1,409 research outputs found
Strong enhancement of spin fluctuations in the low-temperature-tetragonal phase of antiferromagnetically ordered La_{2-x-y}Eu_ySr_xCuO_4
Measurements of the static magnetization, susceptibility and ESR of Gd spin
probes have been performed to study the properties of antiferromagnetically
ordered La_{2-x-y}Eu_ySr_xCuO_4 (x less or equal 0.02) with the low temperature
tetragonal structure. According to the static magnetic measurements the CuO_2
planes are magnetically decoupled in this structural phase. The ESR study
reveals strong magnetic fluctuations at the ESR frequency which are not present
in the orthorhombic phase. It is argued that this drastic enhancement of the
spin fluctuations is due to a considerable weakening of the interlayer exchange
and a pronounced influence of hole motion on the antiferromagnetic properties
of lightly hole doped La_2CuO_4. No evidence for the stripe phase formation at
small hole doping is obtained in the present study.Comment: 10 pages, LaTeX, 3 EPS figures; to be published in Journal of
Physics: Condensed Matte
Diffusion and jump-length distribution in liquid and amorphous CuZr
Using molecular dynamics simulation, we calculate the distribution of atomic
jum ps in CuZr in the liquid and glassy states. In both states
the distribution of jump lengths can be described by a temperature independent
exponential of the length and an effective activation energy plus a
contribution of elastic displacements at short distances. Upon cooling the
contribution of shorter jumps dominates. No indication of an enhanced
probability to jump over a nearest neighbor distance was found. We find a
smooth transition from flow in the liquid to jumps in the g lass. The
correlation factor of the diffusion constant decreases with decreasing
temperature, causing a drop of diffusion below the Arrhenius value, despite an
apparent Arrhenius law for the jump probability
Inhomogeneous Low Frequency Spin Dynamics in La_{1.65}Eu_{0.2}Sr_{0.15}CuO_4
We report Cu and La nuclear magnetic resonance (NMR) measurements in the
title compound that reveal an inhomogeneous glassy behavior of the spin
dynamics. A low temperature peak in the La spin lattice relaxation rate and the
``wipeout'' of Cu intensity both arise from these slow electronic spin
fluctuations that reveal a distribution of activation energies. Inhomogeneous
slowing of spin fluctuations appears to be a general feature of doped lanthanum
cuprate.Comment: 4 pages, 2 figures. Very slight modifications to figure
Dzyaloshinsky-Moriya Spin Canting in the LTT Phase of La2-x-yEuySrxCuO4
The Cu spin magnetism in La2-x-yEuySrxCuO4 (x<=0.17; y<=0.2) has been studied
by means of magnetization measurements up to 14 T. Our results clearly show
that in the antiferromagnetic phase Dzyaloshinsky-Moriya (DM)superexchange
causes Cu spin canting not only in the LTO phase but also in the LTLO and LTT
phases. In La1.8Eu0.2CuO4 the canted DM-moment is about 50% larger than in pure
La2CuO4 which we attribute to the larger octahedral tilt angle. We also find
clear evidence that the size of the DM-moment does not change significantly at
the structural transition at T_LT from LTO to LTLO and LTT. The most important
change induced by the transition is a significant reduction of the magnetic
coupling between the CuO2 planes. As a consequence, the spin-flip transition of
the canted Cu spins which is observed in the LTO phase for magnetic field
perpendicular to the CuO2 planes disappears in the LTT phase. The shape of the
magnetization curves changes from the well known spin-flip type to a
weak-ferromagnet type. However, no spontaneous weak ferromagnetism is observed
even at very low temperatures, which seems to indicate that the interlayer
decoupling in our samples is not perfect. Nonetheless, a small fraction (<15%)
of the DM-moments can be remanently magnetized throughout the entire
antiferromagnetically ordered LTT/LTLO phase, i.e. for T<T_LT and x<0.02. It
appears that the remanent DM-moment is perpendicular to the CuO2 planes. For
magnetic field parallel to the CuO2 planes we find that the critical field of
the spin-flop transition decreases in the LTLO phase, which might indicate a
competition between different in-plane anisotropies. To study the Cu spin
magnetism in La2-x-yEuySrxCuO4, a careful analysis of the Van Vleck
paramagnetism of the Eu3+ ions was performed.Comment: 22 pages, 27 figure
Decrease of the homogeneous width of the Tm3+ electron energy levels in TmBa2CCu3 O6+x at the superconducting transition
Enhanced NMR of 169Tm (I= 1 2) enhanced NMR has been studied in TmBa2Cu3O6+x, x=0, 0.2, 0.4, at temperatures 1.2-40K. The nuclear magnetic relaxation rates at T>20K increase exponentially as 1 T1(2) = R1(2)exp(-Δ/kT), with Δ = 176 K being the energy of the first excited state of the Tm3+ ion, while the R1(2) pre-exponential factors are inversely proportional to the homogenous width Γo of this doublet state. The pre-exponential factors measured at the frequencies of 48 and 69 MHz show homogeneous broadening of the 4f-levels due to the decreasing dipole-dipole transfer of the electron excitations from ion to ion at increasing because of crystal structure disordering. A sharp decrease of Γo (by about 0.9K) is observed in the superconducting compound with x=0.4 (Tc onset at 20K) at low temperatures and is attributed to the weakening of the 4f-electron-phonon interaction. At the temperatures around 6K the same sample displays enhancement of the transverse relaxation due to the relatively slow (W ≈ 109s-1) fluctuations of the internal magnetic fields caused by Cu2+ ions in CuO2 planes. © 1992
Systematic Cu-63 NQR studies of the stripe phase in La(1.6-x)Nd(0.4)Sr(x)CuO(4) for 0.07 <= x <= 0.25
We demonstrate that the integrated intensity of Cu-63 nuclear quadrupole
resonance (NQR) in La(1.6-x)Nd(0.4)Sr(x)CuO(4) decreases dramatically below the
charge-stripe ordering temperature T(charge). Comparison with neutron and X-ray
scattering indicates that the wipeout fraction F(T) (i.e. the missing fraction
of the integrated intensity of the NQR signal) represents the charge-stripe
order parameter. The systematic study reveals bulk charge-stripe order
throughout the superconducting region 0.07 <= x <= 0.25. As a function of the
reduced temperature t = T/T(charge), the temperature dependence of F(t) is
sharpest for the hole concentration x=1/8, indicating that x=1/8 is the optimum
concentration for stripe formation.Comment: 10 pages of text and captions, 11 figures in postscript. Final
version, with new data in Fig.
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