547 research outputs found
Theoretical spin-wave dispersions in the antiferromagnetic phase AF1 of MnWO based on the polar atomistic model in P2
The spin wave dispersions of the low temperature antiferromagnetic phase
(AF1) MnWO have been numerically calculated based on the recently reported
non-collinear spin configuration with two different canting angles. A
Heisenberg model with competing magnetic exchange couplings and single-ion
anisotropy terms could properly describe the spin wave excitations, including
the newly observed low-lying energy excitation mode =0.45 meV
appearing at the magnetic zone centre. The spin wave dispersion and intensities
are highly sensitive to two differently aligned spin-canting sublattices in the
AF1 model. Thus this study reinsures the otherwise hardly provable hidden polar
character in MnWO.Comment: 7 pages, 5 figure
Spin reorientation in Na-doped BaFeAs studied by neutron diffraction
We have studied the magnetic ordering in Na doped BaFeAs by
unpolarized and polarized neutron diffraction using single crystals. Unlike
previously studied FeAs-based compounds that magnetically order,
BaNaFeAs exhibits two successive magnetic transitions: For
x=0.35 upon cooling magnetic order occurs at 70\ K with in-plane magnetic
moments being arranged as in pure or Ni, Co and K-doped BaFeAs samples.
At a temperature of 46\ K a second phase transition occurs, which the
single-crystal neutron diffraction experiments can unambiguously identify as a
spin reorientation. At low temperatures, the ordered magnetic moments in
BaNaFeAs point along the direction. Magnetic
correlations in these materials cannot be considered as Ising like, and
spin-orbit coupling must be included in a quantitative theory.Comment: 5 pages, 4 figure
Evidence of a bond-nematic phase in LiCuVO4
Polarized and unpolarized neutron scattering experiments on the frustrated
ferromagnetic spin-1/2 chain LiCuVO4 show that the phase transition at HQ of 8
Tesla is driven by quadrupolar fluctuations and that dipolar correlations are
short-range with moments parallel to the applied magnetic field in the
high-field phase. Heat-capacity measurements evidence a phase transition into
this high-field phase, with an anomaly clearly different from that at low
magnetic fields. Our experimental data are consistent with a picture where the
ground state above HQ has a next-nearest neighbour bond-nematic order along the
chains with a fluid-like coherence between weakly coupled chains.Comment: 5 pages, 4 figures. To appear in Phys. Rev. Let
Magnetic-field and doping dependence of low-energy spin fluctuations in the antiferroquadrupolar compound Ce(1-x)La(x)B(6)
CeB(6) is a model compound exhibiting antiferroquadrupolar (AFQ) order, its
magnetic properties being typically interpreted within localized models. More
recently, the observation of strong and sharp magnetic exciton modes forming in
its antiferromagnetic (AFM) state at both ferromagnetic and AFQ wave vectors
suggested a significant contribution of itinerant electrons to the spin
dynamics. Here we investigate the evolution of the AFQ excitation upon the
application of an external magnetic field and the substitution of Ce with
non-magnetic La, both parameters known to suppress the AFM phase. We find that
the exciton energy decreases proportionally to T_N upon doping. In field, its
intensity is suppressed, while its energy remains constant. Its disappearance
above the critical field of the AFM phase is preceded by the formation of two
modes, whose energies grow linearly with magnetic field upon entering the AFQ
phase. These findings suggest a crossover from itinerant to localized spin
dynamics between the two phases, the coupling to heavy-fermion quasiparticles
being crucial for a comprehensive description of the magnon spectrum.Comment: Extended version with a longer introduction and an additional figure.
6 pages and 5 figure
Consequences of critical interchain couplings and anisotropy on a Haldane chain
Effects of interchain couplings and anisotropy on a Haldane chain have been
investigated by single crystal inelastic neutron scattering and density
functional theory (DFT) calculations on the model compound SrNiVO.
Significant effects on low energy excitation spectra are found where the
Haldane gap (; where is the intrachain exchange
interaction) is replaced by three energy minima at different antiferromagnetic
zone centers due to the complex interchain couplings. Further, the triplet
states are split into two branches by single-ion anisotropy. Quantitative
information on the intrachain and interchain interactions as well as on the
single-ion anisotropy are obtained from the analyses of the neutron scattering
spectra by the random phase approximation (RPA) method. The presence of
multiple competing interchain interactions is found from the analysis of the
experimental spectra and is also confirmed by the DFT calculations. The
interchain interactions are two orders of magnitude weaker than the
nearest-neighbour intrachain interaction = 8.7~meV. The DFT calculations
reveal that the dominant intrachain nearest-neighbor interaction occurs via
nontrivial extended superexchange pathways Ni--O--V--O--Ni involving the empty
orbital of V ions. The present single crystal study also allows us to
correctly position SrNiVO in the theoretical - phase
diagram [T. Sakai and M. Takahashi, Phys. Rev. B 42, 4537 (1990)] showing where
it lies within the spin-liquid phase.Comment: 12 pages, 12 figures, 3 tables PRB (accepted). in Phys. Rev. B (2015
Improved treatment of the molecular final-states uncertainties for the KATRIN neutrino-mass measurement
The KArlsruhe TRItium Neutrino experiment (KATRIN) aims to determine the
effective mass of the electron antineutrino via a high-precision measurement of
the tritium beta-decay spectrum in its end-point region. The target
neutrino-mass sensitivity of 0.2 eV / c^2 at 90% C.L. can only be achieved in
the case of high statistics and a good control of the systematic uncertainties.
One key systematic effect originates from the calculation of the molecular
final states of T_2 beta decay. In the first neutrino-mass analyses of KATRIN
the contribution of the uncertainty of the molecular final-states distribution
(FSD) was estimated via a conservative phenomenological approach to be 0.02
eV^2 / c^4. In this paper a new procedure is presented for estimating the
FSD-related uncertainties by considering the details of the final-states
calculation, i.e. the uncertainties of constants, parameters, and functions
used in the calculation as well as its convergence itself as a function of the
basis-set size used in expanding the molecular wave functions. The calculated
uncertainties are directly propagated into the experimental observable, the
squared neutrino mass m_nu^2. With the new procedure the FSD-related
uncertainty is constrained to 0.0013 eV^2 / c^4, for the experimental
conditions of the first KATRIN measurement campaign
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Electric current-driven spectral tunability of surface plasmon polaritons in gold coated tapered fibers
Here we introduce the concept of electrically tuning surface plasmon polaritons using current-driven heat dissipation, allowing controlling plasmonic properties via a straightforward-to-access quantity. The key idea is based on an electrical current flowing through the plasmonic layer, changing plasmon dispersion and phase-matching condition via a temperature-imposed modification of the refractive index of one of the dielectric media involved. This scheme was experimentally demonstrated on the example of an electrically connected plasmonic fiber taper that has sensitivities >50000 nm/RIU. By applying a current, dissipative heat generated inside metal film heats the surrounding liquid, reducing its refractive index correspondingly and thus modifying the phase-matching condition to the fundamental taper mode. We observed spectral shifts of the plasmonic resonance up to 300 nm towards shorter wavelength by an electrical power of ≤ 80 mW, clearly showing that our concept is important for applications that demand precise real-time and external control on plasmonic dispersion and resonance wavelengths
Revisiting the ground state of CoAlO: comparison to the conventional antiferromagnet MnAlO
The A-site spinel material, CoAl2O4, is a physical realization of the
frustrated diamond-lattice antiferromagnet, a model in which is predicted to
contain unique incommensurate or `spin-spiral liquid' ground states. Our
previous single-crystal neutron scattering study instead classified it as a
`kinetically-inhibited' antiferromagnet, where the long ranged correlations of
a collinear Neel ground state are blocked by the freezing of domain wall motion
below a first-order phase transition at T* = 6.5 K. The current paper expands
on our original results in several important ways. New elastic and inelastic
neutron measurements are presented that show our initial conclusions are
affected by neither the sample measured nor the instrument resolution, while
measurements to temperatures as low as T = 250 mK limit the possible role being
played by low-lying thermal excitations. Polarized diffuse neutron measurements
confirm reports of short-range antiferromagnetic correlations and diffuse
streaks of scattering, but major diffuse features are explained as signatures
of overlapping critical correlations between neighboring Brillouin zones.
Finally, and critically, this paper presents detailed elastic and inelastic
measurements of magnetic correlations in a single-crystal of MnAl2O4, which
acts as an unfrustrated analogue to CoAl2O4. The unfrustrated material is shown
to have a classical continuous phase transition to Neel order at T_N = 39 K,
with collective spinwave excitations and Lorentzian-like critical correlations
which diverge at the transition. Direct comparison between the two compounds
indicates that CoAl2O4 is unique, not in the nature of high-temperature diffuse
correlations, but rather in the nature of the frozen state below T*. The higher
level of cation inversion in the MnAl2O4 sample indicates that this novel
behavior is primarily an effect of greater next-nearest-neighbor exchange.Comment: 13 pages, 8 figures, acccepted for publication in Physical Review
Spin-Wave and Electromagnon Dispersions in Multiferroic MnWO4 as Observed by Neutron Spectroscopy: Isotropic Heisenberg Exchange versus Anisotropic Dzyaloshinskii-Moriya Interaction
High resolution inelastic neutron scattering reveals that the elementary
magnetic excitations in multiferroic MnWO4 consist of low energy dispersive
electromagnons in addition to the well-known spin-wave excitations. The latter
can well be modeled by a Heisenberg Hamiltonian with magnetic exchange coupling
extending to the 12th nearest neighbor. They exhibit a spin-wave gap of 0.61(1)
meV. Two electromagnon branches appear at lower energies of 0.07(1) meV and
0.45(1) meV at the zone center. They reflect the dynamic magnetoelectric
coupling and persist in both, the collinear magnetic and paraelectric AF1
phase, and the spin spiral ferroelectric AF2 phase. These excitations are
associated with the Dzyaloshinskii-Moriya exchange interaction, which is
significant due to the rather large spin-orbit coupling.Comment: 8 pages, 6 figures, accepted for publication in Physical Review
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