259 research outputs found

    Photo-excited charge carrier lifetime enhanced by slow cation molecular dynamics in lead iodide perovskite FAPbI3_3

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    Using muon spin relaxation (μ\muSR) measurements on formamidinium lead iodide [FAPbI3_3, where FA denotes HC(NH2)2_2)_2] we show that, among the five structurally distinct phases of FAPbI3_3 exhibited through two different temperature hysteresis, the reorientation motion of FA molecules is quasi-static below ≈50\approx50 K over the time scale of 10−6^{-6} s in the low-temperature (LT) hexagonal (Hex-LT, <160<160 K) phase which has relatively longer photo-excited charge carrier lifetime (τc∼\tau_{\rm c}\sim10−6^{-6} s). In contrast, a sharp increase in the FA molecular motion was found above ≈50\approx50 K in the Hex-LT phase, LT-tetragonal phase (Tet-LT, <140<140 K), the high-temperature (HT) hexagonal phase (Hex-HT, 160-380 K), and the HT-tetragonal phase (Tet-HT, 140-280 K) where τc\tau_{\rm c} decreases with increasing temperature. More interestingly, the reorientation motion is further promoted in the cubic phase at higher temperatures (>380/280>380/280 K), while τc\tau_{\rm c} is recovered to comparable or larger than that of the LT phases. These results indicate that there are two factors that determine τc\tau_{\rm c}, one related to the local reorientation of cationic molecules that is not unencumbered by phonons, and the other to the high symmetry of the bulk crystal structure.Comment: 7 pages, 4 figure

    Microscopic Structure of High-Spin Vibrational Excitations in Superdeformed 190,192,194Hg

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    Microscopic RPA calculations based on the cranked shell model are performed to investigate the quadrupole and octupole correlations for excited superdeformed bands in 190Hg, 192Hg, and 194Hg. The K=2 octupole vibrations are predicted to be the lowest excitation modes at zero rotational frequency. At finite frequency, however, the interplay between rotation and vibrations produces different effects depending on neutron number: The lowest octupole phonon is rotationally aligned in 190Hg, is crossed by the aligned two-quasiparticle bands in 192Hg, and retains the K=2 octupole vibrational character up to the highest frequency in 194Hg. The gamma vibrations are predicted to be higher in energy and less collective than the octupole vibrations. From a comparison with the experimental dynamic moments of inertia, a new interpretation of the observed excited bands invoking the K=2 octupole vibrations is proposed, which suggests those octupole vibrations may be prevalent in SD Hg nuclei.Comment: 22 pages, REVTeX, 12 postscript figures are available on reques

    Time-odd components in the mean field of rotating superdeformed nuclei

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    Rotation-induced time-odd components in the nuclear mean field are analyzed using the Hartree-Fock cranking approach with effective interactions SIII, SkM*, and SkP. Identical dynamical moments J(2){{\cal J}^{(2)}} are obtained for pairs of superdeformed bands 151^{151}Tb(2)--152^{152}Dy(1) and 150^{150}Gd(2)--151^{151}Tb(1). The corresponding relative alignments strongly depend on which time-odd mean-field terms are taken into account in the Hartree-Fock equations.Comment: 23 pages, ReVTeX, 6 uuencoded postscript figures include

    Relative spins and excitation energies of superdeformed bands in 190Hg: Further evidence for octupole vibration

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    An experiment using the Eurogam Phase II gamma-ray spectrometer confirms the existence of an excited superdeformed (SD) band in 190Hg and its very unusual decay into the lowest SD band over 3-4 transitions. The energies and dipole character of the transitions linking the two SD bands have been firmly established. Comparisons with RPA calculations indicate that the excited SD band can be interpreted as an octupole-vibrational structure.Comment: 12 pages, latex, 4 figures available via WWW at http://www.phy.anl.gov/bgo/bc/hg190_nucl_ex.htm

    The Moderating Effect of Mental Toughness: Perception of Risk and Belief in the Paranormal

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    This research demonstrates that higher levels of mental toughness provide cognitive-perceptual processing advantages when evaluating risk. No previous research, however, has examined mental toughness in relation to perception of risk and paranormal belief (a variable associated with distorted perception of causality and elevated levels of perceived risk). Accordingly, the present paper investigated relationships between these factors. A sample of 174 participants completed self-report measures assessing mental toughness, general perception of risk, and paranormal belief. Responses were analyzed via correlations and moderation analyses. Results revealed that mental toughness correlated negatively with perception of risk and paranormal belief, whereas paranormal belief correlated positively with perception of risk. For the moderation effects, simple slopes analyses indicated that high levels of MT and subfactors of commitment and confidence reduced the strength of association between paranormal belief and perceived risk. Therefore, MT potentially acts as a protective factor among individuals who believe in the paranormal, reducing the tendency to perceive elevated levels of risk

    An examination of the factorial and convergent validity of four measures of conspiracist ideation, with recommendations for researchers

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    A number scales have been developed to measure conspiracist ideation, but little attention has been paid to the factorial validity of these scales. We reassessed the psychometric properties of four widely-used scales, namely the Belief in Conspiracy Theories Inventory (BCTI), the Conspiracy Mentality Questionnaire (CMQ), the Generic Conspiracist Beliefs Scale (GCBS), and the One-Item Conspiracy Measure (OICM). Eight-hundred-and-three U. S. adults completed all measures, along with measures of endorsement of 9/11 and anti- vaccination conspiracy theories. Through both exploratory and confirmatory factor analysis, we found that only the BCTI had acceptable factorial validity. We failed to confirm the factor structures of the CMQ and the GBCS, suggesting these measures had poor factorial valid- ity. Indices of convergent validity were acceptable for the BCTI, but weaker for the other measures. Based on these findings, we provide suggestions for the future refinement in the measurement of conspiracist ideation

    Understanding conspiracy theories

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    Scholarly efforts to understand conspiracy theories have grown significantly in recent years, and there is now a broad and interdisciplinary literature that we review in this article. We ask three specific questions. First, what are the factors that are associated with conspiracy theorizing? Our review of the literature shows that conspiracy beliefs result from a range of psychological, political and social factors. Next, how are conspiracy theories communicated? Here, we explain how conspiracy theories are shared among individuals and spread through traditional and social media platforms. Next, what are the risks and rewards associated with conspiracy theories? By focusing on politics and science, we argue that conspiracy theories do more harm than good. Finally, because this is a growing literature and many open questions remain, we conclude by suggesting several promising avenues for future research

    Female chromosome X mosaicism is age-related and preferentially affects the inactivated X chromosome

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