16 research outputs found
Magnetic remanent states in antiferromagnetically coupled multilayers
In antiferromagnetically coupled multilayers with perpendicular anisotropy
unusual multidomain textures can be stabilized due to a close competition
between long-range demagnetization fields and short-range interlayer exchange
coupling.
In particular, the formation and evolution of specific topologically stable
planar defects within the antiferromagnetic ground state, i.e. wall-like
structures with a ferromagnetic configuration extended over a finite width,
explain configurational hysteresis phenomena recently observed in
[Co/Pt(Pd)]/Ru and [Co/Pt]/NiO multilayers.
Within a phenomenological theory, we have analytically derived the
equilibrium sizes of these "ferroband" defects as functions of the
antiferromagnetic exchange, a bias magnetic field, and geometrical parameters
of the multilayers. In the magnetic phase diagram, the existence region of the
ferrobands mediates between the regions of patterns with sharp
antiferromagnetic domain walls and regular arrays of ferromagnetic stripes.
The theoretical results are supported by magnetic force microscopy images of
the remanent states observed in [Co/Pt]/Ru.Comment: Paper submitted by the Joint European Magnetics Symposia 2008, Dublin
(4 pages, 3 figures
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V4 tetrahedral units in AV4X8 lacunar spinels: Near degeneracy, charge fluctuations, and configurational mixing within a valence space of up to 21 d orbitals
All properties of a given molecule or solid are determined by the way valence electrons are distributed over single-particle energy levels. For multiple, closely spaced single-particle levels, different occupation patterns may provide many-electron quantum states that are close in energy, interact, and admix. We address such near-degeneracy electron correlation effects for V4 vanadium tetrahedral units as encountered in the lacunar spinel GaV4S8, explicitly taking into account up to 21 vanadium valence orbitals, and find effective orbital occupation numbers much different as compared to the picture previously laid out on the basis of mean-field calculations. In light of these results, a modified theoretical frame seems necessary to explain the peculiar magnetic properties of lacunar spinels and of related compounds
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Chiral Spin Liquid Ground State in YBaCo3FeO7
A chiral spin liquid state is discovered in the highly frustrated, noncentrosymmetric swedenborgite compound YBaCo3FeO7, a layered kagome system of hexagonal symmetry, by advanced polarized neutron scattering from a single domain crystalline sample. The observed diffuse magnetic neutron scattering has an antisymmetric property that relates to its specific chirality, which consists of three cycloidal waves perpendicular to the c axis, forming an entity of cylindrical symmetry. Chirality and symmetry agree with relevant antisymmetric exchanges arising from broken spatial parity. Applying a Fourier analysis to the chiral interference pattern, with distinction between kagome sites and the connecting trigonal interlayer sites of threefold symmetry, the chiral spin correlation function is determined. Characteristic chiral waves originate from the trigonal sites and extend over several periods in the kagome planes. The chiral spin liquid is remarkably stable at low temperatures despite strong antiferromagnetic spin exchange. The observation raises a challenge, since the commonly accepted ground states in condensed matter either have crystalline long-range order or form a quantum liquid. We show that, within the classical theory of magnetic order, a disordered ground state may arise from chirality. The present scenario, with antisymmetric exchange acting as a frustrating gauge background that stabilizes local spin lumps, is similar to the avoided phase transition in coupled gauge and matter fields for subnuclear particles
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Visualization of localized perturbations on a (001) surface of the ferromagnetic semimetal EuB6
We performed scanning tunneling microscopy (STM) and spectroscopy on a (001) surface of the ferromagnetic semimetal EuB6. Large-amplitude oscillations emanating from the elastic scattering of electrons by the surface impurities are observed in topography and in differential conductance maps. Fourier transform of the conductance maps embracing these regions indicate a holelike dispersion centered around the Γ point of the two-dimensional Brillouin zone. Using density functional theory slab calculations, we identify a spin-split surface state, which stems from the dangling pz orbitals of the apical boron atom. Hybridization with bulk electronic states leads to a resonance enhancement in certain regions around the Γ point, contributing to the remarkably strong real-space response around static point defects, which are observed in STM measurements
Modulations in martensitic Heusler alloys originate from nanotwin ordering
Heusler alloys exhibiting magnetic and martensitic transitions enable applications like magnetocaloric refrigeration and actuation based on the magnetic shape memory effect. Their outstanding functional properties depend on low hysteresis losses and low actuation fields. These are only achieved if the atomic positions deviate from a tetragonal lattice by periodic displacements. The origin of the so-called modulated structures is the subject of much controversy: They are either explained by phonon softening or adaptive nanotwinning. Here we used large-scale density functional theory calculations on the Ni2MnGa prototype system to demonstrate interaction energy between twin boundaries. Minimizing the interaction energy resulted in the experimentally observed ordered modulations at the atomic scale, it explained that a/b twin boundaries are stacking faults at the mesoscale, and contributed to the macroscopic hysteresis losses. Furthermore, we found that phonon softening paves the transformation path towards the nanotwinned martensite state. This unified both opposing concepts to explain modulated martensite
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Mesoscale Dzyaloshinskii-Moriya interaction: Geometrical tailoring of the magnetochirality
Crystals with broken inversion symmetry can host fundamentally appealing and technologically relevant periodical or localized chiral magnetic textures. The type of the texture as well as its magnetochiral properties are determined by the intrinsic Dzyaloshinskii-Moriya interaction (DMI), which is a material property and can hardly be changed. Here we put forth a method to create new artificial chiral nanoscale objects with tunable magnetochiral properties from standard magnetic materials by using geometrical manipulations. We introduce a mesoscale Dzyaloshinskii-Moriya interaction that combines the intrinsic spin-orbit and extrinsic curvature-driven DMI terms and depends both on the material and geometrical parameters. The vector of the mesoscale DMI determines magnetochiral properties of any curved magnetic system with broken inversion symmetry. The strength and orientation of this vector can be changed by properly choosing the geometry. For a specific example of nanosized magnetic helix, the same material system with different geometrical parameters can acquire one of three zero-temperature magnetic phases, namely, phase with a quasitangential magnetization state, phase with a periodical state and one intermediate phase with a periodical domain wall state. Our approach paves the way towards the realization of a new class of nanoscale spintronic and spinorbitronic devices with the geometrically tunable magnetochirality
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Signatures of a magnetic field-induced unconventional nematic liquid in the frustrated and anisotropic spin-chain cuprate LiCuSbO4
Modern theories of quantum magnetism predict exotic multipolar states in weakly interacting strongly frustrated spin-1/2 Heisenberg chains with ferromagnetic nearest neighbor (NN) inchain exchange in high magnetic fields. Experimentally these states remained elusive so far. Here we report strong indications of a magnetic field-induced nematic liquid arising above a field of ~13 T in the edge-sharing chain cuprate LiSbCuO4 ≡ LiCuSbO4. This interpretation is based on the observation of a field induced spin-gap in the measurements of the 7Li NMR spin relaxation rate T1−1 as well as a contrasting field-dependent power-law behavior of T1−1 vs. T and is further supported by static magnetization and ESR data. An underlying theoretical microscopic approach favoring a nematic scenario is based essentially on the NN XYZ exchange anisotropy within a model for frustrated spin-1/2 chains and is investigated by the DMRG technique. The employed exchange parameters are justified qualitatively by electronic structure calculations for LiCuSbO4
Magnetic phases and reorientation transitions in antiferromagnetically coupled multilayers
In antiferromagnetically coupled superlattices grown on (001) faces of cubic
substrates, e.g. based on materials combinations as Co/Cu, Fe/Si, Co/Cr, or
Fe/Cr, the magnetic states evolve under competing influence of bilinear and
biquadratic exchange interactions, surface-enhanced four-fold in-plane
anisotropy, and specific finite-size effects. Using phenomenological
(micromagnetic) theory, a comprehensive survey of the magnetic states and
reorientation transitions has been carried out for multilayer systems with even
number of ferromagnetic sub-layers and magnetizations in the plane. In
two-layer systems (N=2) the phase diagrams in dependence on components of the
applied field in the plane include ``swallow-tail'' type regions of
(metastable) multistate co-existence and a number of continuous and
discontinuous reorientation transitions induced by radial and transversal
components of the applied field. In multilayers (N \ge 4) noncollinear states
are spatially inhomogeneous with magnetization varying across the multilayer
stack. For weak four-fold anisotropy the magnetic states under influence of an
applied field evolve by a complex continuous reorientation into the saturated
state. At higher anisotropy they transform into various inhomogeneous and
asymmetric structures. The discontinuous transitions between the magnetic
states in these two-layers and multilayers are characterized by broad ranges of
multi-phase coexistence of the (metastable) states and give rise to specific
transitional domain structures.Comment: Manuscript 34 pages, 14 figures; submitted for publicatio
Effect of Composition Changes on the Structural Relaxation of a Binary Mixture
Within the mode-coupling theory for idealized glass transitions, we study the
evolution of structural relaxation in binary mixtures of hard spheres with size
ratios of the two components varying between 0.5 and 1.0. We find two
scenarios for the glassy dynamics. For small size disparity, the mixing yields
a slight extension of the glass regime. For larger size disparity, a
plasticization effect is obtained, leading to a stabilization of the liquid due
to mixing. For all , a decrease of the elastic moduli at the transition
due to mixing is predicted. A stiffening of the glass structure is found as is
reflected by the increase of the Debye-Waller factors at the transition points.
The critical amplitudes for density fluctuations at small and intermediate wave
vectors decrease upon mixing, and thus the universal formulas for the
relaxation near the plateau values describe a slowing down of the dynamics upon
mixing for the first step of the two-step relaxation scenario. The results
explain the qualitative features of mixing effects reported by Williams and van
Megen [Phys. Rev. E \textbf{64}, 041502 (2001)] for dynamical light-scattering
measurements on binary mixtures of hard-sphere-like colloids with size ratio