18,664 research outputs found
Optical signatures of quantum delocalization over extended domains in photosynthetic membranes
The prospect of coherent dynamics and excitonic delocalization across several
light-harvesting structures in photosynthetic membranes is of considerable
interest, but challenging to explore experimentally. Here we demonstrate
theoretically that the excitonic delocalization across extended domains
involving several light-harvesting complexes can lead to unambiguous signatures
in the optical response, specifically, linear absorption spectra. We
characterize, under experimentally established conditions of molecular assembly
and protein-induced inhomogeneities, the optical absorption in these arrays
from polarized and unpolarized excitation, and demonstrate that it can be used
as a diagnostic tool to determine the coherent coupling among iso-energetic
light-harvesting structures. The knowledge of these couplings would then
provide further insight into the dynamical properties of transfer, such as
facilitating the accurate determination of F\"orster rates.Comment: 4 figures and Supplementary information with 7 figures. To appear in
Journal of physical chemistry A, 201
Feedback in a cavity QED system for control of quantum beats
Conditional measurements on the undriven mode of a two-mode cavity QED system
prepare a coherent superposition of ground states which generate quantum beats.
The continuous system drive induces decoherence through the phase interruptions
from Rayleigh scattering, which manifests as a decrease of the beat amplitude
and an increase of the frequency of oscillation. We report recent experiments
that implement a simple feedback mechanism to protect the quantum beat. We
continuously drive the system until a photon is detected, heralding the
presence of a coherent superposition. We then turn off the drive and let the
superposition evolve in the dark, protecting it against decoherence. At a later
time we reinstate the drive to measure the amplitude, phase, and frequency of
the beats. The amplitude can increase by more than fifty percent, while the
frequency is unchanged by the feedback.Comment: 13 pages, 5 figures, ICAP 2012 23rd International Conference on
Atomic Physic
Relativistic spherical plasma waves
Tightly focused laser pulses as they diverge or converge in underdense plasma
can generate wake waves, having local structures that are spherical waves. Here
we report on theoretical study of relativistic spherical wake waves and their
properties, including wave breaking. These waves may be suitable as particle
injectors or as flying mirrors that both reflect and focus radiation, enabling
unique X-ray sources and nonlinear QED phenomena.Comment: 6 pages; 4 figure
Appearance of the Single Gyroid Network Phase in Nuclear Pasta Matter
Nuclear matter under the conditions of a supernova explosion unfolds into a
rich variety of spatially structured phases, called nuclear pasta. We
investigate the role of periodic network-like structures with negatively curved
interfaces in nuclear pasta structures, by static and dynamic Hartree-Fock
simulations in periodic lattices. As the most prominent result, we identify for
the first time the {\it single gyroid} network structure of cubic chiral
symmetry, a well known configuration in nanostructured soft-matter
systems, both as a dynamical state and as a cooled static solution. Single
gyroid structures form spontaneously in the course of the dynamical
simulations. Most of them are isomeric states. The very small energy
differences to the ground state indicate its relevance for structures in
nuclear pasta.Comment: 7 pages, 4 figure
Structure of steps on As-passivated Si(111): Ab initio calculations and scanning tunneling microscopy
The structures of terrace steps on As-covered Si(111) are examined using ab initio calculations. In scanning tunneling microscope (STM) images, two orientations of steps are found to terminate As-covered Si islands after annealing: [11 (2) over bar] and [(11) over bar2]. Total energy calculations and simulations of STM images yield detailed information on the atomic structures of the steps: In the lowest-energy configuration for both orientations, surplus As atoms replace any exposed Si atoms at the steps. The As atoms rearrange to establish a threefold coordination. For [11 (2) over bar] steps the atom positions of the relaxed configuration are very close to the ideal bulk positions, but for [(11) over bar2] steps the terminating As atoms form dimers in front of the steps. The different atomic structures of the two step orientations clearly show up in the simulated STM images for negative bias (occupied states imaged), the STM images for positive bias (unoccupied states) are much less distinctive. All features of existing experimental positive-bias STM images can be explained by an analysis of the electronic local density of states. With the calculated step energies we construct a phase diagram for the equilibrium shape of As-covered islands. In the accessible range of As chemical potentials between As bulk and As-4 molecules, we expect either triangular islands terminated by [11 (2) over bar] steps or hexagons with long edges of [11 (2) over bar] orientation and short ones with [(11) over bar2] orientation
Speciation in the baboon and its relation to gamma-chain heterogeneity and to the response to induction of HbF by 5-azacytidine
In the baboon (Papio species), the two nonallelic gamma-genes produce gamma-chains that differ at a minimum at residue 75, where isoleucine (I gamma-chain) or valine (V gamma) may be present. This situation obtains in baboons that are sometimes designated as Papio anubis, Papio hamadryas, and Papio papio. However, in Papio cynocephalus, although the I gamma-chains are identical with those in the above mentioned types, the V gamma-chains have the substitutions ala----gly at residue 9 and ala----val at residue 23. The V gamma-chains of P. cynocephalus are called V gamma C to distinguish them from the V gamma A-chains of P. anubis, etc. A single cynocephalus animal has been found to have only normal I gamma-chains and I gamma C-chains (that is, glycine in residue 9, valine in 23, and isoleucine in 75). When HbF is produced in response to stress with 5-azacytidine, P. anubis baboons respond with greater production than do P. cynocephalus, and hybrids fall between. Minimal data on P. hamadryas and P. papio suggest an even lower response than P. cynocephalus. As HbF increases under stress, the ratio of I gamma to V gamma-chains changes from the value in the adult or juvenile baboon toward the ratio in the newborn baboon. However, it does not attain the newborn value. The V gamma A and V gamma C-genes respond differently to stress. In hybrids, the production of V gamma A- chains exceeds that of V gamma C-chains. A controlling factor in cis apparently is present and may be responsible for the species-related extent of total HbF production. It may be concluded that the more primitive the cell in the erythroid maturation series that has been subjected to 5-azacytidine, the more active is the I gamma-gene
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