Generation of optical Schrödinger cat states in intense laser-matter interactions

The physics of intense laser–matter interactions1,2 is described by treating the light pulses classically, anticipating no need to access optical measurements beyond the classical limit. However, the quantum nature of the electromagnetic fields is always present3. Here we demonstrate that intense laser–atom interactions may lead to the generation of highly non-classical light states. This was achieved by using the process of high-harmonic generation in atoms4,5, in which the photons of a driving laser pulse of infrared frequency are upconverted into photons of higher frequencies in the extreme ultraviolet spectral range. The quantum state of the fundamental mode after the interaction, when conditioned on the high-harmonic generation, is a so-called Schrödinger cat state, which corresponds to a superposition of two distinct coherent states: the initial state of the laser and the coherent state reduced in amplitude that results from the interaction with atoms. The results open the path for investigations towards the control of the non-classical states, exploiting conditioning approaches on physical processes relevant to high-harmonic generation.Peer ReviewedPostprint (author's final draft

Knotting fractional-order knots with the polarization state of light

The fundamental polarization singularities of monochromatic light are normally associated with invariance under coordinated rotations: symmetry operations that rotate the spatial dependence of an electromagnetic field by an angle $\theta$ and its polarization by a multiple $\gamma\theta$ of that angle. These symmetries are generated by mixed angular momenta of the form $J_\gamma = L + \gamma S$ and they generally induce M\"obius-strip topologies, with the coordination parameter $\gamma$ restricted to integer and half-integer values. In this work we construct beams of light that are invariant under coordinated rotations for arbitrary $\gamma$, by exploiting the higher internal symmetry of 'bicircular' superpositions of counter-rotating circularly polarized beams at different frequencies. We show that these beams have the topology of a torus knot, which reflects the subgroup generated by the torus-knot angular momentum $J_\gamma$, and we characterize the resulting optical polarization singularity using third-and higher-order field moment tensors, which we experimentally observe using nonlinear polarization tomography.Comment: Submitted Manuscript, including a subset of the figures from the published Supplementary Informatio

Quantum optical analysis of high-order harmonic generation in H2+_2^+ molecular ions

We present a comprehensive theoretical investigation of high-order harmonic generation in H$_2^+$ molecular ions within a quantum optical framework. Our study focuses on characterizing various quantum optical and quantum information measures, highlighting the versatility of HHG in two-center molecules towards quantum technology applications. We demonstrate the emergence of entanglement between electron and light states after the laser-matter interaction. We also identify the possibility of obtaining non-classical states of light in targeted frequency modes by conditioning on specific electronic quantum states, which turn out to be crucial in the generation of highly non-classical entangled states between distinct sets of harmonic modes. Our findings open up avenues for studying strong-laser field-driven interactions in molecular systems, and suggest their applicability to quantum technology applications.Comment: 21 pages (14 main text + 7 appendix), 9 figures (8 main text + 1 appendix

Light with a self-torque: extreme-ultraviolet beams with time-varying orbital angular momentum

Twisted light fields carrying orbital angular momentum (OAM) provide powerful capabilities for applications in optical communications, microscopy, quantum optics and microparticle rotation. Here we introduce and experimentally validate a new class of light beams, whose unique property is associated with a temporal OAM variation along a pulse: the self-torque of light. Self-torque is a phenomenon that can arise from matter-field interactions in electrodynamics and general relativity, but to date, there has been no optical analog. In particular, the self-torque of light is an inherent property, which is distinguished from the mechanical torque exerted by OAM beams when interacting with physical systems. We demonstrate that self-torqued beams in the extreme-ultraviolet (EUV) naturally arise as a necessary consequence of angular momentum conservation in non-perturbative high-order harmonic generation when driven by time-delayed pulses with different OAM. In addition, the time-dependent OAM naturally induces an azimuthal frequency chirp, which provides a signature for monitoring the self-torque of high-harmonic EUV beams. Such self-torqued EUV beams can serve as unique tools for imaging magnetic and topological excitations, for launching selective excitation of quantum matter, and for manipulating molecules and nanostructures on unprecedented time and length scales.Comment: 24 pages, 4 figure

Symphony on strong field approximation

This paper has been prepared by the Symphony collaboration (University of Warsaw, Uniwersytet Jagiellonski, DESY/CNR and ICFO) on the occasion of the 25th anniversary of the 'simple man's models' which underlie most of the phenomena that occur when intense ultrashort laser pulses interact with matter. The phenomena in question include high-harmonic generation (HHG), above-threshold ionization (ATI), and non-sequential multielectron ionization (NSMI). 'Simple man's models' provide both an intuitive basis for understanding the numerical solutions of the time-dependent Schrodinger equation and the motivation for the powerful analytic approximations generally known as the strong field approximation (SFA). In this paper we first review the SFA in the form developed by us in the last 25 years. In this approach the SFA is a method to solve the TDSE, in which the non-perturbative interactions are described by including continuum-continuum interactions in a systematic perturbation-like theory. In this review we focus on recent applications of the SFA to HHG, ATI and NSMI from multi-electron atoms and from multi-atom molecules. The main novel part of the presented theory concerns generalizations of the SFA to: (i) time-dependent treatment of two-electron atoms, allowing for studies of an interplay between electron impact ionization and resonant excitation with subsequent ionization; (ii) time-dependent treatment in the single active electron approximation of 'large' molecules and targets which are themselves undergoing dynamics during the HHG or ATI processes. In particular, we formulate the general expressions for the case of arbitrary molecules, combining input from quantum chemistry and quantum dynamics. We formulate also theory of time-dependent separable molecular potentials to model analytically the dynamics of realistic electronic wave packets for molecules in strong laser fields. We dedicate this work to the memory of Bertrand Carre, who passed away in March 2018 at the age of 60

Opportunities and challenges of the digital lifespan:views of service providers and citizens in the UK

<p>Information about UK citizens’ use of digital technologies is often expressed in statistics – x% lack Internet access; y% get online to engage in online banking, update social media sites, or participate in online auctions. There are many social implications to digital technology use, however – individuals may communicate online as a major way to stay in touch with friends and family, and as Internet access rises and government and public sector budgets shrink, online services become an increasingly attractive way for government and public sector service providers to communicate with citizens. This paper presents selected results of an exploratory study designed to investigate the digital personhood of UK citizens through interviews with participants at three life transitions: leaving secondary school, becoming a parent, and retiring from work. Digital personhood in this paper implies identity information online, and some interaction with others around that information. We then report on our presentation of a selection of these results to thirteen stakeholders who represented UK government departments, public sector organisations, and industry. We found that citizen and stakeholder concerns were quite different, especially at the new parent life transition, and that stakeholders tended to <i>underestimate</i> the willingness and ability of citizens to become involved online with the government and public sector, and <i>overestimate</i> citizens’ vulnerability online. Future research should investigate practical strategies for increasing communication between stakeholders and citizens, and also how to encourage stakeholders to work together to benefit their common clientele – the citizens.</p

Ochreriades fasciatus.

18 pages : illustrations (some color) ; 26 cm.Herein we present information on the nesting behavior of Ochreriades fasciatus (Friese) found occupying beetle galleries in dead trunks and branches of certain trees and shrubs in Israel. We also describe the pre- and postdefecating larvae thereby making known the mature larva for this uncommon Old World genus. Females of O. fasciatus build linear nests in existing burrows in dead wood; depending on the length of the burrow, 1-5 cells are placed in one nest. The cell partitions are made of hardened mud, while the nest plug consists of pebbles fixed together with mud. Ochreriades fasciatus is oligolectic on Lamiaceae and probably strongly associated with the two related genera Ballota and Moluccella. It is hoped that information concerning its nesting biology, host-plant relationships, as well as larval development and anatomy will eventually prove valuable in determining the phylogenetic position of this genus relative to other megachiline bees

Magnetic properties of X-Pt (X=Fe,Co,Ni) alloy systems

We have studied the electronic and magnetic properties of Fe-Pt, Co-Pt and Ni-Pt alloy systems in ordered and disordered phases. The influence of various exchange-correlation functionals on values of equilibrium lattice parameters and magnetic moments in ordered Fe-Pt, Co-Pt and Ni-Pt alloys have been studied using linearized muffin-tin orbital method. The electronic structure calculations for the disordered alloys have been carried out using augmented space recursion technique in the framework of tight binding linearized muffin-tin orbital method. The effect of short range order has also been studied in the disordered phase of these systems. The results show good agreements with available experimental values.Comment: 21 pages, 4 eps figures, accepted for publication in Journal of Physics Condensed Matte