308 research outputs found
Irregular AC losses with long time constants in large cable-in-conduit conductors
科研費報告書収録論文(課題番号:15360491/研究代表者:濱島高太郎/大型超伝導コイルに発生する不規則な交流損失の原因究明)44
Electronic superlattice revealed by resonant scattering from random impurities in Sr3Ru2O7
Resonant elastic x-ray scattering (REXS) is an exquisite element-sensitive
tool for the study of subtle charge, orbital, and spin superlattice orders
driven by the valence electrons, which therefore escape detection in
conventional x-ray diffraction (XRD). Although the power of REXS has been
demonstrated by numerous studies of complex oxides performed in the soft x-ray
regime, the cross section and photon wavelength of the material-specific
elemental absorption edges ultimately set the limit to the smallest
superlattice amplitude and periodicity one can probe. Here we show -- with
simulations and REXS on Mn-substituted SrRuO -- that these
limitations can be overcome by performing resonant scattering experiments at
the absorption edge of a suitably-chosen, dilute impurity. This establishes
that -- in analogy with impurity-based methods used in electron-spin-resonance,
nuclear-magnetic resonance, and M\"ossbauer spectroscopy -- randomly
distributed impurities can serve as a non-invasive, but now momentum-dependent
probe, greatly extending the applicability of resonant x-ray scattering
techniques
Crystal-field level inversion in lightly Mn-doped Sr3Ru2O7
Sr3(Ru1-xMnx)2O7, in which 4d-Ru is substituted by the more localized 3d-Mn,
is studied by x-ray dichroism and spin-resolved density functional theory. We
find that Mn impurities do not exhibit the same 4+ valence of Ru, but act as 3+
acceptors; the extra eg electron occupies the in-plane 3dx2-y2 orbital instead
of the expected out-of-plane 3d3z2-r2. We propose that the 3d-4d interplay, via
the ligand oxygen orbitals, is responsible for this crystal-field level
inversion and the material's transition to an antiferromagnetic, possibly
orbitally-ordered, low-temperature state.Comment: A high-resolution version can be found at
http://www.physics.ubc.ca/~quantmat/ARPES/PUBLICATIONS/Articles/MnSr3Ru2O7_XAS.pd
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