344 research outputs found
Energy-sensitive imaging detector applied to the dissociative recombination of D2H+
We report on an energy-sensitive imaging detector for studying the
fragmentation of polyatomic molecules in the dissociative recombination of fast
molecular ions with electrons. The system is based on a large area (10 cm x 10
cm) position-sensitive, double-sided Si-strip detector with 128 horizontal and
128 vertical strips, whose pulse height information is read out individually.
The setup allows to uniquely identify fragment masses and is thus capable of
measuring branching ratios between different fragmentation channels, kinetic
energy releases, as well as breakup geometries, as a function of the relative
ion-electron energy. The properties of the detection system, which has been
installed at the TSR storage ring facility of the Max-Planck Institute for
Nuclear Physics in Heidelberg, is illustrated by an investigation of the
dissociative recombination of the deuterated triatomic hydrogen cation D2H+. A
huge isotope effect is observed when comparing the relative branching ratio
between the D2+H and the HD+D channel; the ratio 2B(D2+H)/B(HD+D), which is
measured to be 1.27 +/- 0.05 at relative electron-ion energies around 0 eV, is
found to increase to 3.7 +/- 0.5 at ~5 eV.Comment: 11 pages, 12 figures, submitted to Physical Review
Cryogenic micro-calorimeters for mass spectrometric identification of neutral molecules and molecular fragments
We have systematically investigated the energy resolution of a magnetic
micro-calorimeter (MMC) for atomic and molecular projectiles at impact energies
ranging from to 150 keV. For atoms we obtained absolute energy
resolutions down to eV and relative energy resolutions
down to . We also studied in detail the MMC
energy-response function to molecular projectiles of up to mass 56 u. We have
demonstrated the capability of identifying neutral fragmentation products of
these molecules by calorimetric mass spectrometry. We have modeled the MMC
energy-response function for molecular projectiles and conclude that
backscattering is the dominant source of the energy spread at the impact
energies investigated. We have successfully demonstrated the use of a detector
absorber coating to suppress such spreads. We briefly outline the use of MMC
detectors in experiments on gas-phase collision reactions with neutral
products. Our findings are of general interest for mass spectrometric
techniques, particularly for those desiring to make neutral-particle mass
measurements
Dissociative recombination measurements of HCl+ using an ion storage ring
We have measured dissociative recombination of HCl+ with electrons using a
merged beams configuration at the heavy-ion storage ring TSR located at the Max
Planck Institute for Nuclear Physics in Heidelberg, Germany. We present the
measured absolute merged beams recombination rate coefficient for collision
energies from 0 to 4.5 eV. We have also developed a new method for deriving the
cross section from the measurements. Our approach does not suffer from
approximations made by previously used methods. The cross section was
transformed to a plasma rate coefficient for the electron temperature range
from T=10 to 5000 K. We show that the previously used HCl+ DR data
underestimate the plasma rate coefficient by a factor of 1.5 at T=10 K and
overestimate it by a factor of 3.0 at T=300 K. We also find that the new data
may partly explain existing discrepancies between observed abundances of
chlorine-bearing molecules and their astrochemical models.Comment: Accepted for publication in ApJ (July 7, 2013
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Anisotropic fragmentation in low-energy dissociative recombination
On a dense energy grid reaching up to 75 meV electron collision energy the
fragmentation angle and the kinetic energy release of neutral dissociative
recombination fragments have been studied in a twin merged beam experiment. The
anisotropy described by Legendre polynomials and the extracted rotational state
contributions were found to vary on a likewise narrow energy scale as the
rotationally averaged rate coefficient. For the first time angular dependences
higher than 2 order could be deduced. Moreover, a slight anisotropy at
zero collision energy was observed which is caused by the flattened velocity
distribution of the electron beam.Comment: 8 pages, 4 figures; The Article will be published in the proceedings
of DR 2007, a symposium on Dissociative Recombination held in Ameland, The
Netherlands (18.-23. July 2008); Reference 19 has been published meanwhile in
S. Novotny, PRL 100, 193201 (2008
"Safe" Coulomb Excitation of 30Mg
We report on the first radioactive beam experiment performed at the recently
commissioned REX-ISOLDE facility at CERN in conjunction with the highly
efficient gamma spectrometer MINIBALL. Using 30Mg ions accelerated to an energy
of 2.25 MeV/u together with a thin nat-Ni target, Coulomb excitation of the
first excited 2+ states of the projectile and target nuclei well below the
Coulomb barrier was observed. From the measured relative de-excitation gamma
ray yields the B(E2; 0+ -> 2+) value of 30Mg was determined to be 241(31)
e2fm4. Our result is lower than values obtained at projectile fragmentation
facilities using the intermediate-energy Coulomb excitation method, and
confirms the theoretical conjecture that the neutron-rich magnesium isotope
30Mg lies still outside the ``island of inversion''
Radiative rotational lifetimes and state-resolved relative detachment cross sections from photodetachment thermometry of molecular anions in a cryogenic storage ring
Photodetachment thermometry on a beam of OH in a cryogenic storage ring
cooled to below 10 K is carried out using two-dimensional, frequency and time
dependent photodetachment spectroscopy over 20 minutes of ion storage. In
equilibrium with the low-level blackbody field, we find an effective radiative
temperature near 15 K with about 90% of all ions in the rotational ground
state. We measure the J = 1 natural lifetime (about 193 s) and determine the
OH rotational transition dipole moment with 1.5% uncertainty. We also
measure rotationally dependent relative near-threshold photodetachment cross
sections for photodetachment thermometry.Comment: Manuscript LaTeX with 5 pages, 3 figures, and 1 table plus LaTeX
supplement with 12 pages, 3 figures and 3 tables. This article has been
accepted by Physical Review Letter
First Results on In-Beam gamma Spectroscopy of Neutron-Rich Na and Mg Isotopes at REX-ISOLDE
After the successful commissioning of the radioactive beam experiment at
ISOLDE (REX-ISOLDE) - an accelerator for exotic nuclei produced by ISOLDE -
first physics experiments using these beams were performed. Initial experiments
focused on the region of deformation in the vicinity of the neutron-rich Na and
Mg isotopes. Preliminary results show the high potential and physics
opportunities offered by the exotic isotope accelerator REX in conjunction with
the modern Germanium gamma spectrometer MINIBALL.Comment: 7 pages, RNB6 conference contributio
Coulomb excitation of Ni at safe energies
The value in Ni has been measured using Coulomb
excitation at safe energies. The Ni radioactive beam was
post-accelerated at the ISOLDE facility (CERN) to 2.9 MeV/u. The emitted
rays were detected by the MINIBALL detector array. A kinematic
particle reconstruction was performed in order to increase the measured c.m.
angular range of the excitation cross section. The obtained value of
2.8 10 efm is in good agreement with the value
measured at intermediate energy Coulomb excitation, confirming the low
transition probability.Comment: 4 pages, 5 figure
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