of a large free-electron laser (FEL) user facility, to optimize the entire instrumentation towards fundamental measurements of the mechanism of light absorption and excitation energy transfer. A multidisciplinary team formed by laser-, accelerator,- X-ray scientists as well as spectroscopists and biochemists optimizes X-ray pulse parameters, in tandem with sample delivery, crystal size, and advanced X-ray detectors. Ultimately, the new capability, attosecond serial X-ray crystallography and spectroscopy, will be applied to one of the most important problems in structural biology, which is to elucidate the dynamics of light reactions, electron transfer and protein structure in photosynthesis.United States. Air Force. Office of Scientific Research (Contract FA9550-12-1-0499)American Society for Engineering Education. National Defense Science and Engineering Graduate Fellowshi

High-density Au nanorod optical field-emitter arrays

We demonstrate the design, fabrication, characterization, and operation of high-density arrays of Au nanorod electron emitters, fabricated by high-resolution electron beam lithography, and excited by ultrafast femtosecond near-infrared radiation. Electron emission characteristic of multiphoton absorption has been observed at low laser fluence, as indicated by the power-law scaling of emission current with applied optical power. The onset of space-charge-limited current and strong optical field emission has been investigated so as to determine the mechanism of electron emission at high incident laser fluence. Laser-induced structural damage has been observed at applied optical fields above 5 GV m[superscript −1], and energy spectra of emitted electrons have been measured using an electron time-of-flight spectrometer.United States. Defense Advanced Research Projects Agency (Contract N66001-11-1-4192)Gordon and Betty Moore Foundatio

Multi-mJ, kHz, 2.1-μm OPCPA for high-flux soft X-ray high-harmonic radiation

We report on a multi-mJ 2.1-μm OPCPA system operating at a 1-kHz repetition rate, pumped by a picosecond cryogenic Yb:YAG pump laser, and the phase-matched high-flux high-harmonic soft X-ray generation