Magnetic, thermodynamic, and electrical transport properties of the noncentrosymmetric B20 germanides MnGe and CoGe

We present magnetization, specific heat, resistivity, and Hall effect measurements on the cubic B20 phase of MnGe and CoGe and compare to measurements of isostructural FeGe and electronic structure calculations. In MnGe, we observe a transition to a magnetic state at $T_c=275$ K as identified by a sharp peak in the ac magnetic susceptibility, as well as second phase transition at lower temperature that becomes apparent only at finite magnetic field. We discover two phase transitions in the specific heat at temperatures much below the Curie temperature one of which we associate with changes to the magnetic structure. A magnetic field reduces the temperature of this transition which corresponds closely to the sharp peak observed in the ac susceptibility at fields above 5 kOe. The second of these transitions is not affected by the application of field and has no signature in the magnetic properties or our crystal structure parameters. Transport measurements indicate that MnGe is metal with a negative magnetoresistance similar to that seen in isostructural FeGe and MnSi. Hall effect measurements reveal a carrier concentration of about 0.5 carriers per formula unit also similar to that found in FeGe and MnSi. CoGe is shown to be a low carrier density metal with a very small, nearly temperature independent diamagnetic susceptibility.Comment: 16 pages 23 figure

Fermi surface evolution through a heavy fermion superconductor-to-antiferromagnet transition: de Haas-van Alphen effect in Cd-substituted CeCoIn5_5

We report the results of de-Haas-van-Alphen (dHvA) measurements in Cd doped CeCoIn$_5$ and LaCoIn$_5$. Cd doping is known to induce an antiferromagnetic order in the heavy fermion superconductor CeCoIn$_5$, whose effect can be reversed with applied pressure. We find a slight but systematic change of the dHvA frequencies with Cd doping in both compounds, reflecting the chemical potential shift due to the addition of holes. The frequencies and effective masses are close to those found in the nominally pure compounds with similar changes apparent in the Ce and La compounds with Cd substitution. We observe no abrupt changes to the Fermi surface in the high field paramagnetic state for $x \sim x_c$ corresponding to the onset of antiferromagnetic ordering at H=0 in CeCo(In$_{1-x}$Cd$_x$)$_5$. Our results rule out $f-$electron localization as the mechanism for the tuning of the ground state in CeCoIn$_5$ with Cd doping

Local structure and site occupancy of Cd and Hg substitutions in CeTIn5 (T=Co, Rh, Ir)

The CeTIn5 superconductors (T=Co, Rh, or Ir) have generated great interest due to their relatively Tc's, NFL behavior, and their proximity to AF order and quantum critical points. In contrast to small changes with the T-species, electron doping in CeT(In{1-x}Mx)5 with M=Sn and hole doping with Cd or Hg have a dramatic effect on the electronic properties at very low concentrations. The present work reports EXAFS measurements that address the substituent atom distribution as a function of T, M, and x, near the superconducting phase. Together with previous measurements for M=Sn, the proportion of the M atom residing on the In(1) site, f{In(1)}, increases in the order M=Cd, Sn, and Hg, ranging from about 40% to 70%, showing a strong preference for these substituents to occupy the In(1) site (random=20%). In addition, f{In(1)} ranges from 70% to 100% for M=Hg in the order T=Co, Rh, and Ir. These fractions track the changes in the atomic radii of the various species, and help explain the sharp dependence of Tc on substituting into the In site. However, it is difficult to reconcile the small concentrations of M with the dramatic changes in the ground state in the hole-doped materials with only an impurity scattering model. These results therefore indicate that while such substitutions have interesting local atomic structures with important electronic and magnetic consequences, other local changes in the electronic and magnetic structure are equally important in determining the bulk properties of these materials.Comment: 10 pages, 7 figures, to appear in PR

Superconducting fluctuations and the Nernst effect: A diagrammatic approach

We calculate the contribution of superconducting fluctuations above the critical temperature $T_c$ to the transverse thermoelectric response $\alpha_{xy}$, the quantity central to the analysis of the Nernst effect. The calculation is carried out within the microscopic picture of BCS, and to linear order in magnetic field. We find that as $T \to T_c$, the dominant contribution to $\alpha_{xy}$ arises from the Aslamazov-Larkin diagrams, and is equal to the result previously obtained from a stochastic time-dependent Ginzburg-Landau equation [Ussishkin, Sondhi, and Huse, arXiv:cond-mat/0204484]. We present an argument which establishes this correspondence for the heat current. Other microscopic contributions, which generalize the Maki-Thompson and density of states terms for the conductivity, are less divergent as $T \to T_c$.Comment: 11 pages, 5 figure

Observation of the Nernst signal generated by fluctuating Cooper pairs

Long-range order is destroyed in a superconductor warmed above its critical temperature (Tc). However, amplitude fluctuations of the superconducting order parameter survive and lead to a number of well established phenomena such as paraconductivity : an excess of charge conductivity due to the presence of short-lived Cooper pairs in the normal state. According to an untested theory, these pairs generate a transverse thermoelectric (Nernst) signal. In amorphous superconducting films, the lifetime of Cooper pairs exceeds the elastic lifetime of quasi-particles in a wide temperature range above Tc; consequently, the Cooper pairs Nernst signal dominate the response of the normal electrons well above Tc. In two dimensions, the magnitude of the expected signal depends only on universal constants and the superconducting coherence length, so the theory can be unambiguously tested. Here, we report on the observation of a Nernst signal in such a superconductor traced deep into the normal state. Since the amplitude of this signal is in excellent agreement with the theoretical prediction, the result provides the first unambiguous case for a Nernst effect produced by short-lived Cooper pairs

SC-to-AFM transition in CeCo(In1-xCdx)5: De Haas-van Alphen Measurements

The results of de-Haas-van-Alphen (dHvA) measurements on Cd doped CeCoIn5 in the high magnetic field paramagnetic phase are reported. The replacement of trivalent In by divalent Cd is known to induce an antiferromagnetic order coexisting with superconductivity in this heavy fermion superconductor. We find a small but systematic change in the dHvA frequencies with Cd doping, reflecting the chemical potential shift due to the removal of conduction electrons. The frequencies and effective masses are close to those found in the undoped compound. We observe no abrupt change in the electron Fermi surface (FS) volume in the high field paramagnetic phase for x \u3e x c corresponding to the onset of antiferromagnetic ordering at zero magnetic field in CeCo(In1xCdx)5. Our results show that no significant change of the Fermi surface volume occurs to cause the AFM onset inside the SC state in CeCoIn5 with Cd doping. Only slight changes causing the Band 15 electron FS to be more cylindrical are observed making nesting more likely. © Published under licence by IOP Publishing Ltd

Antiferromagnetic Phases in the Fulde-Ferrell-Larkin-Ovchinnikov State of CeCoIn_5

The antiferromagnetic (AFM) order in the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) superconducting state is analyzed on the basis of a Ginzburg-Landau theory. To examine the possible AFM-FFLO state in CeCoIn_5, we focus on the incommensurate AFM order characterized by the wave vector Q = Q_{0} \pm q_inc with Q_0 =(\pi,\pi,\pi) and q_inc \parallel [110] or [1-10] in the tetragonal crystal structure. We formulate the two component Ginzburg-Landau theory and investigate the two degenerate incommensurate AFM order. We show that the pinning of AFM moment due to the FFLO nodal planes leads to multiple phases in magnetic fields along [100] or [010]. The phase diagrams for various coupling constants between the two order parameters are shown for the comparison with CeCoIn_5. Experimental results of the NMR and neutron scattering measurements are discussed.Comment: 6pages, Proceedings of ICHE2010, To appear in J. Phys. Soc. Jpn. Supp

Anomalous dissipation in the mixed state of underdoped cuprates close to the superconductor-insulator boundary

We present a comparative study of Nernst effect and resistivity in underdoped samples of Bi$_2$Sr$_2$CuO$_{6+\delta}$ and La$_{2-x}$Sr$_{x}$CuO$_4$. The Nernst effect presents a peak in a region of the H-T diagram where resistivity shows a non-metallic temperature dependence. Our results illustrate that the mechanism of dissipation in the mixed state of underdoped cuprates is poorly understood. Large quantum superconducting fluctuations and vanishing vortex viscosity are among suggested explanations for an enhanced Nernst signal close to the superconductor-insulator boundary.Comment: 5 pages including 3 figure

Ginzburg-Landau Analysis for the Antiferromagnetic Order in the Fulde-Ferrell-Larkin-Ovchinnikov Superconductor

Incommensurate antiferromangetic (AFM) order in the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) superconductor is investigated on the basis of the Ginzburg-Landau theory. We formulate the two component Ginzburg-Landau model to discuss two degenerate incommensurate AFM states in the tetragonal crystal structure. Owing to the broken translation symmetry in the FFLO state, a multiple phase diagram of single-q phase and double-q phase is obtained under the magnetic field along [100] or [010] direction. Magnetic properties in each phase are investigated and compared with the neutron scattering and NMR measurements for a heavy fermion superconductor CeCoIn_5. An ultrasonic measurement is proposed for a future experimental study to identify the AFM-FFLO state. The field orientation dependence of the AFM order in CeCoIn_5 is discussed.Comment: 8 page