Ultrafast generation of nonthermal magnons in iron: Ab initio parameterized calculations

Ultrafast laser excitation of ferromagnetic metals gives rise to correlated, highly non-equilibrium dynamics of electrons, spins and lattice, which are, however, poorly described by the widely used three-temperature model (3TM). Here, we develop a fully ab initio parameterized out-of-equilibrium theory based on a quantum kinetic approach -- termed (N+2) temperature model -- that describes magnon occupation dynamics due to electron-magnon scattering. We apply this model to perform quantitative simulations on the ultrafast, laser-induced generation of magnons in iron and demonstrate that on these timescales the magnon distribution is non-thermal: predominantly high-energy magnons are created, while the magnon occupation close to the center of the Brillouin zone even decreases, due to a repopulation towards higher energy states via a so-far-overlooked scattering term. Moreover, we show that the 3TM can be derived from our model and compare it with our microscopic calculations. In doing so, we demonstrate that the simple relation between magnetization and temperature computed at equilibrium does not hold in the ultrafast regime and that the 3TM greatly overestimates the demagnetization. Our ab initio-parametrized calculations show that ultrafast generation of non-thermal magnons provides a sizable demagnetization within 200 fs and, thus, emphasize the importance of magnon excitations for the ultrafast demagnetization process

Néel vector switching and terahertz spin-wave excitation in Mn2Au due to femtosecond spin-transfer torques

Efficient and fast manipulation of antiferromagnets has to date remained a challenging task, hindering their application in spintronic devices. For ultrafast operation of such devices, it is highly desirable to be able to control the antiferromagnetic order within picoseconds—a timescale that is difficult to achieve with electrical circuits. Here, we demonstrate that bursts of spin-polarized hot-electron currents emerging due to laser-induced ultrafast demagnetization are able to efficiently excite spin dynamics in antiferromagnetic Mn2Au by exerting a spin-transfer torque on femtosecond timescales. We combine quantitative superdiffusive transport and atomistic spin-model calculations to describe a spin-valve-type trilayer consisting of Fe|Cu|Mn2Au. Our results demonstrate that femtosecond spin-transfer torques can switch the Mn2Au layer within a few picoseconds. In addition, we find that spin waves with high frequencies up to several THz can be excited in Mn2Au

N\'eel-Vector Switching and THz Spin-Wave Excitation in Mn2_2Au due to Femtosecond Spin-Transfer Torques

Efficient and fast manipulation of antiferromagnets has to date remained a challenging task, hindering their application in spintronic devices. For ultrafast operation of such devices, it is highly desirable to be able to control the antiferromagnetic order within picoseconds - a timescale that is difficult to achieve with electrical circuits. Here, we demonstrate that bursts of spin-polarized hot-electron currents emerging due to laser-induced ultrafast demagnetization are able to efficiently excite spin dynamics in antiferromagnetic Mn$_2$Au by exerting a spin-transfer torque on femtosecond timescales. We combine quantitative superdiffusive transport and atomistic spin-model calculations to describe a spin-valve-type trilayer consisting of Fe$|$Cu$|$Mn$_2$Au. Our results demonstrate that femtosecond spin-transfer torques can switch the Mn$_2$Au layer within a few picoseconds. In addition, we find that spin waves with high frequencies up to several THz can be excited in Mn$_2$Au

Skyrmion States in Disk Geometry

In this work, we explore the stability of magnetic skyrmions confined in a disk geometry by analyzing how to switch a skyrmionic state in a circular disk into a uniformly magnetized state when applying an external magnetic field. The technologically highly relevant energy barrier between the skyrmion state and the uniformly magnetized state is a key parameter needed for lifetime calculations. In an infinite sample, this relates to the out-of-plane rupture field against the skyrmion-core direction, while in confined geometries the topological charge can also be changed by interactions with the sample edges. We find that annihilating a skyrmion with an applied field in the direction of the core magnetization—we call this expulsion—the energy barrier to the uniform state is generally around one order of magnitude lower than the annihilation via the rupture of the core in the disk center, which is observed when the applied field is acting in the direction opposite to the core magnetization. For the latter case a Bloch point (BP) needs to be nucleated to change the topological charge to zero. We find that the former case can be realistically calculated using micromagnetic simulations but that the annihilation via rupture, involving a Bloch point, needs to be calculated with the Heisenberg model because the high magnetization gradients present during the annihilation process cannot be accurately described within the micromagnetic framework