Mesoscopic model for the fluctuating hydrodynamics of binary and ternary mixtures

A recently introduced particle-based model for fluid dynamics with continuous velocities is generalized to model immiscible binary mixtures. Excluded volume interactions between the two components are modeled by stochastic multiparticle collisions which depend on the local velocities and densities. Momentum and energy are conserved locally, and entropically driven phase separation occurs for high collision rates. An explicit expression for the equation of state is derived, and the concentration dependence of the bulk free energy is shown to be the same as that of the Widom-Rowlinson model. Analytic results for the phase diagram are in excellent agreement with simulation data. Results for the line tension obtained from the analysis of the capillary wave spectrum of a droplet agree with measurements based on the Laplace's equation. The introduction of "amphiphilic" dimers makes it possible to model the phase behavior and dynamics of ternary surfactant mixtures.Comment: 7 pages including 6 figure

Thermodynamics of the one-dimensional frustrated Heisenberg ferromagnet with arbitrary spin

The thermodynamic quantities (spin-spin correlation functions <{\bf S}_0{\bf S}_n>, correlation length {\xi}, spin susceptibility {\chi}, and specific heat C_V) of the frustrated one-dimensional J1-J2 Heisenberg ferromagnet with arbitrary spin quantum number S below the quantum critical point, i.e. for J2< |J1|/4, are calculated using a rotation-invariant Green-function formalism and full diagonalization as well as a finite-temperature Lanczos technique for finite chains of up to N=18 sites. The low-temperature behavior of the susceptibility {\chi} and the correlation length {\xi} is well described by \chi = (2/3)S^4 (|J1|-4J2) T^{-2} + A S^{5/2} (|J1|-4J2)^{1/2} T^{-3/2} and \xi = S^2 (|J1|-4J2) T^{-1} + B S^{1/2} (|J1|-4J2)^{1/2} T^{-1/2} with A \approx 1.1 ... 1.2 and B \approx 0.84 ... 0.89. The vanishing of the factors in front of the temperature at J2=|J1|/4 indicates a change of the critical behavior of {\chi} and {\xi} at T \to 0. The specific heat may exhibit an additional frustration-induced low-temperature maximum when approaching the quantum critical point. This maximum appears for S=1/2 and S=1, but was not found for S>1.Comment: 8 pages, 7 figure

Green's function theory of quasi-two-dimensional spin-half Heisenberg ferromagnets: stacked square versus stacked kagom\'e lattice

We consider the thermodynamic properties of the quasi-two-dimensional spin-half Heisenberg ferromagnet on the stacked square and the stacked kagom\'e lattices by using the spin-rotation-invariant Green's function method. We calculate the critical temperature $T_C$, the uniform static susceptibility $\chi$, the correlation lengths $\xi_\nu$ and the magnetization $M$ and investigate the short-range order above $T_C$. We find that $T_C$ and $M$ at $T>0$ are smaller for the stacked kagom\'e lattice which we attribute to frustration effects becoming relevant at finite temperatures.Comment: shortened version as published in PR

Particle organization after viscous sedimentation in tilted containers

A series of sedimentation experiments and numerical simulations have been conducted to understand the factors that control the final angle of a static sediment layer formed by quasi-monodisperse particles settling in an inclined container. The set of experiments includes several combinations of fluid viscosity, container angle, and solids concentration. A comparison between the experiments and a set of twodimensional numerical simulations shows that the physical mechanism responsible for the energy dissipation in the system is the collision between the particles. The results provide new insights into the mechanism that sets the morphology of the sediment layer formed by the settling of quasi-monodisperse particles onto the bottom of an inclined container. Tracking the interface between the suspension solids and the clear fluid zone reveals that the final angle adopted by the sediment layer shows strong dependencies on the initial particle concentration and the container inclination, but not the fluid viscosity. It is concluded that (1) the hindrance function plays an important role on the sediment bed angle, (2) the relation between the friction effect and the slope may be explained as a quasi-linear function of the projected velocity along the container bottom, and (3) prior to the end of settling there is a significant interparticle interaction through the fluid affecting to the final bed organization.We can express the sediment bed slope as a function of two dimensionless numbers, a version of the inertial number and the particle concentration. The present experiments confirm some previous results on the role of the interstitial fluid on low Stokes number flows of particulate matter.The authors acknowledge the support of the National Commission for Scientific and Techno- logical Research of Chile, CONICYT, Grant N◦ 21110766, Fondecyt Projects N◦ 11110201 and N◦ 1130910, the Department of Civil Engineering, the Department of Mining Engineering and the Advanced Mining Technology Center of the University of Chile, as well the staff of the G.K. Batchelor Laboratory, Department of Applied Mathematics and Theoretical Physics, University of Cambridge.This is the author accepted manuscript. The final version is available from AIP at http://dx.doi.org/10.1063/1.4958722

Quasiperiodic Tip Splitting in Directional Solidification

We report experimental results on the tip splitting dynamics of seaweed growth in directional solidification of succinonitrile alloys with poly(ethylene oxide) or acetone as solutes. The seaweed or dense branching morphology was selected by solidifying grains which are oriented close to the {111} plane. Despite the random appearance of the growth, a quasiperiodic tip splitting morphology was observed in which the tip alternately splits to the left and to the right. The tip splitting frequency f was found to be related to the growth velocity V as a power law f V^{1.5}. This finding is consistent with the predictions of a tip splitting model that is also presented. Small anisotropies are shown to lead to different kinds of seaweed morphologies.Comment: 4 pages, 7 figures, submitted to Physical Review Letter

Absence of long-range order in a spin-half Heisenberg antiferromagnet on the stacked kagome lattice

We study the ground state of a spin-half Heisenberg antiferromagnet on the stacked kagome lattice by using a spin-rotation-invariant Green's-function method. Since the pure two-dimensional kagome antiferromagnet is most likely a magnetically disordered quantum spin liquid, we investigate the question whether the coupling of kagome layers in a stacked three-dimensional system may lead to a magnetically ordered ground state. We present spin-spin correlation functions and correlation lengths. For comparison we apply also linear spin wave theory. Our results provide strong evidence that the system remains short-range ordered independent of the sign and the strength of the interlayer coupling