34 research outputs found
Lithium Ionization by a Strong Laser Field
We study ab initio computations of the interaction of Lithium with a strong
laser field. Numerical solutions of the time-dependent fully-correlated
three-particle Schroedinger equation restricted to the one-dimensional
soft-core approximation are presented. Our results show a clear transition from
non-sequential to sequential double ionization for increasing intensities. Non
sequential double ionization is found to be sensitive to the spin configuration
of the ionized pair. This asymmetry, also found in experiments of
photoionization of Li with synchrotron radiation, shows the evidence of the
influence of the exclusion principle in the underlying rescattering mechanism
Momentum distributions in time-dependent density functional theory: Product phase approximation for non-sequential double ionization in strong laser fields
We investigate the possibility to deduce momentum space properties from
time-dependent density functional calculations. Electron and ion momentum
distributions after double ionization of a model Helium atom in a strong
few-cycle laser pulse are studied. We show that, in this case, the choice of
suitable functionals for the observables is considerably more important than
the choice of the correlation potential in the time-dependent Kohn-Sham
equations. By comparison with the solution of the time-dependent Schroedinger
equation, the insufficiency of functionals neglecting electron correlation is
demonstrated. We construct a functional of the Kohn-Sham orbitals, which in
principle yields the exact momentum distributions of the electrons and the ion.
The product-phase approximation is introduced, which reduces the problem of
approximating this functional significantly.Comment: 8 pages, 5 figures, RevTeX
Second-harmonic generation in silicon waveguides strained by silicon nitride
Silicon photonics meets the electronics requirement of increased speed and bandwidth with on-chip optical networks.
All-optical data management requires nonlinear silicon photonics. In silicon only third-order optical nonlinearities are present
owing to its crystalline inversion symmetry. Introducing a second-order nonlinearity into silicon photonics by proper material
engineering would be highly desirable. It would enable devices for wideband wavelength conversion operating at relatively low
optical powers. Here we show that a sizeable second-order nonlinearity at optical wavelengths is induced in a silicon waveguide
by using a stressing silicon nitride overlayer. We carried out second-harmonic-generation experiments and first-principle
calculations, which both yield large values of strain-induced bulk second-order nonlinear susceptibility, up to 40pm/V at
2.300 nm. We envisage that nonlinear strained silicon could provide a competing platform for a new class of integrated light
sources spanning the near- to mid-infrared spectrum from 1.2 to 10 micron
Adiabatic Theory of Electron Detachment from Negative Ions in Two-Color Laser Field
Negative ion detachment in bichromatic laser field is considered within the
adiabatic theory. The latter represents a recent modification of the famous
Keldysh model for multiphoton ionization which makes it quantitatively
reliable. We calculate angular differential detachment rates, partial rates for
particular ATD (Above Threshold Detachment) channels and total detachment rates
for the Hydrogen ion in a bichromatic field with 1:3 frequency ratio and
various phase differences. Reliability of the present, extremely simple
approach is testified by comparison with much more elaborate earlier
calculations.Comment: 22 pages, 6 Postscript figure
Mathematical Properties of a New Levin-Type Sequence Transformation Introduced by \v{C}\'{\i}\v{z}ek, Zamastil, and Sk\'{a}la. I. Algebraic Theory
\v{C}\'{\i}\v{z}ek, Zamastil, and Sk\'{a}la [J. Math. Phys. \textbf{44}, 962
- 968 (2003)] introduced in connection with the summation of the divergent
perturbation expansion of the hydrogen atom in an external magnetic field a new
sequence transformation which uses as input data not only the elements of a
sequence of partial sums, but also explicit estimates
for the truncation errors. The explicit
incorporation of the information contained in the truncation error estimates
makes this and related transformations potentially much more powerful than for
instance Pad\'{e} approximants. Special cases of the new transformation are
sequence transformations introduced by Levin [Int. J. Comput. Math. B
\textbf{3}, 371 - 388 (1973)] and Weniger [Comput. Phys. Rep. \textbf{10}, 189
- 371 (1989), Sections 7 -9; Numer. Algor. \textbf{3}, 477 - 486 (1992)] and
also a variant of Richardson extrapolation [Phil. Trans. Roy. Soc. London A
\textbf{226}, 299 - 349 (1927)]. The algebraic theory of these transformations
- explicit expressions, recurrence formulas, explicit expressions in the case
of special remainder estimates, and asymptotic order estimates satisfied by
rational approximants to power series - is formulated in terms of hitherto
unknown mathematical properties of the new transformation introduced by
\v{C}\'{\i}\v{z}ek, Zamastil, and Sk\'{a}la. This leads to a considerable
formal simplification and unification.Comment: 41 + ii pages, LaTeX2e, 0 figures. Submitted to Journal of
Mathematical Physic
High Order Harmonic Generation and Atomic Stabilization in Ultra-Intense Laser Pulses
We present results of recent numerical simulations on the non-linear response of a single-electron atom submitted to an intense laser pulse. We address both the questions of the light scattered by the atom and the possible stabilization against ionization. One of the results of our simulations is the the presence of hyper-Raman lines in the high-order harmonic spectra. We suggest that these lines could be a signature of atomic stabilization
SOME NEW PERSPECTIVES IN BREMSSTRAHLUNG RESEARCH
Nous présentons les résultats de calculs théoriques
nouveaux des amplitudes de transition et sections efficaces relatives à deux
types distincts de processus associés au bremsstrahlung : a) Transitions
stimulées à un photon (transitions "libre-libre") ayant lieu au cours de
collisions électron-atome d' hydrogène, en présence d' un champ extérieur
intense. b) Bremsstrahlung à deux photons, correspondant à l'émission spontanée
de deux photons distincts lors d'une seule collision électron-atome. Les
caractéristiques essentielles de ces processus sont mises en évidence et
discutées.We report the results of new theoretical calculations of
the transition amplitudes and cross-sections for two distinct
bremsstrahlung-related processes : i) Stimulated one-photon transitions
(Free-Free Transitions) occuning in the course of electron-H atom collisions,
in the presence of a strong extemal field. ii) Two-photon Bremsstrahlung,
corresponding to the spontaneous emission of two distinct photons in a single
electron-atom collision event. The main features of these processes will be
outlined and discussed
Two-photon transitions in hydrogenic atoms via a Sturmian basis for the Dirac Coulomb Green's function
Using a Sturmian-like expansion
of the (first-order) Dirac Coulomb Green's
function, the two-photon
probability amplitude for the
transition in hydrogenic systems is calculated as a function
of nuclear charge Z. A comparison between relativistic and
non-relativistic treatments is made, taking care of
the influence of retardation in both cases