Single-photon single ionization of W+^{+} ions: experiment and theory

Experimental and theoretical results are reported for photoionization of Ta-like (W$^{+}$) tungsten ions. Absolute cross sections were measured in the energy range 16 to 245 eV employing the photon-ion merged-beam setup at the Advanced Light Source in Berkeley. Detailed photon-energy scans at 100 meV bandwidth were performed in the 16 to 108 eV range. In addition, the cross section was scanned at 50 meV resolution in regions where fine resonance structures could be observed. Theoretical results were obtained from a Dirac-Coulomb R-matrix approach. Photoionization cross section calculations were performed for singly ionized atomic tungsten ions in their $5s^2 5p^6 5d^4({^5}D)6s \; {^6}{\rm D}_{J}$, $J$=1/2, ground level and the associated excited metastable levels with $J$=3/2, 5/2, 7/2 and 9/2. Since the ion beams used in the experiments must be expected to contain long-lived excited states also from excited configurations, additional cross-section calculations were performed for the second-lowest term, 5d^5 \; ^6{\rm S}_{J}, $J$=5/2, and for the $^4$F term, 5d^3 6s^2 \; ^4{\rm F}_{J}, with $J$ = 3/2, 5/2, 7/2 and 9/2. Given the complexity of the electronic structure of W$^+$ the calculations reproduce the main features of the experimental cross section quite well.Comment: 23 pages, 7 figures, 1 table: Accepted for publication in J. Phys. B: At. Mol. & Opt. Phy

Near--K-edge double and triple detachment of the F- negative ion: observation of direct two-electron ejection by a single photon

Double and triple detachment of the F-(1s2 2s2 2p6) negative ion by a single photon have been investigated in the photon energy range 660 to 1000 eV. The experimental data provide unambiguous evidence for the dominant role of direct photo-double-detachment with a subsequent single-Auger process in the reaction channel leading to F2+ product ions. Absolute cross sections were determined for the direct removal of a (1s+2p) pair of electrons from F- by the absorption of a single photon

Interference effects in the photorecombination of argonlike Sc3+ ions: Storage-ring experiment and theory

Absolute total electron-ion recombination rate coefficients of argonlike Sc3+(3s2 3p6) ions have been measured for relative energies between electrons and ions ranging from 0 to 45 eV. This energy range comprises all dielectronic recombination resonances attached to 3p -> 3d and 3p -> 4s excitations. A broad resonance with an experimental width of 0.89 +- 0.07 eV due to the 3p5 3d2 2F intermediate state is found at 12.31 +- 0.03 eV with a small experimental evidence for an asymmetric line shape. From R-Matrix and perturbative calculations we infer that the asymmetric line shape may not only be due to quantum mechanical interference between direct and resonant recombination channels as predicted by Gorczyca et al. [Phys. Rev. A 56, 4742 (1997)], but may partly also be due to the interaction with an adjacent overlapping DR resonance of the same symmetry. The overall agreement between theory and experiment is poor. Differences between our experimental and our theoretical resonance positions are as large as 1.4 eV. This illustrates the difficulty to accurately describe the structure of an atomic system with an open 3d-shell with state-of-the-art theoretical methods. Furthermore, we find that a relativistic theoretical treatment of the system under study is mandatory since the existence of experimentally observed strong 3p5 3d2 2D and 3p5 3d 4s 2D resonances can only be explained when calculations beyond LS-coupling are carried out.Comment: 11 pages, 7 figures, 3 tables, Phys. Rev. A (in print), see also: http://www.strz.uni-giessen.de/~k

The use of online support by people with intellectual disabilities living independently during COVID‐19

Background During the COVID-19 outbreak, service providers in the Netherlands had to switch towards providing remote support for people with intellectual disabilities living independently. This study aims to provide insight into the use of online support during the outbreak. Methods We analysed quantitative data on planned and unplanned contacts between the online support service DigiContact and its service users. Results The results indicate that the COVID-19 outbreak and the related containment measures had a strong impact on online support use, specifically on the unplanned use of online support. Conclusion Offering online support as a standard component of services for independently living people with intellectual disability enables service providers to be flexible and responsive towards fluctuations in both support needs and onsite support availability during a social crisis such as COVID-19

Double-K-vacancy states in electron-impact single ionization of metastable two-electron N5+(1s2s 3S1) ions

The role of hollow states intermediately produced in electron-impact ionization of metastable He-like N5+(1s2s3S1) ions has been investigated in detail. A crossed-beam setup and suitable experimental techniques were employed for the measurement of accurate absolute cross sections and precise energy-scan data. Fine structures arising from K-shell excitations and associated resonances have been observed for this two-electron ion with less than ±0.5 eV uncertainty on the energy scale. Fine details, such as interference of the reaction pathways of direct ionization and excitation with capture of the incident electron followed by double-Auger decay, could be revealed. Ab initio calculations based on the convergent close coupling (CCC) approach are in good agreement with the experiment

Absolute rate coefficients for photorecombination and electron-impact ionization of magnesium-like iron ions from measurements at a heavy-ion storage ring

Rate coefficients for photorecombination (PR) and cross sections for electron-impact ionization (EII) of Fe$^{14+}$ forming Fe$^{13+}$ and Fe$^{15+}$, respectively, have been measured by employing the electron-ion merged-beams technique at a heavy-ion storage ring. Rate coefficients for PR and EII of Fe$^{14+}$ ions in a plasma are derived from the experimental measurements. Simple parametrizations of the experimentally derived plasma rate coefficients are provided for use in the modeling of photoionized and collisionally ionized plasmas. In the temperature ranges where Fe$^{14+}$ is expected to form in such plasmas the latest theoretical rate coefficients of Altun et al. [Astron. Astrophys. 474, 1051 (2007)] for PR and of Dere [Astron. Astrophys. 466, 771 (2007)] for EII agree with the experimental results to within the experimental uncertainties. Common features in the PR and EII resonance structures are identified and discussed.Comment: 12 pages, 6 figures, 3 tables, submitted for publication to Physical Review

Absolute rate coefficients for photorecombination of berylliumlike and boronlike silicon ions

We report measured rate coefficients for electron-ion recombination for Si10+ forming Si9+ and for Si9+ forming Si8+, respectively. The measurements were performed using the electron-ion merged-beams technique at a heavy-ion storage ring. Electron-ion collision energies ranged from 0 to 50 eV for Si9+ and from 0 to 2000 eV for Si10+, thus, extending previous measurements for Si10+ [Orban et al. 2010, Astrophys. J. 721, 1603] to much higher energies. Experimentally derived rate coefficients for the recombination of Si9+ and Si10+ ions in a plasma are presented along with simple parameterizations. These rate coefficients are useful for the modeling of the charge balance of silicon in photoionized plasmas (Si9+ and Si10+) and in collisionally ionized plasmas (Si10+ only). In the corresponding temperature ranges, the experimentally derived rate coefficients agree with the latest corresponding theoretical results within the experimental uncertainties.Comment: 17 pages, 7 figures, 3 tables, 66 references, submitted to the J. Phys. B special issue on atomic and molecular data for astrophysicist