Thickness dependent Curie temperatures of ferromagnetic Heisenberg films

We develop a procedure for calculating the magnetic properties of a ferromagnetic Heisenberg film with single-ion anisotropy which is valid for arbitrary spin and film thickness. Applied to sc(100) and fcc(100) films with spin S=7/2 the theory yields the layer dependent magnetizations and Curie temperatures of films of various thicknesses making it possible to investigate magnetic properties of films at the interesting 2D-3D transition.Comment: 9 pages, 2 figures, accepted (Solid State Commun.

Nonlinear Dynamics of Nuclear-Electronic Spin Processes in Ferromagnets

Spin dynamics is considered in ferromagnets consisting of electron and nuclear subsystems interacting with each other through hyperfine forces. In addition, the ferromagnetic sample is coupled with a resonance electric circuit. Under these conditions, spin relaxation from a strongly nonequilibrium initial state displays several peculiarities absent for the standard set-up in studying spin relaxation. The main feature of the nonlinear spin dynamics considered in this communication is the appearance of ultrafast coherent relaxation, with characteristic relaxation times several orders shorter than the transverse relaxation time $T_2$. This type of coherent spin relaxation can be used for extracting additional information on the intrinsic properties of ferromagnetic materials and also can be employed for different technical applications.Comment: 1 file, 4 pages, RevTex, no figure

Magnonic Crystal with Two-Dimensional Periodicity as a Waveguide for Spin Waves

We describe a simple method of including dissipation in the spin wave band structure of a periodic ferromagnetic composite, by solving the Landau-Lifshitz equation for the magnetization with the Gilbert damping term. We use this approach to calculate the band structure of square and triangular arrays of Ni nanocylinders embedded in an Fe host. The results show that there are certain bands and special directions in the Brillouin zone where the spin wave lifetime is increased by more than an order of magnitude above its average value. Thus, it may be possible to generate spin waves in such composites decay especially slowly, and propagate especially large distances, for certain frequencies and directions in ${\bf k}$-space.Comment: 13 pages, 4 figures, submitted to Phys Rev

Manipulating nanoscale structure to control functionality in printed organic photovoltaic, transistor and bioelectronic devices.

Printed electronics is simultaneously one of the most intensely studied emerging research areas in science and technology and one of the fastest growing commercial markets in the world today. For the past decade the potential for organic electronic (OE) materials to revolutionize this printed electronics space has been widely promoted. Such conviction in the potential of these carbon-based semiconducting materials arises from their ability to be dissolved in solution, and thus the exciting possibility of simply printing a range of multifunctional devices onto flexible substrates at high speeds for very low cost using standard roll-to-roll printing techniques. However, the transition from promising laboratory innovations to large scale prototypes requires precise control of nanoscale material and device structure across large areas during printing fabrication. Maintaining this nanoscale material control during printing presents a significant new challenge that demands the coupling of OE materials and devices with clever nanoscience fabrication approaches that are adapted to the limited thermodynamic levers available. In this review we present an update on the strategies and capabilities that are required in order to manipulate the nanoscale structure of large area printed organic photovoltaic (OPV), transistor and bioelectronics devices in order to control their device functionality. This discussion covers a range of efforts to manipulate the electroactive ink materials and their nanostructured assembly into devices, and also device processing strategies to tune the nanoscale material properties and assembly routes through printing fabrication. The review finishes by highlighting progress in printed OE devices that provide a feedback loop between laboratory nanoscience innovations and their feasibility in adapting to large scale printing fabrication. The ability to control material properties on the nanoscale whilst simultaneously printing functional devices on the square metre scale is prompting innovative developments in the targeted nanoscience required for OPV, transistor and biofunctional devices

Anomalous frequency and intensity scaling of collective and local modes in a coupled spin tetrahedron system

We report on the magnetic excitation spectrum of the coupled spin tetrahedral system Cu$_{2}$Te$_{2}$O$_{5}$Cl$_{2}$ using Raman scattering on single crystals. The transition to an ordered state at T$_{N}^{Cl}$=18.2 K evidenced from thermodynamic data leads to the evolution of distinct low-energy magnetic excitations superimposed by a broad maximum. These modes are ascribed to magnons with different degree of localization and a two-magnon continuum. Two of the modes develop a substantial energy shift with decreasing temperature similar to the order parameter of other Neel ordered systems. The other two modes show only a negligible temperature dependence and dissolve above the ordering temperature in a continuum of excitations at finite energies. These observations point to a delicate interplay of magnetic inter- and intra-tetrahedra degrees of freedom and an importance of singlet fluctuations in describing a spin dynamics.Comment: 7pages, 6figures, 1tabl

Chandra and XMM Observations of the ADC Source 0921-630

We analyze observations of the low mass X-ray binary 2S0921-63 obtained with the gratings and CCDs on Chandra and XMM. This object is a high inclination system showing evidence for an accretion disk corona (ADC). Such a corona has the potential to constrain the properties of the heated accretion disk in this system, and other LMXBs by extension. We find evidence for line emission which is generally consistent with that found by previous experiments, although we are able to detect more lines. For the first time in this source, we find that the iron K line has multiple components. We set limits on the line widths and velocity offsets, and we fit the spectra to photoionization models and discuss the implications for accretion disk corona models. For the first time in any ADC source we use these fits, together with density constraints based on the O VII line ratio, in order to constrain the flux in the medium-ionization region of the ADC. Under various assumptions about the source luminosity this constrains the location of the emitting region. These estimates, together with estimates for the emission measure, favor a scenario in which the intrinsic luminosity of the source is comparable to what we observe.Comment: 40 pages, 11 figures submitted to Ap.

Implications of X-Ray Line Variations for 4U1822-371

4U 1822-371 is one of the proto-type accretion disk coronal sources with an orbital period of about 5.6 hours. The binary is viewed almost edge-on at a high inclination angle of 83 degrees, which makes it a unique candidate to study binary orbital and accretion disk dynamics in high powered X-ray sources. We observed the X-ray source in 4U 1822-371 with the Chandra High Energy Transmission Grating Spectrometer (HETGS) for almost nine binary orbits. X-ray eclipse times provide an update of the orbital ephemeris. We find that our result follows the quadratic function implied by previous observations; however, it suggests a flatter trend. Detailed line dynamics also confirm a previous suggestion that the observed photo-ionized line emission originates from a confined region in the outer edge of the accretion disk near the hot spot. Line properties allow us to impose limits on the size of accretion disk, the central corona, and the emission region. The photo-ionized plasma is consistent with ionization parameters of log(xi) > 2, and when combined with disk size and reasonable assumptions for the plasma density, this suggests illuminating disk luminosities which are over an order of magnitude higher than what is actually observed. That is, we do not directly observe the central emitting X-ray source. The spectral continua are best fit by a flat power law with a high energy cut-off and partial covering absorption (N_H ranging from 5.4-6.3x10^{22} cm^{-2}) with a covering fraction of about 50%. We discuss some implications of our findings with respect to the photo-ionized line emission for the basic properties of the X-ray source.Comment: Submitted to the Astrophysical Journa