326 research outputs found
Direct observation of t2g orbital ordering in magnetite
Using soft-x-ray diffraction at the site-specific resonances in the Fe L23
edge, we find clear evidence for orbital and charge ordering in magnetite below
the Verwey transition. The spectra show directly that the (001/2) diffraction
peak (in cubic notation) is caused by t2g orbital ordering at octahedral Fe2+
sites and the (001) by a spatial modulation of the t2g occupation.Comment: to appear in Phys. Rev. Let
XANES study of rare-earth valency in LRu4P12 (L = Ce and Pr)
Valency of Ce and Pr in LRu4P12 (L = Ce and Pr) was studied by L2,3-edge
x-ray absorption near-edge structure (XANES) spectroscopy. The Ce-L3 XANES
spectrum suggests that Ce is mainly trivalent, but the 4f state strongly
hybridizes with ligand orbitals. The band gap of CeRu4P12 seems to be formed by
strong hybridization of 4f electrons. Pr-L2 XANES spectra indicate that Pr
exists in trivalent state over a wide range in temperature, 20 < T < 300 K. We
find that the metal-insulator (MI) transition at TMI = 60 K in PrRu4P12 does
not originate from Pr valence fluctuation.Comment: 4 page
Spatial Symmetry of Superconducting Gap in YBa2Cu3O7-\delta Obtained from Femtosecond Spectroscopy
The polarized femtosecond spectroscopies obtained from well characterized
(100) and (110) YBa2Cu3O7-\delta thin films are reported. This bulk-sensitive
spectroscopy, combining with the well-textured samples, serves as an effective
probe to quasiparticle relaxation dynamics in different crystalline
orientations. The significant anisotropy in both the magnitude of the
photoinduced transient reflectivity change and the characteristic relaxation
time indicates that the nature of the relaxation channel is intrinsically
different in various axes and planes. By the orientation-dependent analysis,
d-wave symmetry of the bulk-superconducting gap in cuprate superconductors
emerges naturally.Comment: 8 pages, 4 figures. To be published in Physical Review B, Rapid
Communication
Parity forbidden excitations of Sr2CuO2Cl2 revealed by optical third-harmonic spectroscopy
We present the first study of nonlinear optical third harmonic generation in
the strongly correlated charge-transfer insulator Sr2CuO2Cl2. For fundamental
excitation in the near-infrared, the THG spectrum reveals a strongly resonant
response for photon energies near 0.7 eV. Polarization analysis reveals this
novel resonance to be only partially accounted for by three-photon excitation
to the optical charge-transfer exciton, and indicates that an even-parity
excitation at 2 eV, with a_1g symmetry, participates in the third harmonic
susceptibility.Comment: Requires RevTeX v4.0beta
Relaxation Dynamics of Photoinduced Changes in the Superfluid Weight of High-Tc Superconductors
In the transient state of d-wave superconductors, we investigate the temporal
variation of photoinduced changes in the superfluid weight. We derive the
formula that relates the nonlinear response function to the nonequilibrium
distribution function. The latter qunatity is obtained by solving the kinetic
equation with the electron-electron and the electron-phonon interaction
included. By numerical calculations, a nonexponential decay is found at low
temperatures in contrast to the usual exponential decay at high temperatures.
The nonexponential decay originates from the nonmonotonous temporal variation
of the nonequilibrium distribution function at low energies. The main physical
process that causes this behavior is not the recombination of quasiparticles as
previous phenomenological studies suggested, but the absorption of phonons.Comment: 18 pages, 12 figures; to be published in J. Phys. Soc. Jpn. Vol. 80,
No.
Characteristic features of the temperature dependence of the surface impedance in polycrystalline MgB samples
The real and imaginary parts of the surface impedance
in polycrystalline MgB samples of different density
with the critical temperature K are measured at the frequency
of 9.4 GHz and in the temperature range K. The normal skin-effect
condition at holds only for the samples of the
highest density with roughness sizes not more than 0.1 m. For such samples
extrapolation of the linear at temperature dependences
and results in values of the London
penetration depth \AA and residual surface resistance
m. In the entire temperature range the dependences
and are well described by the modified two-fluid model.Comment: 7 pages, 3 figures. Europhysics Letters, accepted for publicatio
Direct observation of electron doping in La0.7Ce0.3MnO3 using x-ray absorption spectroscopy
We report on a X-ray absorption spectroscopic (XAS) study on a thin film of
La0.7Ce0.3MnO3, a manganite which was previously only speculated to be an
electron doped system. The measurements clearly show that the cerium is in the
Ce(IV) valence state and that the manganese is present in a mixture of Mn2+ and
Mn3+ valence states. These data unambiguously demonstrate that La0.7Ce0.3MnO3
is an electron doped colossal magnetoresistive manganite, a finding that may
open up new opportunities both for device applications as well as for further
basic research towards a better modelling of the colossal magnetoresistance
phenomenon in these materials.Comment: 4 pages, 3 figures, revised versio
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