Microscopic study of induced fission dynamics of 226^{226}Th with covariant energy density functionals

Static and dynamic aspects of the fission process of $^{226}$Th are analyzed in a self-consistent framework based on relativistic energy density functionals. Constrained relativistic mean-field (RMF) calculations in the collective space of axially symmetric quadrupole and octupole deformations, based on the energy density functional PC-PK1 and a $\delta$-force pairing, are performed to determine the potential energy surface of the fissioning nucleus, the scission line, the single-nucleon wave functions, energies and occupation probabilities, as functions of deformation parameters. Induced fission dynamics is described using the time-dependent generator coordinate method in the Gaussian overlap approximation. A collective Schr\"odinger equation, determined entirely by the microscopic single-nucleon degrees of freedom, propagates adiabatically in time the initial wave packet built by boosting the ground-state solution of the collective Hamiltonian for $^{226}$Th. The position of the scission line and the microscopic input for the collective Hamiltonian are analyzed as functions of the strength of the pairing interaction. The effect of static pairing correlations on the pre-neutron emission charge yields and total kinetic energy of fission fragments is examined in comparison with available data, and the distribution of fission fragments is analyzed for different values of the initial excitation energy.Comment: 25 pages, 14 figures, accepted for publication in Phys. Rev.

Spectroscopy of reflection-asymmetric nuclei with relativistic energy density functionals

Quadrupole and octupole deformation energy surfaces, low-energy excitation spectra and transition rates in fourteen isotopic chains: Xe, Ba, Ce, Nd, Sm, Gd, Rn, Ra, Th, U, Pu, Cm, Cf, and Fm, are systematically analyzed using a theoretical framework based on a quadrupole-octupole collective Hamiltonian (QOCH), with parameters determined by constrained reflection-asymmetric and axially-symmetric relativistic mean-field calculations. The microscopic QOCH model based on the PC-PK1 energy density functional and $\delta$-interaction pairing is shown to accurately describe the empirical trend of low-energy quadrupole and octupole collective states, and predicted spectroscopic properties are consistent with recent microscopic calculations based on both relativistic and non-relativistic energy density functionals. Low-energy negative-parity bands, average octupole deformations, and transition rates show evidence for octupole collectivity in both mass regions, for which a microscopic mechanism is discussed in terms of evolution of single-nucleon orbitals with deformation.Comment: 36 pages, 21 figures, Accepted for Publication in Physical Review

Catastrophic Photo-z Errors and the Dark Energy Parameter Estimates with Cosmic Shear

We study the impact of catastrophic errors occurring in the photometric redshifts of galaxies on cosmological parameter estimates with cosmic shear tomography. We consider a fiducial survey with 9-filter set and perform photo-z measurement simulations. It is found that a fraction of 1% galaxies at z_{spec}~0.4 is misidentified to be at z_{phot}~3.5. We then employ both chi^2 fitting method and the extension of Fisher matrix formalism to evaluate the bias on the equation of state parameters of dark energy, w_0 and w_a, induced by those catastrophic outliers. By comparing the results from both methods, we verify that the estimation of w_0 and w_a from the fiducial 5-bin tomographic analyses can be significantly biased. To minimize the impact of this bias, two strategies can be followed: (A) the cosmic shear analysis is restricted to 0.5<z<2.5 where catastrophic redshift errors are expected to be insignificant; (B) a spectroscopic survey is conducted for galaxies with 3<z_{phot}<4. We find that the number of spectroscopic redshifts needed scales as N_{spec} \propto f_{cata}\times A where f_{cata}=1% is the fraction of catastrophic redshift errors (assuming a 9-filter photometric survey) and A is the survey area. For A=1000 {deg}^2, we find that N_{spec}>320 and 860 respectively in order to reduce the joint bias in (w_0,w_a) to be smaller than 2\sigma and 1\sigma. This spectroscopic survey (option B) will improve the Figure of Merit of option A by a factor \times 1.5 thus making such a survey strongly desirable.Comment: 25 pages, 9 figures. Revised version, as accepted for publication in Ap

Electron-Angular-Distribution Reshaping in Quantum Radiation-Dominated Regime

Dynamics of an electron beam head-on colliding with an ultraintense focused ultrashort circularly-polarized laser pulse are investigated in the quantum radiation-dominated regime. Generally, the ponderomotive force of the laser fields may deflect the electrons transversely, to form a ring structure on the cross-section of the electron beam. However, we find that when the Lorentz factor of the electron $\gamma$ is approximately one order of magnitude larger than the invariant laser field parameter $\xi$, the stochastic nature of the photon emission leads to electron aggregation abnormally inwards to the propagation axis of the laser pulse. Consequently, the electron angular distribution after the interaction exhibits a peak structure in the beam propagation direction, which is apparently distinguished from the "ring"-structure of the distribution in the classical regime, and therefore, can be recognized as a proof of the fundamental quantum stochastic nature of radiation. The stochasticity signature is robust with respect to the laser and electron parameters and observable with current experimental techniques

Catalytic efficiency and stability of cobalt hydroxide for decomposition of ozone and p-chloronitrobenzene in water

Cobalt hydroxide, a stable and efficient catalyst prepared in the laboratory, has been successfully used in the decomposition of ozone and trace quantities of p-chloronitrobenzene (pCNB) in water. The cobalt hydroxide was characterized by X-ray diffraction (XRD), scanning electron microscopy (SEM) and the Brunauer-Emmet-Teller (BET) method. The decomposition rate of aqueous ozone was increased by 1.527 times in the presence of cobalt hydroxide. Increasing the catalyst loading from 0 to 500 mg/L increased the removal efficiency of pCNB from 59% to 99%. The catalyst morphology and its composition were found to be unaltered after the catalytic reaction. After five successive recycles, the catalyst remained stable in the catalytic ozonation of pCNB