Dark-state suppression and optimization of laser cooling and fluorescence in a trapped alkaline-earth-metal single ion

We study the formation and destabilization of dark states in a single trapped 88Sr+ ion caused by the cooling and repumping laser fields required for Doppler cooling and fluorescence detection of the ion. By numerically solving the time-dependent density matrix equations for the eight-level system consisting of the sublevels of the 5s 2S1/2, 5p 2P1/2, and 4d 2D3/2 states, we analyze the different types of dark states and how to prevent them in order to maximize the scattering rate, which is crucial for both the cooling and the detection of the ion. The influence of the laser linewidths and ion motion on the scattering rate and the dark resonances is studied. The calculations are then compared with experimental results obtained with an endcap ion trap system located at the National Research Council of Canada and found to be in good agreement. The results are applicable also to other alkaline earth ions and isotopes without hyperfine structure

Unpolarized, incoherent repumping light for prevention of dark states in a trapped and laser-cooled single ion

Many ion species commonly used for laser-cooled ion trapping studies have a low-lying metastable 2D3/2 state that can become populated due to spontaneous emission from the 2P1/2 excited state. This requires a repumper laser to maintain the ion in the Doppler cooling cycle. Typically the 2D3/2 state, or some of its hyperfine components if the ion has nuclear spin, has a higher multiplicity than the upper state of the repumping transition. This can lead to dark states, which have to be destabilized by an external magnetic field or by modulating the polarization of the repumper laser. We propose using unpolarized, incoherent amplified spontaneous emission (ASE) to drive the repumping transition. An ASE source offers several advantages compared to a laser. It prevents the buildup of dark states without external polarization modulation even in zero magnetic field, it can drive multiple hyperfine transitions simultaneously, and it requires no frequency stabilization. These features make it very compact and robust, which is essential for the development of practical, transportable optical ion clocks. We construct a theoretical model for the ASE radiation, including the possibility of the source being partially polarized. Using 88Sr+ as an example, the performance of the ASE source compared to a single-mode laser is analyzed by numerically solving the eight-level density matrix equations for the involved energy levels. Finally a reduced three-level system is derived, yielding a simple formula for the excited state population and scattering rate, which can be used to optimize the experimental parameters. The required ASE power spectral density can be obtained with current technology

Trapping atoms on a transparent permanent-magnet atom chip

We describe experiments on trapping of atoms in microscopic magneto-optical traps on an optically transparent permanent-magnet atom chip. The chip is made of magnetically hard ferrite-garnet material deposited on a dielectric substrate. The confining magnetic fields are produced by miniature magnetized patterns recorded in the film by magneto-optical techniques. We trap Rb atoms on these structures by applying three crossed pairs of counter-propagating laser beams in the conventional magneto-optical trapping (MOT) geometry. We demonstrate the flexibility of the concept in creation and in-situ modification of the trapping geometries through several experiments.Comment: Modifications: A) Reference I. Barb et al., Eur. Phys. JD, 35, 75 (2005) added. B)Sentence rewritten: We routinely capture more than 10^6 atoms in a micro-MOT on a magnetized pattern. C) The magnetic field strengths are now given in Teslas. D) The second sentence in the fourth paragraph has been rewritten in order to more clearly describe the geometry and purpose of the compensation coils.E) In the seventh paragraph we have rewritten the sentence about the creation of the external magnetic field for the magnetic-domain patterning. F) In the ninth paragraph, we clarify the way to shift the trap center. G) Caption of Fig. 4 changed. H) We have modified paragraph 12 to improve the description on the guiding of the trap center along a toroidal pattern. I) The last two sentences of the manuscript have been rewritte

151Eu Mössbauer spectroscopy and x-ray-diffraction studies on the Pb2Ba2EuCu3O8+[delta] system

Simultaneous replacement of Sr by Ba and Y by Eu in the Pb-2213 system was found to yield single-phase Pb2Ba2EuCu3O8+δ samples, suitable for Eu151 Mössbauer measurements. The samples were synthesized by a solid-state reaction of metal oxides and carbonates under an inert atmosphere. An oxygen-rich sample corresponding to δ=1.79 was obtained by annealing the as-synthesized material (δ=0.16) in oxygen. The oxygen annealing increased the size of the lattice constants and led to an orthorhombic-to-tetragonal phase transition of the structure. The samples were also oriented in an 11.7-T magnetic field. The x-ray-diffraction spectra showed that the c axes tended to orient perpendicular to the applied field. The measured Mössbauer spectra exhibited an electric quadrupole interaction typical of the Eu site in high-Tc cuprates. The average orientation angles obtained from fittings of the Mössbauer spectra were in accordance with the results from the x-ray-diffraction measurements.Peer reviewe

Short pulse, diode pumped, passively Q-switched Nd:YAG laser at 946 nm quadrupled for UV production

We report on a compact UV-laser with a short pulse length of 1.9 ns at 236 nm. A passively Q-switched quasi-three-level Nd:YAG laser at 946 nm acts as the pump source. UV pulses are produced by two consecutive single-pass frequency doubling events, the first one from IR to blue with a BIBO crystal and the second one from blue to deep-UV with a beta-BBO crystal. Conversion efficiency from 946 nm to 473 nm is 28% and from blue to UV 7%. Average power for UV is 7.6 mW with a energy and peak power of 230 nJ, and 120 W respectively

Precise determination of the hyperfine parameters of europium in multifluorite perovskites by 151Eu Mössbauer spectroscopy

The hyperfine interactions at the europium lattice sites in samples of the homologous (Fe,Cu)Sr2(Eu,Ce)nCu2O4+2n+z (n=2,3) series were studied by Eu151 Mössbauer spectroscopy. The work was motivated by the search for new superconducting phases. This homologous series is based on the YBa2Cu3O7−δ (1:2:3) structure. The samples used in the Mössbauer measurements consisted of crystallites with random orientation and grain oriented crystallites. The texture of oriented samples was analyzed by x-ray diffraction. The complete quadrupole Hamiltonian of the 21.5-keV γ-transition of Eu151 was successfully applied in the analyses of all the Mössbauer spectra. In samples having n≤2 the europium atoms occupy a single lattice site, whereas the spectra of the n=3 samples exhibit hyperfine interactions of the two different europium sites. Analyzing the hyperfine parameters of the latter samples was made possible by simultaneous fitting of three spectra, corresponding to three different crystal orientations of the same specimen. This fitting scheme also enables more precise determination of the hyperfine parameters in the n=2 samples. In these samples an electric field gradient (EFG), with a large negative-valued main component (Vzz) parallel with the crystal c axis, was found. In the n=3 samples, the two EFG’s of the europium sites were found to have Vzz components of opposite signs. The negative Vzz value was attributed to the rare-earth site adjacent to the CuO layer. This site, found in all samples of the series, corresponds to the rare-earth site of the 1:2:3 system.Peer reviewe

Europium-based high-temperature superconductors studied by x-ray diffraction and 151Eu Mössbauer spectroscopy

Isotropic powders and magnetically aligned crystallites of EuBa2Cu3O7−δ (1:2:3) and europium-doped Bi2Sr2CaCu2O8 (2:2:1:2) were studied by means of x-ray diffraction and Eu151 Mössbauer spectroscopy. The degree of crystallite orientation of the samples and the values of the lattice constants were determined by x-ray diffraction. The Mössbauer spectra were analyzed considering the full hyperfine Hamiltonian of the nuclear states of the 21.5-keV γ transition. The Mössbauer hyperfine parameters obtained from the superconducting and semiconducting phases are presented. A small change is seen in the Eu151 isomer shift when the oxygen deficiency δ of the 1:2:3 compound is varied. The shift can be explained by a decrease in the s-electron density due to lattice expansion. The changes in the oxidation state of the copper atoms with varying δ were determined from the Mössbauer data: The Cu(2) atoms retain their oxidation state, whereas the Cu(1) atoms adjust their valence according to the value of δ. In the 2:2:1:2 samples, the Eu concentration clearly affected the value of the electric-field gradient at the Eu nucleus. Using a standard procedure, magnetically aligned 2:2:1:2 samples were prepared. The preferred direction of the crystal c axis changed from parallel to perpendicular alignment with the external magnetic field, when the Eu concentration exceeded 20% of the Ca atoms.Peer reviewe

Europium substitution effects in superconducting YBa2Cu4O8 synthesized under one atmosphere oxygen pressure

Y1−xEuxBa2Cu4O8 powder samples, with x=0, 0.25, 0.5, 0.75, and 1.0, were synthesized at ambient pressure using either an acetate-tartrate sol-gel method or a LiF flux process. The lattice parameters and purity of the samples were checked using X-ray diffraction. The superconducting transition was monitored by magnetic-susceptibility measurements. Replacing yttrium with europium increased the unit-cell volume, decreased the orthorhombicity (b/a) and the critical temperature. The hyperfine interactions at the europium site were studied by Eu151 Mössbauer spectroscopy. The complete quadrupole Hamiltonian of the 21.5-keV γ transition of Eu151 was successfully applied in the analyses of the Mössbauer spectra. The Mössbauer parameters obtained were found to resemble those measured for the EuBa2Cu3Cu3O7−δ (1:2:3) system. It was demonstrated that magnetic alignment of the crystallites could not be obtained with an 11.7-T field, contrary to the 1:2:3 and other high-Tc systems. The magnetic susceptibility for 1:2:4 single crystals appears to be isotropic.Peer reviewe

Cooling of a mirror by radiation pressure

We describe an experiment in which a mirror is cooled by the radiation pressure of light. A high-finesse optical cavity with a mirror coated on a mechanical resonator is used as an optomechanical sensor of the Brownian motion of the mirror. A feedback mechanism controls this motion via the radiation pressure of a laser beam reflected on the mirror. We have observed either a cooling or a heating of the mirror, depending on the gain of the feedback loop.Comment: 4 pages, 6 figures, RevTe

Optomechanical scheme for the detection of weak impulsive forces

We show that a cooling scheme and an appropriate quantum nonstationary strategy can be used to improve the signal to noise ratio for the optomechanical detection of weak impulsive forces.Comment: 4 pages, Revtex, 1 figur