Scaling of the microwave magneto-impedance in Tl2_2Ba2_2CaCu2_2O8+δ_{8+\delta} thin films

We present measurements of the magnetic field-induced microwave complex resistivity changes at 47 GHz in Tl$_2$Ba$_2$CaCu$_2$O$_{8+\delta}$ (TBCCO) thin films, in the ranges 58 K$<T<T_{c}$ and 0$<\mu_{0}H<$0.8 T. The large imaginary part $\Delta\rho_{2}(H)$ points to strong elastic response, but the data are not easily reconciled with a rigid vortex model. We find that, over a wide range of temperatures, all the pairs of curves $\Delta\rho_{1}(H)$ and $\Delta\rho_{2}(H)$ can be collapsed on a pair of scaling curves $\Delta\rho_{1}[H/H^{*}(T)]$, $\Delta\rho_{2}[H/H^{*}(T)]$, with the same scaling field $H^{*}(T)$. We argue that $H^{*}(T)$ is related to the loss of vortex rigidity due to a vortex transformation.Comment: Two printed pages, Proceedings of M2S (Dresden, 2006), to appear in Physica

Vortex state microwave resistivity in Tl-2212 thin films

We present measurements of the field induced changes in the 47 GHz complex resistivity, $\Delta \tilde \rho(H,T)$, in Tl$_{2}$Ba$_{2}$CaCu$_{2}$O$_{8+x}$ (TBCCO) thin films with $T_{c}\simeq$ 105 K, prepared on CeO$_{2}$ buffered sapphire substrates. At low fields ($\mu_{0}H<$10 mT) a very small irreversible feature is present, suggesting a little role of intergranular phenomena. Above that level $\Delta \tilde \rho(H,T)$ exhibits a superlinear dependence with the field, as opposed to the expected (at high frequencies) quasilinear behaviour. We observe a crossover between predominantly imaginary to predominantly real (dissipative) response with increasing temperature and/or field. In addition, we find the clear scaling property $\Delta \tilde \rho(H,T)=\Delta \tilde \rho[H/H^{*}(T)]$, where the scaling field $H^{*}(T)$ maps closely the melting field measured in single crystals. We discuss our microwave results in terms of loss of flux lines rigidity.Comment: 8 pages, 3 figures, proceedings of 9th HTSHFF, accepted for publication on J. Supercon

Microwave vortex dynamics in Tl-2212 thin films

We present measurements of the effective surface impedance changes due to a static magnetic field, \Delta Z(H,T)=\Delta R(H,T)+\rmi \Delta X(H,T), in a Tl-2212 thin film with $T_c>$ 103 K, grown on a CeO$_2$ buffered sapphire substrate. Measurements were performed through a dielectric resonator operating at 47.7 GHz, for temperatures 60 K$\leq T<T_c$ and magnetic fields $\leq0.8$ T. We observe exceptionally large field induced variations and pronounced super-linear field dependencies in both $\Delta R(H)$ and $\Delta X(H)$ with $\Delta X(H)>\Delta R(H)$ in almost the whole $(H,T)$ range explored. A careful analysis of the data allows for an interpretation of these results as dominated by vortex dynamics. In the intermediate-high field range we extract the main vortex parameters by resorting to standard high frequency model and by taking into proper account the creep contribution. The pinning constant shows a marked decrease with the field which can be interpreted in terms of flux lines softening associated to an incipient layer decoupling. Small vortex viscosity, by an order of magnitude lower than in Y-123 are found. Some speculations about these findings are provided.Comment: pdfTeX, 4 pages, 3 figures, VORTEX 2007 proceedings, to appear in Physica

Spin-Wave and Electromagnon Dispersions in Multiferroic MnWO4 as Observed by Neutron Spectroscopy: Isotropic Heisenberg Exchange versus Anisotropic Dzyaloshinskii-Moriya Interaction

High resolution inelastic neutron scattering reveals that the elementary magnetic excitations in multiferroic MnWO4 consist of low energy dispersive electromagnons in addition to the well-known spin-wave excitations. The latter can well be modeled by a Heisenberg Hamiltonian with magnetic exchange coupling extending to the 12th nearest neighbor. They exhibit a spin-wave gap of 0.61(1) meV. Two electromagnon branches appear at lower energies of 0.07(1) meV and 0.45(1) meV at the zone center. They reflect the dynamic magnetoelectric coupling and persist in both, the collinear magnetic and paraelectric AF1 phase, and the spin spiral ferroelectric AF2 phase. These excitations are associated with the Dzyaloshinskii-Moriya exchange interaction, which is significant due to the rather large spin-orbit coupling.Comment: 8 pages, 6 figures, accepted for publication in Physical Review

Consequences of critical interchain couplings and anisotropy on a Haldane chain

Effects of interchain couplings and anisotropy on a Haldane chain have been investigated by single crystal inelastic neutron scattering and density functional theory (DFT) calculations on the model compound SrNi$_2$V$_2$O$_8$. Significant effects on low energy excitation spectra are found where the Haldane gap ($\Delta_0 \approx 0.41J$; where $J$ is the intrachain exchange interaction) is replaced by three energy minima at different antiferromagnetic zone centers due to the complex interchain couplings. Further, the triplet states are split into two branches by single-ion anisotropy. Quantitative information on the intrachain and interchain interactions as well as on the single-ion anisotropy are obtained from the analyses of the neutron scattering spectra by the random phase approximation (RPA) method. The presence of multiple competing interchain interactions is found from the analysis of the experimental spectra and is also confirmed by the DFT calculations. The interchain interactions are two orders of magnitude weaker than the nearest-neighbour intrachain interaction $J$ = 8.7~meV. The DFT calculations reveal that the dominant intrachain nearest-neighbor interaction occurs via nontrivial extended superexchange pathways Ni--O--V--O--Ni involving the empty $d$ orbital of V ions. The present single crystal study also allows us to correctly position SrNi$_2$V$_2$O$_8$ in the theoretical $D$-$J_{\perp}$ phase diagram [T. Sakai and M. Takahashi, Phys. Rev. B 42, 4537 (1990)] showing where it lies within the spin-liquid phase.Comment: 12 pages, 12 figures, 3 tables PRB (accepted). in Phys. Rev. B (2015

Revisiting the ground state of CoAl2_2O4_4: comparison to the conventional antiferromagnet MnAl2_2O4_4

The A-site spinel material, CoAl2O4, is a physical realization of the frustrated diamond-lattice antiferromagnet, a model in which is predicted to contain unique incommensurate or `spin-spiral liquid' ground states. Our previous single-crystal neutron scattering study instead classified it as a `kinetically-inhibited' antiferromagnet, where the long ranged correlations of a collinear Neel ground state are blocked by the freezing of domain wall motion below a first-order phase transition at T* = 6.5 K. The current paper expands on our original results in several important ways. New elastic and inelastic neutron measurements are presented that show our initial conclusions are affected by neither the sample measured nor the instrument resolution, while measurements to temperatures as low as T = 250 mK limit the possible role being played by low-lying thermal excitations. Polarized diffuse neutron measurements confirm reports of short-range antiferromagnetic correlations and diffuse streaks of scattering, but major diffuse features are explained as signatures of overlapping critical correlations between neighboring Brillouin zones. Finally, and critically, this paper presents detailed elastic and inelastic measurements of magnetic correlations in a single-crystal of MnAl2O4, which acts as an unfrustrated analogue to CoAl2O4. The unfrustrated material is shown to have a classical continuous phase transition to Neel order at T_N = 39 K, with collective spinwave excitations and Lorentzian-like critical correlations which diverge at the transition. Direct comparison between the two compounds indicates that CoAl2O4 is unique, not in the nature of high-temperature diffuse correlations, but rather in the nature of the frozen state below T*. The higher level of cation inversion in the MnAl2O4 sample indicates that this novel behavior is primarily an effect of greater next-nearest-neighbor exchange.Comment: 13 pages, 8 figures, acccepted for publication in Physical Review

Role of commensurate and incommensurate low-energy excitations in the paramagnetic to hidden-order transition of URu2_2Si2_2

We report low-energy inelastic neutron scattering data of the paramagnetic (PM) to hidden-order (HO) phase transition at $T_0=17.5\,{\rm K}$ in URu$_2$Si$_2$. While confirming previous results for the HO and PM phases, our data reveal a pronounced wavevector dependence of low-energy excitations across the phase transition. To analyze the energy scans we employ a damped harmonic oscillator model containing a fit parameter $1/\Gamma$ which is expected to diverge at a second-order phase transition. Counter to expectations the excitations at $\vec{Q}_1=(1.44,0,0)$ show an abrupt step-like suppression of $1/\Gamma$ below $T_0$, whereas excitations at $\vec{Q}_0=(1,0,0)$, associated with large-moment antiferromagnetism (LMAF) under pressure, show an enhancement and a pronounced peak of $1/\Gamma$ at $T_0$. Therefore, at the critical HO temperature $T_0$, LMAF fluctuations become nearly critical as well. This is the behavior expected of a super-vector order parameter with nearly degenerate components for the HO and LMAF leading to nearly isotropic fluctuations in the combined order-parameter space.Comment: 6 pages; v3 accepted journal version; minor modifications compared to v

Normal-State Spin Dynamics and Temperature-Dependent Spin Resonance Energy in an Optimally Doped Iron Arsenide Superconductor

The proximity of superconductivity and antiferromagnetism in the phase diagram of iron arsenides, the apparently weak electron-phonon coupling and the "resonance peak" in the superconducting spin excitation spectrum have fostered the hypothesis of magnetically mediated Cooper pairing. However, since most theories of superconductivity are based on a pairing boson of sufficient spectral weight in the normal state, detailed knowledge of the spin excitation spectrum above the superconducting transition temperature Tc is required to assess the viability of this hypothesis. Using inelastic neutron scattering we have studied the spin excitations in optimally doped BaFe1.85Co0.15As2 (Tc = 25 K) over a wide range of temperatures and energies. We present the results in absolute units and find that the normal state spectrum carries a weight comparable to underdoped cuprates. In contrast to cuprates, however, the spectrum agrees well with predictions of the theory of nearly antiferromagnetic metals, without complications arising from a pseudogap or competing incommensurate spin-modulated phases. We also show that the temperature evolution of the resonance energy follows the superconducting energy gap, as expected from conventional Fermi-liquid approaches. Our observations point to a surprisingly simple theoretical description of the spin dynamics in the iron arsenides and provide a solid foundation for models of magnetically mediated superconductivity.Comment: 8 pages, 4 figures, and an animatio