176 research outputs found
Controlling shot noise in double-barrier magnetic tunnel junctions
We demonstrate that shot noise in Fe/MgO/Fe/MgO/Fe double-barrier magnetic
tunnel junctions is determined by the relative magnetic configuration of the
junction and also by the asymmetry of the barriers. The proposed theoretical
model, based on sequential tunneling through the system and including spin
relaxation, successfully accounts for the experimental observations for bias
voltages below 0.5V, where the influence of quantum well states is negligible.
A weak enhancement of conductance and shot noise, observed at some voltages
(especially above 0.5V), indicates the formation of quantum well states in the
middle magnetic layer. The observed results open up new perspectives for a
reliable magnetic control of the most fundamental noise in spintronic
structures.Comment: 8 pages, 4 figure
Anomalous Spin and Charge Dynamics of the 2D t-J Model at low doping
We present an exact diagonalization study of the dynamical spin and density
correlation function of the 2D t-J model for hole doping < 25%. Both
correlation functions show a remarkably regular, but completely different
scaling behaviour with both hole concentration and parameter values: the
density correlation function is consistent with that of bosons corresponding to
the doped holes and condensed into the lowest state of the noninteracting band
of width 8t, the spin correlation function is consistent with Fermions in a
band of width J. We show that the spin bag picture gives a natural explanation
for this unusual behaviour.Comment: Revtex-file, 4 PRB pages + 5 figures attached as uu-encoded ps-files
Hardcopies of figures (or the entire manuscript) can also be obtained by
e-mailing to: [email protected]
Interaction of a Magnetic Impurity with Strongly Correlated Conduction Electrons
We consider a magnetic impurity which interacts by hybridization with a
system of strongly correlated conduction electrons. The latter are described by
a Hubbard Hamiltonian. By means of a canconical transformation the charge
degrees of freedom of the magnetic impurity are eliminated. The resulting
effective Hamiltonian is investigated and various limiting cases
are considered. If the Hubbard interaction between the conduction electrons
is neglected reduces to a form obtained by the Schrieffer-Wolff
transformation, which is essentially the Kondo Hamiltonian. If is large and
the correlations are strong is changed. One modification concerns
the coefficient of the dominant exchange coupling of the magnetic impurity with
the nearest lattice site. When the system is hole doped, there is also an
antiferromagnetic coupling to the nearest neighbors of that site involving
additionally a hole. Furthermore, it is found that the magnetic impurity
attracts a hole. In the case of electron doping, double occupancies are
repelled by the impurity. In contrast to the hole-doped case, we find no
magnetic coupling which additionally involves a doubly occupied site.Comment: 16 pages, Revtex 3.
Hole-Hole Contact Interaction in the t-J Model
Using an analytical variational approach we calculate the hole-hole contact
interaction on the N\'{e}el background. Solution of the Bethe-Salpeter equation
with this interaction gives bound states in - and p-waves with binding
energies close to those obtained by numerical methods. At the
bound state disappears. In conclusion we discuss the relation between short
range and long range interactions and analogy with the problem of pion
condensation in nuclear matter.Comment: 11 pp. (LATEX), 7 figures (PostScript) appended, report N
Propagation of a hole on a Neel background
We analyze the motion of a single hole on a N\'eel background, neglecting
spin fluctuations. Brinkman and Rice studied this problem on a cubic lattice,
introducing the retraceable-path approximation for the hole Green's function,
exact in a one-dimensional lattice. Metzner et al. showed that the
approximationalso becomes exact in the infinite-dimensional limit. We introduce
a new approach to this problem by resumming the Nagaoka expansion of the
propagator in terms of non-retraceable skeleton-paths dressed by
retraceable-path insertions. This resummation opens the way to an almost
quantitative solution of the problemin all dimensions and, in particular sheds
new light on the question of the position of the band-edges. We studied the
motion of the hole on a double chain and a square lattice, for which deviations
from the retraceable-path approximation are expected to be most pronounced. The
density of states is mostly adequately accounted for by the
retra\-ce\-able-path approximation. Our band-edge determination points towards
an absence of band tails extending to the Nagaoka energy in the spectrums of
the double chain and the square lattice. We also evaluated the spectral density
and the self-energy, exhibiting k-dependence due to finite dimensionality. We
find good agreement with recent numerical results obtained by Sorella et al.
with the Lanczos spectra decoding method. The method we employ enables us to
identify the hole paths which are responsible for the various features present
in the density of states and the spectral density.Comment: 26 pages,Revte
Hole dynamics in generalized spin backgrounds in infinite dimensions
We calculate the dynamical behaviour of a hole in various spin backgrounds in
infinite dimensions, where it can be determined exactly. We consider hypercubic
lattices with two different types of spin backgrounds. On one hand we study an
ensemble of spin configurations with an arbitrary spin probability on each
sublattice. This model corresponds to a thermal average over all spin
configurations in the presence of staggered or uniform magnetic fields. On the
other hand we consider a definite spin state characterized by the angle between
the spins on different sublattices, i.e a classical spin system in an external
magnetic field. When spin fluctuations are considered, this model describes the
physics of unpaired particles in strong coupling superconductors.Comment: Accepted in Phys. Rev. B. 18 pages of text (1 fig. included) in Latex
+ 2 figures in uuencoded form containing the 2 postscripts (mailed
separately
Spatial Structure of Spin Polarons in the t-J Model
The deformation of the quantum Neel state induced by a spin polaron is
analyzed in a slave fermion approach. Our method is based on the selfconsistent
Born approximation for Green's and the wave function for the quasiparticle. The
results of various spin-correlation functions relative to the position of the
moving hole are discussed and shown to agree with those available from small
cluster calculations. Antiferromagnetic correlations in the direct neighborhood
of the hole are reduced, but they remain antiferromagnetic even for J as small
as 0.1 t. These correlation functions exhibit dipolar distortions in the spin
structure, which sensitively depend on the momentum of the quasiparticle. Their
asymptotic decay with the distance from the hole is governed by power laws, yet
the spectral weight of the quasiparticles does not vanish.Comment: 12 pages, 2 postscipt files with figures; uses REVTeX, to be
published in Phys. Rev. B, Feb. 199
Efficacy assessment of sustained intraperitoneal paclitaxel therapy in a murine model of ovarian cancer using bioluminescent imaging
We evaluated the pre-clinical efficacy of a novel intraperitoneal (i.p.) sustained-release paclitaxel formulation (PTXePC) using bioluminescent imaging (BLI) in the treatment of ovarian cancer. Human ovarian carcinoma cells stably expressing the firefly luciferase gene (SKOV3Luc) were injected i.p. into SCID mice. Tumour growth was evaluated during sustained or intermittent courses of i.p. treatment with paclitaxel (PTX). In vitro bioluminescence strongly correlated with cell survival and cytotoxicity. Bioluminescent imaging detected tumours before their macroscopic appearance and strongly correlated with tumour weight and survival. As compared with intermittent therapy with Taxol®, sustained PTXePC therapy resulted in significant reduction of tumour proliferation, weight and BLI signal intensity, enhanced apoptosis and increased survival times. Our results demonstrate that BLI is a useful tool in the pre-clinical evaluation of therapeutic interventions for ovarian cancer. Moreover, these results provide evidence of enhanced therapeutic efficacy with the sustained PTXePC implant system, which could potentially translate into successful clinical outcomes
Redox-controlled potassium intercalation into two polyaromatic hydrocarbon solids
Alkali metal intercalation into polyaromatic hydrocarbons (PAHs) has been studied intensely after reports of superconductivity in a number of potassium- and rubidium-intercalated materials. There are, however, no reported crystal structures to inform our understanding of the chemistry and physics because of the complex reactivity of PAHs with strong reducing agents at high temperature. Here we present the synthesis of crystalline K2Pentacene and K2Picene by a solid–solid insertion protocol that uses potassium hydride as a redox-controlled reducing agent to access the PAH dianions, and so enables the determination of their crystal structures. In both cases, the inserted cations expand the parent herringbone packings by reorienting the molecular anions to create multiple potassium sites within initially dense molecular layers, and thus interact with the PAH anion π systems. The synthetic and crystal chemistry of alkali metal intercalation into PAHs differs from that into fullerenes and graphite, in which the cation sites are pre-defined by the host structure
Formation of polycyclic aromatic hydrocarbon grains using anthracene and their stability under UV irradiation
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