743 research outputs found
Magnetic circular dichroism in X-ray fluorescence of Heusler alloys at threshold excitation
The results of fluorescence measurements of magnetic circular dichroism (MCD)
in Mn L_2,L_3 X-ray emission and absorption for Heusler alloys NiMnSb and
Co2MnSb are presented. Very intense resonance Mn L_3 emission is found at the
Mn 2p_3/2 threshold and is attributed to a peculiarity of the threshold
excitation in materials with the half-metallic character of the electronic
structure. A theoretical model for the description of resonance scattering of
polarized x-rays is suggested.Comment: 3 pages, 2 figures. Discussed at conferences, submitting process in
progres
Electronic structure investigation of CoO by means of soft X-ray scattering
The electronic structure of CoO is studied by resonant inelastic soft X-ray
scattering spectroscopy using photon energies across the Co 2p absorption
edges. The different spectral contributions from the energy-loss structures are
identified as Raman scattering due to d-d and charge-transfer excitations. For
excitation energies close to the L3 resonance, the spectral features are
dominated by quartet-quartet and quartet-doublet transitions of the 3d7
configuration. At excitation energies corresponding to the satellites in the Co
2p X-ray absorption spectrum of CoO, the emission features are instead
dominated by charge-transfer transitions to the 3d8L-1 final state. The spectra
are interpreted and discussed with the support of simulations within the single
impurity Anderson model with full multiplet effects which are found to yield
consistent spectral functions to the experimental data.Comment: 8 pages, 2 figures, 2 tables,
http://link.aps.org/doi/10.1103/PhysRevB.65.20510
Large magnetic circular dichroism in resonant inelastic x-ray scattering at the Mn L-edge of Mn-Zn ferrite
We report resonant inelastic x-ray scattering (RIXS) excited by circularly
polarized x-rays on Mn-Zn ferrite at the Mn L2,3-resonances. We demonstrate
that crystal field excitations, as expected for localized systems, dominate the
RIXS spectra and thus their dichroic asymmetry cannot be interpreted in terms
of spin-resolved partial density of states, which has been the standard
approach for RIXS dichroism. We observe large dichroic RIXS at the L2-resonance
which we attribute to the absence of metallic core hole screening in the
insulating Mn-ferrite. On the other hand, reduced L3-RIXS dichroism is
interpreted as an effect of longer scattering time that enables spin-lattice
core hole relaxation via magnons and phonons occurring on a femtosecond time
scale.Comment: 7 pages, 2 figures,
http://link.aps.org/doi/10.1103/PhysRevB.74.17240
A High-Resolution Study of the HI Content of Local Group Dwarf Irregular Galaxy WLM
Dwarf irregular galaxies are unique laboratories for studying the interaction
between stars and the interstellar medium in low mass environments. We present
the highest spatial resolution observations to date of the neutral hydrogen
content of the Local Group dwarf irregular galaxy WLM. We find that WLM's
neutral hydrogen distribution is typical for a galaxy of its type and size and
derive an HI mass of 6.3e7 Msun for WLM. In addition, we derive an HI extent
for WLM of 30 arcmin, which is much less than the 45 arcmin extent found by
Huchtmeier, Seiradakis, and Materne (1981). We show that the broken ring of
high column density neutral hydrogen surrounding the center of WLM is likely
the result of star formation propagating out from the center of the galaxy. The
young stars and Ha emission in this galaxy are mostly correlated with the high
column density neutral hydrogen. The gap in the central ring is the result of
star formation in that region using up, blowing out, or ionizing all of the
neutral hydrogen. Like many late-type galaxies, WLM's velocity field is
asymmetric with the approaching (northern) side appearing to be warped and a
steeper velocity gradient for the approaching side than for the receding side
in the inner region of the galaxy. We derive a dynamical mass for WLM of 2.16e9
Msun.Comment: 38 pages, 15 figures, 5 tables, accepted by AJ, high resolution
version at http://www.astro.wisc.edu/~kepley/kepley_wlm.p
Theoretical Limb Darkening for Classical Cepheids: II. Corrections for the Geometric Baade-Wesselink Method
The geometric Baade-Wesselink method is one of the most promising techniques
for obtaining a better calibration of the Cepheid period-luminosity relation by
means of interferometric measurements of accurate diameters. In this paper we
present new wavelength- and phase-dependent limb darkening corrections based on
our time-dependent hydrodynamic models of the classical Cepheid zeta Gem. We
show that a model simulation of a Cepheid atmosphere, taking into account the
hydrodynamic effects associated with the pulsation, shows strong departures
from the limb darkening otherwise predicted by a static model. For most of its
pulsational cycle the hydrodynamic model predicts a larger limb darkening then
the equivalent static model. The hydrodynamics affects the limb darkening
mainly at UV and optical wavelengths. Most of these effects evolve slowly as
the star pulsates, but there are phases, associated with shocks propagating
into the photosphere, in which significant changes in the limb darkening take
place on time-scales of the order of less than a day. We assess the implication
of our model LD corrections fitting the geometric Baade-Wesselink distance of
zeta Gem for the available near-IR PTI data. We discuss the effects of our
model limb darkening on the best fit result, and analyze the requirements
needed to test the time-dependence of the limb darkening with future
interferometric measurements.Comment: 22 pages, 5 figures, to be published on the Astrophysical Journal,
June 1 2003 issu
Electronic structure and chemical bonding in Ti4SiC3 investigated by soft x-ray emission spectroscopy and first principle theory
The electronic structure in the new transition metal carbide Ti4SiC3 has been
investigated by bulk-sensitive soft x-ray emission spectroscopy and compared to
the well-studied Ti3SiC2 and TiC systems. The measured high-resolution Ti L, C
K and Si L x-ray emission spectra are discussed with ab initio calculations
based on density-functional theory including core-to-valence dipole matrix
elements. The detailed investigations of the Ti-C and Ti-Si chemical bonds
provide increased understanding of the physical properties of these
nanolaminates. A strongly modified spectral shape is detected for the buried Si
monolayers due to Si 3p hybridization with the Ti 3d orbitals. As a result of
relaxation of the crystal structure and the charge-transfer from Ti (and Si) to
C, the strength of the Ti-C covalent bond is increased. The differences between
the electronic and crystal structures of Ti4SiC3 and Ti3SiC2 are discussed in
relation to the number of Si layers per Ti layer in the two systems and the
corresponding change of materials properties.Comment: 12 pages, 7 figures, 1 tabl
Resonant soft X-ray Raman scattering of NiO
Resonant soft X-ray Raman scattering measurements on NiO have been made at
photon energies across the Ni 2p absorption edges. The details of the spectral
features are identified as Raman scattering due to d-d and charge-transfer
excitations. The spectra are interpreted within the single impurity Anderson
model, including multiplets, crystal-field and charge-transfer effects. At
threshold excitation, the spectral features consists of triplet-triplet and
triplet-singlet transitions of the 3d8 configuration. For excitation energies
corresponding to the charge-transfer region in the Ni 2p X-ray absorption
spectrum of NiO, the emission spectra are instead dominated by charge-transfer
transitions to the 3d9L-1 final state. Comparisons of the final states with
other spectroscopical techniques are also made.Comment: 9 pages, 2 figures, 2 tables,
http://iopscience.iop.org/0953-8984/14/13/32
Doping Dependent Changes in Nitrogen 2 States in the Diluted Magnetic Semiconductor GaCrN
We study the electronic structure of the recently discovered diluted magnetic
semiconductor GaCrN ( = 0.01-0.10). A systematic study of the
changes in the and ligand (N) partial density of states
(DOS) of the host lattice is carried out using N 1 soft x-ray emission and
absorption spectroscopy, respectively. X-ray absorption measurements confirm
the wurtzite N 2 DOS and substitutional doping of Cr into Ga-sites. Coupled
changes in the and N 2 character DOS of
GaCrN identify states responsible for ferromagnetism consistent
with band structure calculations.Comment: 5 pages, 4 figures, submitted to Phys. Rev.
Electronic structure investigation of CeB6 by means of soft X-ray scattering
The electronic structure of the heavy fermion compound CeB6 is probed by
resonant inelastic soft X-ray scattering using photon energies across the Ce 3d
and 4d absorption edges. The hybridization between the localized 4f orbitals
and the delocalized valence-band states is studied by identifying the different
spectral contributions from inelastic Raman scattering and normal fluorescence.
Pronounced energy-loss structures are observed below the elastic peak at both
the 3d and 4d thresholds. The origin and character of the inelastic scattering
structures are discussed in terms of charge-transfer excitations in connection
to the dipole allowed transitions with 4f character. Calculations within the
single impurity Anderson model with full multiplet effects are found to yield
consistent spectral functions to the experimental data.Comment: 9 pages, 4 figures, 1 table,
http://link.aps.org/doi/10.1103/PhysRevB.63.07510
Observation of Strong Resonant Behavior in the Inverse Photoelectron Spectroscopy of Ce Oxide
X-ray emission spectroscopy and resonant inverse photoelectron spectroscopy (RIPES) have been used to investigate the photon emission associated with the Ce 3d5/2 and Ce 3d3/2 thresholds. Strong resonant behavior has been observed in the RIPES of a Ce oxide near the 5/2 and 3/2 edges
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