791 research outputs found
Differential probability for surface and volume electronic excitations in Fe, Pd and Pt
The normalized differential mean free path for volume scattering and the
differential surface excitation probability for medium energy electrons
travelling in Fe, Pd and Pt are extracted from Reflection Electron Energy Loss
Spectra (REELS). This was achieved by means of a recently introduced procedure
in which two REELS spectra taken under different experimental conditions are
simultaneously deconvoluted. In this way, it is possible to obtain the unique
reconstruction for the surface and volume single scattering loss distribution.
The employed method is compared with a procedure that is frequently used for
this purpose [Tougaard and Chorkendorff, Phys. Rev. B 35(1987)6570]. It is
shown, both theoretically and through analysis of model spectra as well as
experimental data that this method does not result in a {\em single} scattering
loss distribution. Rather, it gives a mixture of surface, bulk and mixed
scattering of any order
Properties of a beam splitter entangler with Gaussian input states
An explicit formula is given for the quantity of entanglement in the output
state of a beam splitter, given the squeezed vacuum states input in each mode.Comment: To appear in Phys. Rev.
Bell's inequalities for states with positive partial transpose
We study violations of n particle Bell inequalities (as developed by Mermin
and Klyshko) under the assumption that suitable partial transposes of the
density operator are positive. If all transposes with respect to a partition of
the system into p subsystems are positive, the best upper bound on the
violation is 2^((n-p)/2). In particular, if the partial transposes with respect
to all subsystems are positive, the inequalities are satisfied. This is
supporting evidence for a recent conjecture by Peres that positivity of partial
transposes could be equivalent to existence of local classical models.Comment: 4 pages, REVTe
Chemical inâdepth analysis of (Ca/Sr)F2 coreâshell like nanoparticles by Xâray photoelectron spectroscopy with tunable excitation energy
The fluorolytic solâgel synthesis is applied with the intention to obtain two different types of coreâshell nanoparticles, namely, SrF2âCaF2 and CaF2âSrF2. In two separate fluorination steps for core and shell formation, the corresponding metal lactates are reacted with anhydrous HF in ethylene glycol. Scanning transmission electron microscopy (STEM) and dynamic light scattering (DLS) confirm the formation of particles with mean dimensions between 6.4 and 11.5 nm. The overall chemical composition of the particles during the different reaction steps is monitored by quantitative Al Kα excitation X-ray photoelectron spectroscopy (XPS). Here, the formation of stoichiometric metal fluorides (MF2) is confirmed, both for the core and the final coreâshell particles. Furthermore, an in-depth analysis by synchrotron radiation XPS (SR-XPS) with tunable excitation energy is performed to confirm the coreâshell character of the nanoparticles. Additionally, Ca2p/Sr3d XPS intensity ratio in-depth profiles are simulated using the software Simulation of Electron Spectra for Surface Analysis (SESSA). In principle, coreâshell like particle morphologies are formed but without a sharp interface between calcium and strontium containing phases. Surprisingly, the in-depth chemical distribution of the two types of nanoparticles is equal within the error of the experiment. Both comprise a SrF2-rich core domain and CaF2-rich shell domain with an intermixing zone between them. Consequently, the internal morphology of the final nanoparticles seems to be independent from the synthesis chronology.European Metrology Programme for Innovation and Research (EMPIR)
http://dx.doi.org/10.13039/100014132Peer Reviewe
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Chemical in-depth analysis of (Ca/Sr)F2 coreâshell like nanoparticles by X-ray photoelectron spectroscopy with tunable excitation energy
The fluorolytic solâgel synthesis is applied with the intention to obtain two different types of coreâshell nanoparticles, namely, SrF2âCaF2 and CaF2âSrF2. In two separate fluorination steps for core and shell formation, the corresponding metal lactates are reacted with anhydrous HF in ethylene glycol. Scanning transmission electron microscopy (STEM) and dynamic light scattering (DLS) confirm the formation of particles with mean dimensions between 6.4 and 11.5 nm. The overall chemical composition of the particles during the different reaction steps is monitored by quantitative Al Kα excitation X-ray photoelectron spectroscopy (XPS). Here, the formation of stoichiometric metal fluorides (MF2) is confirmed, both for the core and the final coreâshell particles. Furthermore, an in-depth analysis by synchrotron radiation XPS (SR-XPS) with tunable excitation energy is performed to confirm the coreâshell character of the nanoparticles. Additionally, Ca2p/Sr3d XPS intensity ratio in-depth profiles are simulated using the software Simulation of Electron Spectra for Surface Analysis (SESSA). In principle, coreâshell like particle morphologies are formed but without a sharp interface between calcium and strontium containing phases. Surprisingly, the in-depth chemical distribution of the two types of nanoparticles is equal within the error of the experiment. Both comprise a SrF2-rich core domain and CaF2-rich shell domain with an intermixing zone between them. Consequently, the internal morphology of the final nanoparticles seems to be independent from the synthesis chronology
Separability and entanglement in 2x3xN composite quantum systems
The separability and entanglement of quantum mixed states in \Cb^2 \otimes
\Cb^3 \otimes \Cb^N composite quantum systems are investigated. It is shown
that all quantum states with positive partial transposes and rank
are separable.Comment: Latex, 15 page
MiniBooNE Results and Neutrino Schemes with 2 sterile Neutrinos: Possible Mass Orderings and Observables related to Neutrino Masses
The MiniBooNE and LSND experiments are compatible with each other when two
sterile neutrinos are added to the three active ones. In this case there are
eight possible mass orderings. In two of them both sterile neutrinos are
heavier than the three active ones. In the next two scenarios both sterile
neutrinos are lighter than the three active ones. The remaining four scenarios
have one sterile neutrino heavier and another lighter than the three active
ones. We analyze all scenarios with respect to their predictions for
mass-related observables. These are the sum of neutrino masses as constrained
by cosmological observations, the kinematic mass parameter as measurable in the
KATRIN experiment, and the effective mass governing neutrinoless double beta
decay. It is investigated how these non-oscillation probes can distinguish
between the eight scenarios. Six of the eight possible mass orderings predict
positive signals in the KATRIN and future neutrinoless double beta decay
experiments. We also remark on scenarios with three sterile neutrinos. In
addition we make some comments on the possibility of using decays of high
energy astrophysical neutrinos to discriminate between the mass orderings in
presence of two sterile neutrinos.Comment: 33 pages, 8 figures. Comments added, to appear in JHE
Detecting genuine multipartite continuous-variable entanglement
We derive necessary conditions in terms of the variances of position and
momentum linear combinations for all kinds of separability of a multi-party
multi-mode continuous-variable state. Their violations can be sufficient for
genuine multipartite entanglement, provided the combinations contain both
conjugate variables of all modes. Hence a complete state determination, for
example by detecting the entire correlation matrix of a Gaussian state, is not
needed.Comment: 13 pages, 3 figure
Magnetic and charge structures in itinerant-electron magnets: Coexistence of multiple SDW and CDW
A theory of Kondo lattices is applied to studying possible magnetic and
charge structures of itinerant-electron antiferromagnets. Even helical spin
structures can be stabilized when the nesting of the Fermi surface is not sharp
and the superexchange interaction, which arises from the virtual exchange of
pair excitations across the Mott-Hubbard gap, is mainly responsible for
magnetic instability. Sinusoidal spin structures or spin density waves (SDW)
are only stabilized when the nesting of the Fermi surface is sharp enough and a
novel exchange interaction arising from that of pair excitations of
quasi-particles is mainly responsible for magnetic instability. In particular,
multiple SDW are stabilized when their incommensurate ordering wave-numbers
are multiple; magnetizations of different components
are orthogonal to each other in double and triple SDW when magnetic anisotropy
is weak enough. Unless are commensurate, charge density waves
(CDW) with coexist with SDW with . Because the
quenching of magnetic moments by the Kondo effect depends on local numbers of
electrons, the phase of CDW or electron densities is such that magnetic moments
are large where the quenching is weak. It is proposed that the so called stipe
order in cuprate-oxide high-temperature superconductors must be the coexisting
state of double incommensurate SDW and CDW.Comment: 10 pages, no figure
Soliton Lattices in the Incommensurate Spin-Peierls Phase: Local Distortions and Magnetizations
It is shown that nonadiabatic fluctuations of the soliton lattice in the
spin-Peierls system CuGeO_3 lead to an important reduction of the NMR line
widths. These fluctuations are the zero-point motion of the massless phasonic
excitations. Furthermore, we show that the discrepancy of X-ray and NMR soliton
widths can be understood as the difference between a distortive and a magnetic
width. Their ratio is controlled by the frustration of the spin system. By this
work, theoretical and experimental results can be reconciled in two important
points.Comment: 9 pages, 5 figures included, Revtex submitted to Physical Review
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