Charge Ordering and Spin Dynamics in NaV2O5

We report high-resolution neutron inelastic scattering experiments on the spin excitations of NaV2O5. Below Tc, two branches associated with distinct energy gaps are identified. From the dispersion and intensity of the spin excitation modes, we deduce the precise zig-zag charge distribution on the ladder rungs and the corresponding charge order (about 0.6). We argue that the spin gaps observed in the low-T phase of this compound are primarily due to the charge transfer.Comment: 4 pages, 5 figures, to appear in Phys. Rev. Let

Deviations from Matthiessen's Rule for SrRuO3{\rm SrRuO_3} and CaRuO3{\rm CaRuO_3}

We have measured the change in the resistivity of thin films of ${\rm SrRuO_3}$ and ${\rm CaRuO_3}$ upon introducing point defects by electron irradiation at low temperatures, and we find significant deviations from Matthiessen's rule. For a fixed irradiation dose, the induced change in resistivity {\it decreases} with increasing temperature. Moreover, for a fixed temperature, the increase in resistivity with irradiation is found to be {\it sublinear}. We suggest that the observed behavior is due to the marked anisotropic scattering of the electrons together with their relatively short mean free path (both characteristic of many metallic oxides including cuprates) which amplify effects related to the Pippard ineffectiveness condition

Weak spin-orbit interactions induce exponentially flat mini-bands in magnetic metals without inversion symmetry

In metallic magnets like MnSi the interplay of two very weak spin-orbit coupling effects can strongly modify the Fermi surface. In the absence of inversion symmetry even a very small Dzyaloshinsky-Moriya interaction of strength delta<<1 distorts a ferromagnetic state into a chiral helix with a long pitch of order 1/delta. We show that additional small spin-orbit coupling terms of order delta in the band structure lead to the formation of exponentially flat minibands with a bandwidth of order exp(-1/sqrt(delta)) parallel to the direction of the helix. These flat minibands cover a rather broad belt of width sqrt(delta) on the Fermi surface where electron motion parallel to the helix practically stops. We argue that these peculiar band-structure effects lead to pronounced features in the anomalous skin effect.Comment: 7 pages, minor corrections, references adde

Ab-initio study of the thermopower of biphenyl-based single-molecule junctions

Employing ab-initio electronic structure calculations combined with the non-equilibrium Green's function technique, we study the dependence of the thermopower Q on the conformation in biphenyl-based single-molecule junctions. For the series of experimentally available biphenyl molecules, alkyl side chains allow us to gradually adjust the torsion angle \phi\ between the two phenyl rings from 0 to 90{\deg} and to control in this way the degree of \pi-electron conjugation. Studying different anchoring groups and binding positions, our theory predicts that the absolute values of the thermopower decrease slightly towards larger torsion angles, following an a+b*cos^{2}\phi\ dependence. The anchoring group determines the sign of Q and a,b, simultaneously. Sulfur and amine groups give rise to Q,a,b>0, while for cyano Q,a,b<0. The different binding positions can lead to substantial variations of the thermopower mostly due to changes in the alignment of the frontier molecular orbital levels and the Fermi energy. We explain our ab-initio results in terms of a \pi-orbital tight-binding model and a minimal two-level model, which describes the pair of hybridizing frontier orbital states on the two phenyl rings. The variations of the thermopower with \phi\ seem to be within experimental resolution.Comment: 8 pages, 4 figues, 3 table

The localization transition at finite temperatures: electric and thermal transport

The Anderson localization transition is considered at finite temperatures. This includes the electrical conductivity as well as the electronic thermal conductivity and the thermoelectric coefficients. An interesting critical behavior of the latter is found. A method for characterizing the conductivity critical exponent, an important signature of the transition, using the conductivity and thermopower measurements, is outlined.Comment: Article for the book: "50 Years of Anderson Localization", edited by E. Abrahams (World Scientific, Singapore, 2010

Heat transport in ultra-thin dielectric membranes and bridges

Phonon modes and their dispersion relations in ultrathin homogenous dielectric membranes are calculated using elasticity theory. The approach differs from the previous ones by a rigorous account of the effect of the film surfaces on the modes with different polarizations. We compute the heat capacity of membranes and the heat conductivity of narrow bridges cut out of such membranes, in a temperature range where the dimensions have a strong influence on the results. In the high temperature regime we recover the three-dimensional bulk results. However, in the low temperature limit the heat capacity, $C_V$, is proportional with $T$ (temperature), while the heat conductivity, $\kappa$, of narrow bridges is proportional to $T^{3/2}$, leading to a thermal cut-off frequency $f_c=\kappa/C_V\propto T^{1/2}$.Comment: 6 pages and 6 figure

Incomplete quantum process tomography and principle of maximal entropy

The main goal of this paper is to extend and apply the principle of maximum entropy (MaxEnt) to incomplete quantum process estimation tasks. We will define a so-called process entropy function being the von Neumann entropy of the state associated with the quantum process via Choi-Jamiolkowski isomorphism. It will be shown that an arbitrary process estimation experiment can be reformulated in a unified framework and MaxEnt principle can be consistently exploited. We will argue that the suggested choice for the process entropy satisfies natural list of properties and it reduces to the state MaxEnt principle, if applied to preparator devices.Comment: 8 pages, comments welcome, references adde

Sequential and co-tunneling behavior in the temperature-dependent thermopower of few-electron quantum dots

We have studied the temperature dependent thermopower of gate-defined, lateral quantum dots in the Coulomb blockade regime using an electron heating technique. The line shape of the thermopower oscillations depends strongly on the contributing tunneling processes. Between 1.5 K and 40 mK a crossover from a pure sawtooth- to an intermitted sawtooth-like line shape is observed. The latter is attributed to the increasing dominance of cotunneling processes in the Coulomb blockade regime at low temperatures.Comment: 4 pages, 4 figures, submitted to Phys. Rev.

Kinetic Limit for Wave Propagation in a Random Medium

We study crystal dynamics in the harmonic approximation. The atomic masses are weakly disordered, in the sense that their deviation from uniformity is of order epsilon^(1/2). The dispersion relation is assumed to be a Morse function and to suppress crossed recollisions. We then prove that in the limit epsilon to 0 the disorder averaged Wigner function on the kinetic scale, time and space of order epsilon^(-1), is governed by a linear Boltzmann equation.Comment: 71 pages, 3 figure

Theory of helimagnons in itinerant quantum systems II: Nonanalytic corrections to Fermi-liquid behavior

A recent theory for the ordered phase of helical or chiral magnets such as MnSi is used to calculate observable consequences of the helical Goldstone modes or helimagnons. In systems with no quenched disorder, the helimagnon contributions to the specific heat coefficient is shown to have a linear temperature dependence, while the quasi-particle inelastic scattering rate is anisotropic in momentum space and depends on the electronic dispersion relation. For cubic lattices the generic temperature dependence is given by a non-Fermi-liquid T^(3/2) behavior. The contribution to the temperature dependence of the resistivity is shown to be T^(5/2) in a Boltzmann approximation. The helimagnon thus leads to nonanalytic corrections to Fermi-liquid behavior. Implications for experiments, and for transport theories beyond the Boltzmann level, are discussed.Comment: 15 pp., 5 figs, includes Erratum to PRB versio