Nuclear Ground-State Masses and Deformations

We tabulate the atomic mass excesses and nuclear ground-state deformations of 8979 nuclei ranging from $^{16}$O to $A=339$. The calculations are based on the finite-range droplet macroscopic model and the folded-Yukawa single-particle microscopic model. Relative to our 1981 mass table the current results are obtained with an improved macroscopic model, an improved pairing model with a new form for the effective-interaction pairing gap, and minimization of the ground-state energy with respect to additional shape degrees of freedom. The values of only 9 constants are determined directly from a least-squares adjustment to the ground-state masses of 1654 nuclei ranging from $^{16}$O to $^{263}$106 and to 28 fission-barrier heights. The error of the mass model is 0.669~MeV for the entire region of nuclei considered, but is only 0.448~MeV for the region above $N=65$.Comment: 50 pages plus 20 PostScript figures and 160-page table obtainable by anonymous ftp from t2.lanl.gov in directory masses, LA-UR-93-308

Ambiguities in statistical calculations of nuclear fragmentation

The concept of freeze out volume used in many statistical approaches for disassembly of hot nuclei leads to ambiguities. The fragmentation pattern and the momentum distribution (temperature) of the emanated fragments are determined by the phase space at the freeze-out volume where the interaction among the fragments is supposedly frozen out. However, to get coherence with the experimental momentum distribution of the charged particles, one introduces Coulomb acceleration beyond this freeze-out. To be consistent, we investigate the effect of the attractive nuclear force beyond this volume and find that the possible recombination of the fragments alters the physical observables significantly casting doubt on the consistency of the statistical model.Comment: 11 pages+3 figure

True ternary fission of superheavy nuclei

We found that a true ternary fission with formation of a heavy third fragment (a new type of radioactivity) is quite possible for superheavy nuclei due to the strong shell effects leading to a three-body clusterization with the two doubly magic tin-like cores. The simplest way to discover this phenomenon in the decay of excited superheavy nuclei is a detection of two tin-like clusters with appropriate kinematics in low-energy collisions of medium mass nuclei with actinide targets. The three-body quasi-fission process could be even more pronounced for giant nuclear systems formed in collisions of heavy actinide nuclei. In this case a three-body clusterization might be proved experimentally by detection of two coincident lead-like fragments in low-energy U+U collisions.Comment: 4 pages, 7 figure

Stability of bubble nuclei through Shell-Effects

We investigate the shell structure of bubble nuclei in simple phenomenological shell models and study their binding energy as a function of the radii and of the number of neutron and protons using Strutinsky's method. Shell effects come about, on the one hand, by the high degeneracy of levels with large angular momentum and, on the other, by the big energy gaps between states with a different number of radial nodes. Shell energies down to -40 MeV are shown to occur for certain magic nuclei. Estimates demonstrate that the calculated shell effects for certain magic numbers of constituents are probably large enough to produce stability against fission, alpha-, and beta-decay. No bubble solutions are found for mass number A < 450.Comment: 9 pages and 9 figures in the eps format include

Modelling of compound nucleus formation in fusion of heavy nuclei

A new model that includes the time-dependent dynamics of the single-particle (s.p.) motion in conjunction with the macroscopic evolution of the system is proposed for describing the compound nucleus (CN) formation in fusion of heavy nuclei. The diabaticity initially keeps the entrance system around its contact configuration, but the gradual transition from the diabatic to the adiabatic potential energy surface (PES) leads to fusion or quasifission. Direct measurements of the probability for CN formation are crucial to discriminate between the current models.Comment: 4 pages,2 figures,1 table, Submitted to PR

Microscopic Enhancement of Heavy-Element Production

Realistic fusion barriers are calculated in a macroscopic-microscopic model for several soft-fusion heavy-ion reactions leading to heavy and superheavy elements. The results obtained in such a realistic picture are very different from those obtained in a purely macroscopic model. For reactions on 208:Pb targets, shell effects in the entrance channel result in fusion-barrier energies at the touching point that are only a few MeV higher than the ground state for compound systems near Z = 110. The entrance-channel fragment-shell effects remain far inside the touching point, almost to configurations only slightly more elongated than the ground-state configuration, where the fusion barrier has risen to about 10 MeV above the ground-state energy. Calculated single-particle level diagrams show that few level crossings occur until the peak in the fusion barrier very close to the ground-state shape is reached, which indicates that dissipation is negligible until very late in the fusion process. Whereas the fission valley in a macroscopic picture is several tens of MeV lower in energy than is the fusion valley, we find in the macroscopic-microscopic picture that the fission valley is only about 5 MeV lower than the fusion valley for soft-fusion reactions leading to compound systems near Z = 110. These results show that no significant ``extra-extra-push'' energy is needed to bring the system inside the fission saddle point and that the typical reaction energies for maximum cross section in heavy-element synthesis correspond to only a few MeV above the maximum in the fusion barrier.Comment: 7 pages. LaTeX. Submitted to Zeitschrift fur Physik A. 5 figures not included here. Complete preprint, including device-independent (dvi), PostScript, and LaTeX versions of the text, plus PostScript files of the figures, available at http://t2.lanl.gov/publications/publications.html or at ftp://t2.lanl.gov/pub/publications/mehe

Equilibration in the time-dependent Hartree-Fock approach probed with the Wigner distribution function

Calculating the Wigner distribution function in the reaction plane, we are able to probe the phase-space behavior in time-dependent Hartree-Fock during a heavy-ion collision. We compare the Wigner distribution function with the smoothed Husimi distribution function. Observables are defined to give a quantitative measure for local and global equilibration. We present different reaction scenarios by analyzing central and non-central $^{16}O+$$^{16}O$ and $^{96}Zr+$$^{132}Zn$ collisions. It is shown that the initial phase-space volumes of the fragments barely merge. The mean values of the observables are conserved in fusion reactions and indicate a "memory effect" in time-dependent Hartree-Fock. We observe strong dissipation but no evidence for complete equilibration.Comment: 12 pages, 10 figure